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Non-equilibrium dynamics of multi-orbital system under time-depending electric field

時間変動する電場の下での多軌道系の非平衡ダイナミクス

大西 弘明  

Onishi, Hiroaki

We investigate the real-time dynamics under time-depending electric fields in a one-dimensional orbital degenerate Hubbard model, using a time-dependent density matrix renormalization group method. Considering a chain along the $$z$$ direction with $$e_{rm g}$$-orbital degrees of freedom on each site, electrons preferably occupy itinerant $$d_{3z^2-r^2}$$ orbitals rather than localized $$d_{x^2-y^2}$$ orbitals to gain kinetic energy. Thus, in the ground state at quarter filling, $$d_{3z^2-r^2}$$ orbital is singly occupied, while the spin state exhibits antiferromagnetic correlations for small Hund's rule coupling. After the oscillating electric field is turned on, holon-doublon pairs are introduced when the frequency of the applied electric field exceeds a charge excitation gap. During the time evolution, the ferro-orbital state is deformed due to the pair-hopping interaction that is characteristic of multi-orbital systems.

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