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Journal Articles

In situ neutron imaging of lithium-ion batteries during heating to thermal runaway

Nozaki, Hiroshi*; Kondo, Hiroki*; Shinohara, Takenao; Setoyama, Daigo*; Matsumoto, Yoshihiro*; Sasaki, Tsuyoshi*; Isegawa, Kazuhisa*; Hayashida, Hirotoshi*

Scientific Reports (Internet), 13, p.22082_1 - 22082_8, 2023/12

 Times Cited Count:0 Percentile:0(Multidisciplinary Sciences)

Journal Articles

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Chazono, Yoshiki*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

 Times Cited Count:1 Percentile:64.66(Astronomy & Astrophysics)

Gamma decays were observed in $$^{56}$$Ca and $$^{58}$$Ca following quasi-free one-proton knockout reactions from $$^{57,59}$$Sc. For $$^{56}$$Ca, a $$gamma$$ ray transition was measured to be 1456(12) keV, while for $$^{58}$$Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the $$2^{+}_{1} rightarrow 0^{+}_{gs}$$ decays. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for $$2^{+}_{1}$$ level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the N = 34 shell. Its constituents, the $$0_{f5/2}$$ and $$0_{g9/2}$$ orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic $$^{60}$$Ca and potentially drives the dripline of Ca isotopes to $$^{70}$$Ca or even beyond.

Journal Articles

The Formation mechanism of radiocesium-bearing microparticles derived from the Fukushima Daiichi Nuclear Power Plant using electron microscopy

Hagiwara, Hiroki; Kondo, Keietsu; Hidaka, Akihide

Journal of Radioanalytical and Nuclear Chemistry, 331(12), p.5905 - 5914, 2022/12

 Times Cited Count:3 Percentile:50.96(Chemistry, Analytical)

Journal Articles

"Southwestern" boundary of the $$N = 40$$ island of inversion; First study of low-lying bound excited states in $$^{59}$$V and $$^{61}$$V

Elekes, Z.*; Juh$'a$sz, M. M.*; Sohler, D.*; Sieja, K.*; Yoshida, Kazuki; Ogata, Kazuyuki*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; Baba, Hidetada*; et al.

Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12

 Times Cited Count:2 Percentile:49.92(Physics, Nuclear)

The low-lying level structure of $$^{59}$$V and $$^{61}$$V was investigated for the first time. The neutron knockout reaction and inelastic proton scattering were applied for $$^{61}$$V while the neutron knock-out reaction provided the data for $$^{59}$$V. Four and five new transitions were determined for $$^{59}$$V and $$^{61}$$V, respectively. Based on the comparison to our shell-model calculations using the Lenzi-Nowacki-Poves-Sieja (LNPS) interaction, three of the observed $$gamma$$ rays for each isotope could be placed in the level scheme and assigned to the decay of the first 11/2$$^{-}$$ and 9/2$$^{-}$$ levels. The ($$p$$,$$p'$$) excitation cross sections for $$^{61}$$V were analyzed by the coupled-channels formalism assuming quadrupole plus hexadecapole deformations. Due to the role of the hexadecapole deformation, $$^{61}$$V could not be unambiguously placed on the island of inversion.

Journal Articles

Extended $$p_{3/2}$$ neutron orbital and the $$N = 32$$ shell closure in $$^{52}$$Ca

Enciu, M.*; Liu, H. N.*; Obertelli, A.*; Doornenbal, P.*; Nowacki, F.*; Ogata, Kazuyuki*; Poves, A.*; Yoshida, Kazuki; Achouri, N. L.*; Baba, Hidetada*; et al.

