Overview of development program for engineering scale extraction chromatography MA(III) recovery system

Watanabe, So; Takahatake, Yoko; Hasegawa, Kenta; Goto, Ichiro*; Miyazaki, Yasunori; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki

Mechanical Engineering Journal (Internet), 11(2), p.23-00461_1 - 23-00461_10, 2024/04

https://doi.org/10.1299/mej.23-00461

Development of coupling technology for high temperature gas-cooled reactors and hydrogen production facility; HTTR heat application test project plan

Ishii, Katsunori; Morita, Keisuke; Noguchi, Hiroki; Aoki, Takeshi; Mizuta, Naoki; Hasegawa, Takeshi; Nagatsuka, Kentaro; Nomoto, Yasunobu; Shimizu, Atsushi; Iigaki, Kazuhiko; et al.

Dai-27-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (Internet), 4 Pages, 2023/09

https://doi.org/10.1299/jsmepes.2023.27.A242

Kinetic mass transfer behavior of Eu(III) in nitrilotriacetamide-impregnated polymer-coated silica particles

Miyagawa, Akihisa*; Hayashi, Naoki*; Kuzure, Yoshiaki*; Takahashi, Takumi*; Iwamoto, Hibiki*; Arai, Tsuyoshi*; Nagatomo, Shigenori*; Miyazaki, Yasunori; Hasegawa, Kenta; Sano, Yuichi; et al.

Bulletin of the Chemical Society of Japan, 96(7), p.671 - 676, 2023/07

https://doi.org/10.1246/bcsj.20230087

We investigated the distribution mechanism of Eu(III) in a single polymer-coated silica particle including nitrilotriacetamide (NTA) extractants known as HONTA and TOD2EHNTA. The present study provides a valuable approach for the evaluation and enhancement of the functionality of "single extractant-impregnated polymer-coated silica particle".

Development of engineering scale extraction chromatography separation system, 2; Spray drying granulation of silica support for adsorbent

Hasegawa, Kenta; Goto, Ichiro*; Miyazaki, Yasunori; Ambai, Hiromu; Watanabe, So; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 5 Pages, 2023/05

Phase transition and domain formation in ferroaxial crystals

Hayashida, Takeshi*; Uemura, Yohei*; Kimura, Kenta*; Matsuoka, Satoshi*; Hagihara, Masato; Hirose, Sakyo*; Morioka, Hitoshi*; Hasegawa, Tatsuo*; Kimura, Tsuyoshi*

Physical Review Materials (Internet), 5(12), p.124409_1 - 124409_10, 2021/12

https://doi.org/10.1103/PhysRevMaterials.5.124409

Verification of dose estimation of Auger electrons emitted from Cu-64 using a combination of FNTD measurements and Monte Carlo simulations

Kusumoto, Tamon*; Matsuya, Yusuke; Baba, Kentaro*; Ogawara, Ryo*; Akselrod, M. S.*; Harrison, J.*; Fomenko, V.*; Kai, Takeshi; Ishikawa, Masayori*; Hasegawa, Sumitaka*; et al.

Radiation Measurements, 132, p.106256_1 - 106256_4, 2020/03

https://doi.org/10.1016/j.radmeas.2020.106256

Internal radiation therapy with Cu-64 concentrates energy deposition in tumor cells by virtue of released Auger electrons with low energy. In our previous study, we have attached the solutions at the surface of Fluorescent Nuclear Track Detector (FNTD) and succeeded in measuring the absorbed doses of Auger electrons registered in FNTD. However, because there are several types of radiation emitted from the source, i.e., beta rays, positron etc., the contribution degree of Auger electron to energy concentration remain uncertain. In this study, we quantitatively analyzed the spatial dose distribution in the FNTD based on Monte Carlo simulation with PHITS and GEANT4, and evaluated high dose deposited by Auger electrons. The dose distribution calculated by the PHITS code is exactly equivalent to that by Geant4. Also, the simulations are well agreement with experimental results. If the contribution of Auger electrons is ignored, the significantly high absorbed dose proximal to the source is not properly reduced. These findings demonstrate that Auger electrons work very effectively to kill cancer cells proximal to Cu-64 source while minimizing damage effects on normal cells distal to the source.

Negative muonium ion production with a C12A7 electride film

Otani, Masashi*; Fukao, Yoshinori*; Futatsukawa, Kenta*; Kawamura, Naritoshi*; Matoba, Shiro*; Mibe, Tsutomu*; Miyake, Yasuhiro*; Shimomura, Koichiro*; Yamazaki, Takayuki*; Hasegawa, Kazuo; et al.

