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system and integration with JAEA's thermodynamic database for geochemical calculationsThe latest available thermodynamic data were critically reviewed and the selected values were included into the JAEA-TDB for performance assessment of geological disposal of high-level radioactive and TRU wastes. This critical review specifically addressed thermodynamic data for (1) a zirconium-hydroxide system through comparison of thermodynamic data selected by the Nuclear Energy Agency within the Organisation for Economic Co-operation and Development (OECD/NEA), (2) complexation of metal ions with isosaccharinic acid based on the latest review papers. Furthermore, the author performed (3) tentative selection of thermodynamic data on ternary complexes among alkaline-earth metal, uranyl and carbonate ions, and (4) integration with the latest version of JAEA's thermodynamic database for geochemical calculations. The internal consistency of the selected data was checked by the author. Text files of the updated and integrated thermodynamic database have been prepared for geochemical calculation programs of PHREEQC and Geochemist's Workbench.
Language |
: | English |
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Report No. |
: | JAEA-Data/Code 2018-018 |
Pages |
: | 103 Pages |
Publication Year/Month |
: | 2019/03 |
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Paper URL |
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Keywords |
: | Geological Disposal; High-level Radioactive Waste; TRU Waste; Thermodynamic Database; Update of JAEA-TDB; Zirconium; Isosaccharinate; Uranium(VI); Geochemical Calculation |
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