Physical Review Letters, 129(26), p.262501_1 - 262501_7, 2022/12

 Times Cited Count:5 Percentile:65.23(Physics, Multidisciplinary)

The one-neutron knockout from $$^{52}$$Ca was performed at $$sim$$230 MeV/nucleon combined with prompt $$gamma$$ spectroscopy. The momentum distributions corresponding to the removal of $$1f_{7/2}$$ and $$2p_{3/2}$$ neutrons were measured. The cross sections are consistent with a shell closure at the neutron number $$N = 32$$, found as strong as at $$N = 28$$ and $$N = 34$$ in Ca isotopes from the same observables. The analysis of the momentum distributions leads to a difference of the root-mean-square radii of the neutron $$1_{f7/2}$$ and $$2p_{3/2}$$ orbitals of 0.61(23) fm, in agreement with the modified-shell-model prediction of 0.7 fm suggesting that the large root-mean-square radius of the $$2p_{3/2}$$ orbital in neutron-rich Ca isotopes is responsible for the unexpected linear increase of the charge radius with the neutron number.

Journal Articles

Beam physics design of a 30-MW beam transport to the target for an accelerator-driven subcritical system

Yee-Rendon, B.; Meigo, Shinichiro; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Iwamoto, Hiroki; Sugawara, Takanori; Nishihara, Kenji

Journal of Instrumentation (Internet), 17(10), p.P10005_1 - P10005_21, 2022/10

 Times Cited Count:0 Percentile:0(Instruments & Instrumentation)

To reduce the hazard of minor actinides in nuclear waste, JAEA proposed an accelerator-driven subcritical system (JAEA-ADS). The JAEA-ADS drives a subcritical reactor 800-MWth by 30-MW proton linac delivering the beam to the spallation neutron target inside the reactor. The beam transport to the target (BTT) is required for high-beam power stability and low peak density to ensure the integrity of the beam window. Additionally, the design should have compatible with the reactor design for the maintenance and replacement of the fuel and the beam window. A robust-compact BTT design was developed through massive multiparticle simulations. The beam optics was optimized to guarantee beam window feasibility requirements by providing a low peak density of less than 0.3 $$mu$$A/mm$$^2$$. Beam stability was evaluated and improved by simultaneously applying the linac's input beam and element errors. The input beam errors to the reactor were based on the beam degradation obtained by implementing fast fault compensation in the linac. Those results show that the BTT fulfills the requirements for JAEA-ADS.

Journal Articles

Status of decommissioning for prototype ATR Fugen and FBR Monju

Ito, Kenji; Kondo, Tetsuo; Nakamura, Yasuyuki; Matsuno, Hiroki; Nagaoki, Yoshihiro; Sakuma, Yuichi

Dekomisshoningu Giho, (63), p.1 - 26, 2022/05

The prototype advanced thermal reactor Fugen entered into the decommissioning phases with the approval of the decommissioning plan in February 2008. The prototype fast breeder reactor Monju entered into the decommissioning stage with the approval of the decommissioning plan in March 2018. In April 2018, the head office of Tsuruga decommissioning demonstration was newly established to oversee the decommissioning operations in Tsuruga area, and decommissioning projects for two unique reactors have progressed safely and steadily.

Journal Articles

A First glimpse at the shell structure beyond $$^{54}$$Ca; Spectroscopy of $$^{55}$$K, $$^{55}$$Ca, and $$^{57}$$Ca

Koiwai, Takuma*; Wimmer, K.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Duguet, T.*; Holt, J. D.*; Miyagi, Takayuki*; Navr$'a$til, P.*; Ogata, Kazuyuki*; et al.

Physics Letters B, 827, p.136953_1 - 136953_7, 2022/04

 Times Cited Count:4 Percentile:74.12(Astronomy & Astrophysics)

no abstracts in English

Journal Articles

Pairing forces govern population of doubly magic $$^{54}$$Ca from direct reactions

Browne, F.*; Chen, S.*; Doornenbal, P.*; Obertelli, A.*; Ogata, Kazuyuki*; Utsuno, Yutaka; Yoshida, Kazuki; Achouri, N. L.*; Baba, Hidetada*; Calvet, D.*; et al.

