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Yakushev, A.*; Lens, L.*; Dllmann, Ch. E.*; Khuyagbaatar, J.*; Jger, E.*; Krier, J.*; Runke, J.*; Albers, H. M.*; 浅井 雅人; Block, M.*; et al.
Frontiers in Chemistry (Internet), 10, p.976635_1 - 976635_11, 2022/08
被引用回数:8 パーセンタイル:81.08(Chemistry, Multidisciplinary)114番元素フレロビウム(Fl)は現在その化学的性質が研究されている最も重い元素である。Flに関する最初の化学実験では、Flは貴ガス的な性質を持つ元素であると報告された。一方、2番目の研究では、Flは揮発性金属の性質を示すと報告された。より信頼性の高い結論を得るため、我々は更なる実験的研究を行い、二酸化ケイ素と金表面におけるFlの吸着挙動を調べた。その結果、Flは揮発性金属の水銀よりも高い揮発性と低い反応性を示し、一方、貴ガスのラドンよりは反応性が高いことを明らかにした。
Brunet, M.*; Podolyk, Zs.*; Berry, T. A.*; Brown, B. A.*; Carroll, R. J.*; Lica, R.*; Sotty, Ch.*; Andreyev, A. N.; Borge, M. J. G.*; Cubiss, J. G.*; et al.
Physical Review C, 103(5), p.054327_1 - 054327_13, 2021/05
被引用回数:2 パーセンタイル:58.42(Physics, Nuclear)The structure of Po populated through the EC/ decay of At is investigated using -ray spectroscopy at the ISOLDE Decay Station. The presented level scheme contains 27 new excited states and 43 new transitions, as well as a further 50 previously observed rays which have been (re)assigned a position. Through the analysis using the shell model calculations approximately half of the -decay strength of At is found to proceed via allowed decay and half via first-forbidden decay. The first-forbidden transitions predominantly populate core excited states at high excitation energies, which is qualitatively understood using shell model considerations.
Berry, T. A.*; Podolyk, Zs.*; Carroll, R. J.*; Lic, R.*; Grawe, H.*; Timofeyuk, N. K.*; Alexander, T.*; Andreyev, A. N.; Ansari, S.*; Borge, M. J. G.*; et al.
Physics Letters B, 793, p.271 - 275, 2019/06
被引用回数:5 パーセンタイル:48.53(Astronomy & Astrophysics)Gamow-Teller decay is forbidden if the number of nodes in the radial wave functions of the initial and final states is different. This = 0 requirement plays a major role in the decay of heavy neutron-rich nuclei, affecting the nucleosynthesis through the increased half-lives of nuclei on the astrophysical -process pathway below both = 50 (for 82) and = 82 (for 126). The level of forbiddenness of the = 1 10 transition has been investigated from the decay of the ground state of Hg into the single-proton-hole nucleus Tl in an experiment at the ISOLDE Decay Station. From statistical observational limits on possible -ray transitions depopulating the 0 state in Tl, an upper limit of 3.910 % was obtained for the probability of this decay, corresponding to log 8.8 within a 95% confidence limit. This is the most stringent test of the = 0 selection rule to date.
Lens, L.*; Yakushev, A.*; Dllmann, Ch. E.*; 浅井 雅人; Ballof, J.*; Block, M.*; David, H. M.*; Despotopulos, J.*; Di Nitto, A.*; Eberhardt, K.*; et al.
Radiochimica Acta, 106(12), p.949 - 962, 2018/12
被引用回数:6 パーセンタイル:63.44(Chemistry, Inorganic & Nuclear)半減期449秒の短寿命同位体を用いて、水銀(Hg), タリウム(Tl), 鉛(Pb)の単一原子レベルでのSiO及びAu表面への固体吸着挙動をオンライン気相実験により調べた。超重元素Cn, Nh, Flの吸着エンタルピー測定のためのモデル実験として実施した。短寿命同位体はドイツ重イオン研究所の反跳核分離装置TASCAを用いて生成・分離した。生成核はヘリウムガス中に捕集された後、SiOあるいはAuで表面を覆われたSi検出器で作製されたガスクロマトグラフィーカラムへと導入した。短寿命Tl及びPb同位体は室温においてSiO表面に吸着し、Si検出器で測定することに成功した。一方、HgはSiO表面には吸着せず、Au表面に吸着した。この結果より、本実験のセットアップを用いることで短寿命Hg, Tl, Pb同位体の吸着特性を調べることができると証明され、この手法がCn, Nh, Flの実験にも適用できることが確認された。
Lund, M. V.*; Andreyev, A. N.; Borge, M. J. G.*; Cederkll, J.*; De Witte, H.*; Fraile, L. M.*; Fynbo, H. O. U.*; Greenlees, P. T.*; Harkness-Brennan, L. J.*; Howard, A. M.*; et al.
European Physical Journal A, 52(10), p.304_1 - 304_14, 2016/10
被引用回数:16 パーセンタイル:75.97(Physics, Nuclear)Beta-delayed proton emission from Mg has been measured at ISOLDE, CERN, with the ISOLDE Decay Station setup including both charged-particle and -ray detection capabilities. A total of 27 delayed proton branches were measured including seven so far unobserved. An updated decay scheme, including three new resonances above the proton separation energy in Na and more precise resonance energies, is presented. Beta-decay feeding to two resonances above the Isobaric Analogue State in Na is observed. This may allow studies of the 4032.9(2.4) keV resonance in Ne through the beta decay of Mg, which is important for the astrophysically relevant reaction O(,)Ne. Beta-delayed protons were used to obtain a more precise value for the half-life of Mg, 91.4(1.0) ms.
Lic, R.*; Mach, H.*; Fraile, L. M.*; Gargano, A.*; Borge, M. J. G.*; Mrginean, N.*; Sotty, C. O.*; Vedia, V.*; Andreyev, A. N.; Benzoni, G.*; et al.
Physical Review C, 93(4), p.044303_1 - 044303_7, 2016/04
被引用回数:5 パーセンタイル:39.74(Physics, Nuclear)The levels in Sn populated from the decay of In isomers were investigated at the ISOLDE facility of CERN using the newly commissioned ISOLDE Decay Station. The lowest 1/2 state and the 3/2 ground state in Sn are expected to have configurations dominated by the neutron (=0) and (=2) single-particle states, respectively. Consequently, these states should be connected by a somewhat slow -forbidden transition. Using fast-timing spectroscopy we have measured the half-life of the 1/2 315.3-keV state, = 19(10) ps, which corresponds to a moderately fast transition. Shell-model calculations using the CD-Bonn effective interaction, with standard effective charges and factors, predict a 4-ns half-life for this level. We can reconcile the shell-model calculations to the measured value by the renormalization of the effective operator for neutron holes.