Kinetic mass transfer behavior of Eu(III) in nitrilotriacetamide-impregnated polymer-coated silica particles

Miyagawa, Akihisa*; Hayashi, Naoki*; Kuzure, Yoshiaki*; Takahashi, Takumi*; Iwamoto, Hibiki*; Arai, Tsuyoshi*; Nagatomo, Shigenori*; Miyazaki, Yasunori; Hasegawa, Kenta; Sano, Yuichi; et al.

Bulletin of the Chemical Society of Japan, 96(7), p.671 - 676, 2023/07

https://doi.org/10.1246/bcsj.20230087

We investigated the distribution mechanism of Eu(III) in a single polymer-coated silica particle including nitrilotriacetamide (NTA) extractants known as HONTA and TOD2EHNTA. The present study provides a valuable approach for the evaluation and enhancement of the functionality of "single extractant-impregnated polymer-coated silica particle".

Cs transfer from soils contaminated by resuspended particles to Japanese mustard spinach in difficult-to-return zone of Fukushima

Tatsuno, Takahiro*; Nihei, Naoto*; Yoshimura, Kazuya; Ote, Nobuhito*

Journal of Radioanalytical and Nuclear Chemistry, 332(6), p.1677 - 1686, 2023/06

https://doi.org/10.1007/s10967-023-08899-0

Collection of strength characteristic data used for analysis evaluation in reactor pressure vessel and in-core structures in accident

Shimomura, Kenta; Yamashita, Takuya; Nagae, Yuji

JAEA-Data/Code 2022-012, 270 Pages, 2023/03

JAEA-Data-Code-2022-012.pdf:38.25MB

In a light water reactor, which is a commercial nuclear power plant, a severe accident such as loss of cooling function in the reactor pressure vessel (RPV) and exposure of fuel rods due to a drop in the water level in the reactor can occur when a trouble like loss of all AC power occurs. In the event of such a severe accident, the RPV may be damaged due to in-vessel conditions (temperature, molten materials, etc.) and leakage of radioactive materials from the reactor may occur. Verification and estimation of the process of RPV damage, molten fuel debris spillage and expansion, etc. during accident progression will provide important information for decommissioning work. Possible causes of RPV failure include failure due to loads and restraints applied to the RPV substructure (mechanical failure), failure due to the current eutectic state of low-melting metals and high-melting oxides with the RPV bottom members (failure due to inter-material reactions), and failure near the melting point of the structural members at the RPV bottom. Among the failure factors, mechanical failure is verified by numerical analysis (thermal hydraulics and structural analysis). When conducting such a numerical analysis, the heat transfer properties (thermal conductivity, specific heat, density) and material properties (thermal conductivity, Young's modulus, Poisson's ratio, tensile, creep) of the materials (zirconium, boron carbide, stainless steel, nickel-based alloy, low alloy steel, etc.) constituting the RPV and in-core structures to near the melting point are required to evaluate the creep failure of the RPV. In this document, we compiled data on the properties of base materials up to the melting point of each material constituting the RPV and in-core structures, based on published literature. In addition, because welds exist in the RPV and in-core structures, the data on welds are also included in this report, although they are limited.

Multinucleon-transfer-induced fission

Nishio, Katsuhisa

Handbook of Nuclear Physics (Internet), 43 Pages, 2022/11

Experimental investigation of natural convection and gas mixing behaviors driven by outer surface cooling with and without density stratification consisting of an air-helium gas mixture in a large-scale enclosed vessel

Abe, Satoshi; Hamdani, A.; Ishigaki, Masahiro*; Shibamoto, Yasuteru

Annals of Nuclear Energy, 166, p.108791_1 - 108791_18, 2022/02

https://doi.org/10.1016/j.anucene.2021.108791

A 3D particle-based analysis of molten pool-to-structural wall heat transfer in a simulated fuel subassembly

Zhang, T.*; Morita, Koji*; Liu, X.*; Liu, W.*; Kamiyama, Kenji

Extended abstracts of the 2nd Asian Conference on Thermal Sciences (Internet), 2 Pages, 2021/10

For the Japanese sodium cooled fast reactor, a fuel subassembly with an inner duct structure (FAIDUS) was designed to avoid the re-criticality by preventing the large-scale pool formation. In the present study, using the finite volume particle method, the EAGLE ID1 test which was an in-pile test performed to demonstrate the effectiveness of FAIDUS was numerically simulated and the thermal-hydraulic mechanisms underlying the heat transfer process were analyzed.

Numerical simulation of heat transfer behavior in EAGLE ID1 in-pile test using finite volume particle method

Zhang, T.*; Funakoshi, Kanji*; Liu, X.*; Liu, W.*; Morita, Koji*; Kamiyama, Kenji

Annals of Nuclear Energy, 150, p.107856_1 - 107856_10, 2021/01

https://doi.org/10.1016/j.anucene.2020.107856

Study on chemisorption model of cesium hydroxide onto stainless steel type 304

Nakajima, Kunihisa; Nishioka, Shunichiro*; Suzuki, Eriko; Osaka, Masahiko

Mechanical Engineering Journal (Internet), 7(3), p.19-00564_1 - 19-00564_14, 2020/06

https://doi.org/10.1299/mej.19-00564

A large amount of cesium (Cs) chemisorbed onto stainless steel is predicted to be present especially in the upper region of reactor pressure vessel (RPV) during light water reactor severe accident (LWR SA) and a chemisorption model was developed for estimation of such amounts of Cs for stainless steel type 304 (SS304). However, this existing chemisorption model cannot accurately reproduce experimental results. Therefore, in this study, a modified Cs chemisorption model which accounts for silicon content in SS304 and concentration of cesium hydroxide (CsOH) in gaseous phases was constructed by combining penetration theory for gas-liquid mass transfer with chemical reaction and mass action law for CsOH decomposition at interface between gaseous and solid phases. As a result, it was found that the modified model was able to reproduce the experimental data more accurately than the existing model.

Flow separation at inlet causing transition and intermittency in circular pipe flow

Ogawa, Masuro*

JAEA-Technology 2019-010, 22 Pages, 2019/07

JAEA-Technology-2019-010.pdf:1.5MB

Transition phenomena from laminar to turbulent flow are roughly classified into three categories. Circular pipe flow of the third category is linearly stable against any small disturbance, despite that flow actually transitions and transitional flow exhibits intermittency. These are among major challenges that are yet to be resolved in fluid dynamics. Thus, author proposes hypothesis as follows; "Flow in a circular pipe transitions from laminar flow because of vortices released from separation bubble forming in vicinity of inlet of pipe, and transitional flow becomes intermittent because vortex-shedding is intermittent." Present hypothesis can easily explain why linear stability theory has not been able to predict transition in circular pipe flow, why circular pipe flow actually transitions, why transitional flow actually exhibits intermittency even due to small disturbance, and why numerical analysis has not been able to predict intermittency of transitional flow in circular pipe.

Free convective heat transfer experiment to validate air-cooling performance analysis of fuel debris

Uesawa, Shinichiro; Yamashita, Susumu; Shibata, Mitsuhiko; Yoshida, Hiroyuki

Proceedings of 11th Korea-Japan Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-11) (Internet), 6 Pages, 2018/11