Physical Review Letters, 126(25), p.252501_1 - 252501_7, 2021/06

 Times Cited Count:10 Percentile:74.2(Physics, Multidisciplinary)

Direct proton-knockout reactions of $$^{55}$$Sc were studied at the RIKEN Radioactive Isotope Beam Factory. Populated states of $$^{54}$$Ca were investigated through $$gamma$$-ray and invariant-mass spectroscopy. Level energies were calculated from the nuclear shell model employing a phenomenological inter-nucleon interaction. Theoretical cross sections to states were calculated from distorted-wave impulse approximation estimates multiplied by the shell model spectroscopic factors. Despite the calculations showing a significant amplitude of excited neutron configurations in the ground-state of $$^{55}$$Sc, valence proton removals populated predominantly the ground-state of $$^{54}$$Ca. This counter-intuitive result is attributed to pairing effects leading to a dominance of the ground-state spectroscopic factor. Owing to the ubiquity of the pairing interaction, this argument should be generally applicable to direct knockout reactions from odd-even to even-even nuclei.

Journal Articles

First spectroscopic study of $$^{51}$$Ar by the ($$p$$,2$$p$$) reaction

Juh$'a$sz, M. M.*; Elekes, Z.*; Sohler, D.*; Utsuno, Yutaka; Yoshida, Kazuki; Otsuka, Takaharu*; Ogata, Kazuyuki*; Doornenbal, P.*; Obertelli, A.*; Baba, Hidetada*; et al.

Physics Letters B, 814, p.136108_1 - 136108_8, 2021/03

AA2020-0747.pdf:0.83MB

 Times Cited Count:5 Percentile:63.69(Astronomy & Astrophysics)

The nuclear structure of $$^{51}$$Ar was studied by the ($$p$$,2$$p$$) reaction using $$gamma$$-ray spectroscopy for the bound and unbound states. Comparing the results to our shell-model calculations, two bound and six unbound states were established. The low cross sections populating the two bound states of $$^{51}$$Ar could be interpreted as a clear signature for the presence of significant sub-shell closures at neutron numbers 32 and 34 in argon isotopes.

Journal Articles

High temperature gas-cooled reactors

Takeda, Tetsuaki*; Inagaki, Yoshiyuki; Aihara, Jun; Aoki, Takeshi; Fujiwara, Yusuke; Fukaya, Yuji; Goto, Minoru; Ho, H. Q.; Iigaki, Kazuhiko; Imai, Yoshiyuki; et al.

High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02

As a general overview of the research and development of a High Temperature Gas-cooled Reactor (HTGR) in JAEA, this book describes the achievements by the High Temperature Engineering Test Reactor (HTTR) on the designs, key component technologies such as fuel, reactor internals, high temperature components, etc., and operational experience such as rise-to-power tests, high temperature operation at 950$$^{circ}$$C, safety demonstration tests, etc. In addition, based on the knowledge of the HTTR, the development of designs and component technologies such as high performance fuel, helium gas turbine and hydrogen production by IS process for commercial HTGRs are described. These results are very useful for the future development of HTGRs. This book is published as one of a series of technical books on fossil fuel and nuclear energy systems by the Power Energy Systems Division of the Japan Society of Mechanical Engineers.

Journal Articles

$$N$$ = 32 shell closure below calcium; Low-lying structure of $$^{50}$$Ar

Cort$'e$s, M. L.*; Rodriguez, W.*; Doornenbal, P.*; Obertelli, A.*; Holt, J. D.*; Men$'e$ndez, J.*; Ogata, Kazuyuki*; Schwenk, A.*; Shimizu, Noritaka*; Simonis, J.*; et al.