Journal of Physics; Conference Series, 1350, p.012067_1 - 012067_6, 2019/12

https://doi.org/10.1088/1742-6596/1350/1/012067

Negative muonium atom (ee, Mu) has unique features stimulating potential interesting for several scientific fields. Since its discovery in late 1980's in vacuum, it has been discussed that the production efficiency would be improved using a low-work function material. C12A7 was a well-known insulator as a constituent of alumina cement, but was recently confirmed to exhibit electric conductivity by electron doping. The C12A7 electride has relatively low-work function (2.9 eV). In this paper, the negative muonium production measurement with several materials including a C12A7 electride film will be presented. Measured production rate of the Mu were 10/s for all the Al, electride, and SUS target. Significant enhancement on electride target was not observed, thus it is presumed that the surface condition should be more carefully treated. There was no material dependence of the Mu averaged energy: it was 0.20.1keV.

Bunch size measurement with high time resolution for RF accelerated muon beam

Sue, Yuki*; Iijima, Toru*; Inami, Kenji*; Yotsuzuka, Mai*; Iinuma, Hiromi*; Nakazawa, Yuga*; Otani, Masashi*; Kawamura, Naritoshi*; Shimomura, Koichiro*; Futatsukawa, Kenta*; et al.

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.55 - 60, 2019/07

https://www.pasj.jp/web_publish/pasj2019/proceedings/PDF/WEOI/WEOI05.pdf

The result of bunch size measurement of muon accelerated by RFQ up to 89 keV is presented in this paper. A four-stage muon linac for precise measurement of muon property is under construction in the J-PARC. The demonstration of the first muon RF acceleration with an RFQ linac was conducted and the transverse profile of the accelerated muons was measured in 2017. As one of the remaining issues for the beam diagnostic system, the longitudinal beam profile after the RFQ should be measured to match the profile to the designed acceptance of the subsequent accelerator. For this purpose, the new longitudinal beam monitor using the microchannel plate is under development. The time resolution of the monitor aims to be around 30 to 40 ps corresponding to 1% of a period of an operating frequency of the accelerator, which is 324 MHz. On November 2018, the bunch size of accelerated negative muonium ion of 89 keV with the RFQ was measured using this monitor at the J-PARC MLF. The measured bunch width is ns, which is consistent with the simulation.

Development of the longitudinal beam monitor with high time resolution for a muon linac in the J-PARC E34 experiment

Yotsuzuka, Mai*; Iijima, Toru*; Inami, Kenji*; Sue, Yuki*; Iinuma, Hiromi*; Nakazawa, Yuga*; Saito, Naohito; Hasegawa, Kazuo; Kondo, Yasuhiro; Kitamura, Ryo; et al.

Proceedings of 10th International Particle Accelerator Conference (IPAC '19) (Internet), p.2571 - 2574, 2019/06

https://doi.org/10.18429/JACoW-IPAC2019-WEPGW042

The J-PARC E34 experiment aims to measure the muon anomalous magnetic moment and the electric dipole moment with a high precision. In this experiment, thermal muonium is produced and ionized by laser resonance to generate ultra-slow muons, which are then accelerated in a multistage muon linac. In order to satisfy the experimental requirements, suppression of the emittance growth during the acceleration is necessary. Because the main cause of the emittance growth is beam mismatching between the accelerating stages, the transverse and longitudinal beam monitoring is important. The longitudinal beam monitor has to measure the bunch length with the resolution equivalent to tens of picoseconds, which is 1% of the acceleration phase of 324 MHz. In addition, it should be sensitive to single muon because the beam intensity is limited during the commissioning phase. To realize above requirements, we are developing a longitudinal beam monitor with a micro channel plate, and the test bench to evaluate the monitor performance. So far, the time resolution of the beam monitor was obtained to be 65 ps in RMS including the jitter on the test bench. We also succeeded in measuring the longitudinal bunch size of the muon beam accelerated by RFQ using the beam monitor. Further improvement of the measurement system is needed to guarantee the required accuracy. In this paper, the results of the performance evaluation for this beam monitor are reported.

Muon profile measurement after acceleration with a radio-frequency quadrupole linac

Otani, Masashi*; Sue, Yuki*; Fukao, Yoshinori*; Futatsukawa, Kenta*; Kawamura, Naritoshi*; Mibe, Tsutomu*; Miyake, Yasuhiro*; Shimomura, Koichiro*; Yamazaki, Takayuki*; Iijima, Toru*; et al.

Journal of Physics; Conference Series, 1067(5), p.052012_1 - 052012_7, 2018/09

https://doi.org/10.1088/1742-6596/1067/5/052012

We have measured the muon beam profile after acceleration using a radio frequency quadrupole linac (RFQ). Positive muons are injected to an aluminum degrader and negative muoniums (Mu) are generated. The generated Mus are extracted by an electrostatic lens and accelerated to 89 keV by the RFQ. The accelerated Mus are transported to a beam profile monitor (BPM) through a quadrupole magnet pair and a bending magnet. The BPM consists of a micro-channel plate, a phospher screen, and a CCD camera. Measured profile in the vertical direction is consistent to the simulation. This profile measurement is one of milestones for realizing a muon linac for measurement of the muon anomalous magnetic moment at the Japan Proton Accelerator Research Complex.