Physical Review C, 102(6), p.064320_1 - 064320_9, 2020/12

AA2020-0748.pdf:0.75MB

 Times Cited Count:11 Percentile:78.75(Physics, Nuclear)

Low-lying excited states in the $$N$$ = 32 isotope $$^{50}$$Ar were investigated by in-beam $$gamma$$-ray spectroscopy following proton- and neutron-knockout, multinucleon removal, and proton inelastic scattering at the RIKEN Radioactive Isotope Beam Factory. The energies of the two previously reported transitions have been confirmed, and five additional states are presented for the first time, including a candidate for a 3$$^{-}$$ state. The level scheme built using $$gamma$$ $$gamma$$ coincidences was compared to shell-model calculations in the $$sd-pf$$ model space and to ${it ab initio}$ predictions based on chiral two- and three-nucleon interactions. Theoretical proton- and neutron-knockout cross sections suggest that two of the new transitions correspond to 2$$^{+}$$ states, while the previously proposed 4$$^{+}_{1}$$ state could also correspond to a 2$$^{+}$$ state.

Journal Articles

High-temperature short-range order in Mn$$_3$$RhSi

Yamauchi, Hiroki; Sari, D. P.*; Watanabe, Isao*; Yasui, Yukio*; Chang, L.-J.*; Kondo, Keietsu; Ito, Takashi; Ishikado, Motoyuki*; Hagihara, Masato*; Frontzek, M. D.*; et al.

Communications Materials (Internet), 1, p.43_1 - 43_6, 2020/07

High-temperature short-range order is discovered up to 720 K in Mn$$_3$$RhSi by complementary use of neutron scattering and muon spin relaxation measurements.

Journal Articles

Shell evolution of $$N$$ = 40 isotones towards $$^{60}$$Ca; First spectroscopy of $$^{62}$$Ti

Cort$'e$s, M. L.*; Rodriguez, W.*; Doornenbal, P.*; Obertelli, A.*; Holt, J. D.*; Lenzi, S. M.*; Men$'e$ndez, J.*; Nowacki, F.*; Ogata, Kazuyuki*; Poves, A.*; et al.

Physics Letters B, 800, p.135071_1 - 135071_7, 2020/01

 Times Cited Count:31 Percentile:96.48(Astronomy & Astrophysics)

Excited states in the $$N$$ = 40 isotone $$^{62}$$Ti were populated via the $$^{63}$$V($$p$$,$$2p$$)$$^{62}$$Ti reaction at $$sim$$200 MeV/nucleon at the Radioactive Isotope Beam Factory and studied using $$gamma$$-ray spectroscopy. The energies of the $$2_1^+ rightarrow 0_{rm gs}^+$$ and $$4_1^+ rightarrow 2_1^+$$ transitions, observed here for the first time, indicate a deformed Ti ground state. These energies are increased compared to the neighboring $$^{64}$$Cr and $$^{66}$$Fe isotones, suggesting a small decrease of quadrupole collectivity. The present measurement is well reproduced by large-scale shell-model calculations based on effective interactions, while ab initio and beyond mean-field calculations do not yet reproduce our findings.

Journal Articles

Quasifree neutron knockout from $$^{54}$$Ca corroborates arising $$N=34$$ neutron magic number

Chen, S.*; Lee, J.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Chazono, Yoshiki*; Navr$'a$til, P.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Raimondi, F.*; et al.

Physical Review Letters, 123(14), p.142501_1 - 142501_7, 2019/10

AA2019-0306.pdf:0.57MB

 Times Cited Count:49 Percentile:92.61(Physics, Multidisciplinary)

no abstracts in English

JAEA Reports

Report of summer holiday practical training 2018; Feasibility study on nuclear battery using HTTR core; Feasibility study for nuclear design

Ishitsuka, Etsuo; Matsunaka, Kazuaki*; Ishida, Hiroki*; Ho, H. Q.; Ishii, Toshiaki; Hamamoto, Shimpei; Takamatsu, Kuniyoshi; Kenzhina, I.*; Chikhray, Y.*; Kondo, Atsushi*; et al.

JAEA-Technology 2019-008, 12 Pages, 2019/07

JAEA-Technology-2019-008.pdf:2.37MB

As a summer holiday practical training 2018, the feasibility study for nuclear design of a nuclear battery using HTTR core was carried out. As a result, it is become clear that the continuous operations for about 30 years at 2 MW, about 25 years at 3 MW, about 18 years at 4 MW, about 15 years at 5 MW are possible. As an image of thermal design, the image of the nuclear battery consisting a cooling system with natural convection and a power generation system with no moving equipment is proposed. Further feasibility study to confirm the feasibility of nuclear battery will be carried out in training of next fiscal year.

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:8 Percentile:55.71(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Operation and commissioning of IFMIF (International Fusion Materials Irradiation Facility) LIPAc injector

Okumura, Yoshikazu; Gobin, R.*; Knaster, J.*; Heidinger, R.*; Ayala, J.-M.*; Bolzon, B.*; Cara, P.*; Chauvin, N.*; Chel, S.*; Gex, D.*; et al.

Review of Scientific Instruments, 87(2), p.02A739_1 - 02A739_3, 2016/02

 Times Cited Count:8 Percentile:34.96(Instruments & Instrumentation)

IFMIF is an accelerator based neutron facility having two set of linear accelerators each producing 125mA/CW deuterium ion beams (250mA in total) at 40MeV. The LIPAc (Linear IFMIF Prototype Accelerator) being developed in the IFMIF-EVEDA project consists of an injector, a RFQ accelerator, and a part of superconducting Linac, whose target is to demonstrate 125mA/CW deuterium ion beam acceleration up to 9MeV. The injector has been developed in CEA Saclay and already demonstrated 140mA/100keV deuterium beam. The injector was disassembled and delivered to the International Fusion Energy Research Center (IFERC) in Rokkasho, Japan, and the commissioning has started after its reassembly 2014; the first beam production has been achieved in November 2014. Up to now, 100keV/120mA/CW hydrogen ion beam has been produced with a low beam emittance of 0.2 $$pi$$.mm.mrad (rms, normalized).

Journal Articles

Measurement of ion species in high current ECR H$$^+$$/D$$^+$$ ion source for IFMIF (International Fusion Materials Irradiation Facility)

Shinto, Katsuhiro; Sen$'e$e, F.*; Ayala, J.-M.*; Bolzon, B.*; Chauvin, N.*; Gobin, R.*; Ichimiya, Ryo; Ihara, Akira; Ikeda, Yukiharu; Kasugai, Atsushi; et al.

Review of Scientific Instruments, 87(2), p.02A727_1 - 02A727_3, 2016/02

 Times Cited Count:9 Percentile:38.89(Instruments & Instrumentation)

Journal Articles

Present status of the injector for IFMIF Linear Prototype Accelerator (LIPAc)

Shinto, Katsuhiro; Ichikawa, Masahiro; Takahashi, Hiroki; Kondo, Keitaro; Kasugai, Atsushi; Gobin, R.*; Sen$'e$e, F.*; Chauvin, N.*; Ayala, J.-M.*; Marqueta, A.*; et al.

Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.493 - 495, 2015/09

Development of the prototype accelerator (LIPAc) for the engineering validation of the International Fusion Materials Irradiation Facility (IFMIF) which is an accelerator driven neutron source has been progressed at Rokkasho. The LIPAc is a deuteron linear accelerator consisting of an injector, a radio-frequency quadrupole (RFQ) linac and a superconducting linac. The objective of LIPAc is to produce a CW beam with the energy and current of 9 MeV and 125 mA, respectively. The injector was developed at CEA/Saclay and succeeded to produce CW proton and deuteron beams of 100 keV/140 mA by autumn 2012. After the test at CEA/Saclay, the injector was shipped to the International Fusion Energy Research Centre (IFERC) in Rokkasho, Aomori and started to reassemble from the end of 2013. It was successfully produced proton beams in November 2014 at Rokkasho. While the ion source conditioning was done, the beam test was progressed. In this paper, the present status of the LIPAc injector at Rokkasho with some experimental results will be presented.

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