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Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*; Yokoyama, Kaoru; Takahashi, Nobuo; Hata, Haruhi; Sugitsue, Noritake
JAEA-Research 2011-035, 53 Pages, 2012/01
System decontamination has been generally carried out with the aim of reducing the amount of radioactive waste generated and minimizing exposure to radiation released from nuclear fuel facilities. At the Ningyo-Toge Environmental Engineering Center, metal surfaces that are contaminated by uranium are dry decontaminated by using iodine heptafluoride (IF) as a system decontaminator. Only a few studies have been carried out on the decontamination efficiency, mechanism, level, etc. of dry decontamination techniques that use a decontamination gas. Therefore, the generalization of dry decontamination techniques is required. In the present study, the efficiency of a dry decontamination technique was assessed by a numerical method using decontamination data obtained at the Ningyo-Toge Environmental Engineering Center. A concrete analytical content is a depositing of uranium hexafluoride.
Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*; Yokoyama, Kaoru; Takahashi, Nobuo; Hata, Haruhi; Sugitsue, Noritake
JAEA-Research 2010-032, 32 Pages, 2010/10
System decontamination has been generally carried out with the aim of reducing the amount of radioactive waste generated and minimizing human exposure to radiation released from nuclear fuel facilities. At the Ningyo-Toge Environmental Engineering Center, metal surfaces that are contaminated by uranium are dry decontaminated by using iodine heptafluoride (IF) as a system decontaminator. In this dry decontamination technique, a chemical reaction occurs between the uranium compound attached to the metal surface and IF. Only a few studies have been carried out on the decontamination efficiency, mechanism, level, etc. of dry decontamination techniques that use a decontamination gas. Therefore, the generalization of dry decontamination technique was assessed by a numerical method using decontamination data obtained at the Ningyo-Toge Environmental Engineering Center. A concrete analytical content is a depositing of Uranium Hexafluoride.
Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*; Yokoyama, Kaoru; Takahashi, Nobuo; Tsunashima, Yasumichi; Ema, Akira; Sugitsue, Noritake
JAEA-Research 2009-047, 92 Pages, 2010/01
System decontamination has been generally carried out with the aim of reducing the amount of radioactive waste generated and minimizing human exposure to radiation released from nuclear fuel facilities. At the Ningyo-Toge Environmental Engineering Center, metal surfaces that are contaminated by uranium are dry decontaminated by using iodine heptafluoride (IF) as a system decontaminator. In this dry decontamination technique, a chemical reaction occurs between the uranium compound attached to the metal surface and IF. Only a few studies have been carried out on the decontamination efficiency, mechanism, level, etc. of dry decontamination techniques that use a decontamination gas. Therefore, the generalization of dry decontamination techniques is required. In the present study, the efficiency of a dry decontamination technique was assessed by a numerical method using decontamination data obtained at the Ningyo-Toge Environmental Engineering Center.
Yokoyama, Kaoru; Hata, Haruhi; Sugitsue, Noritake; Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*
no journal, ,
The decontamination technique using the iodine heptafluoride is known as a system decontamination technique of facilities like the uranium enrichment plant where the uranium hexafluoride was handled. In this report, the mechanism of the system decontamination using the iodine heptafluoride is clarified at a molecular level. The generation process of the uranium tetrafluoride is estimated using the plant operation data. In addition, the generation speed of the uranium tetrafluoride and the activation energy are of the uranium tetrafluoride and iodine heptafluoride reaction are estimated.
Hata, Haruhi; Yokoyama, Kaoru; Sugitsue, Noritake; Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*
no journal, ,
As a first step to elucidate the molecular mechanism of decontamination systems for iodine heptafluoride, uranium hexafluoride and the metal (iron), the possibility of physical adsorption and chemical reactions with uranium hexafluoride and uranium tetrafluoride (solid), we investigate the possibility of physical adsorption and chemical reactions of this. Therefore, the intermolecular of uranium hexafluorides, iron and uranium hexafluoride, uranium tetrafluoride and uranium hexafluoride (solid) and evaluated by molecular orbital method to the intermolecular potential between, based on this data, MD law adhesion mechanism was estimated by uranium hexafluoride.
Yokoyama, Kaoru; Hata, Haruhi; Takahashi, Nobuo; Sugitsue, Noritake; Hyakutake, Toru*; Sasakura, Mariko*; Minowa, Hirotsugu*
no journal, ,
Fundamental study in the molecular level about the system decontamination using iodine heptafluoride was performed. When UF entered to the surface to which UF stuck, activation energy for UF to perform a chemical reaction on the surface of a wall was analyzed. The molecular dynamics method was used for calculation.
Hata, Haruhi; Yokoyama, Kaoru; Takahashi, Nobuo; Sugitsue, Noritake; Hyakutake, Toru*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*
no journal, ,
The IF treatment technique belongs to the systematic decontamination technology. It has the high performance decontamination technique for the plant that accumulates the uranium intermediate fluoride, such as UF, UF, UF, and UF, which exist in the uranium enrichment plant. This report will show the chemical reactions and the physical adsorption between the metal and the uranium fluoride on the molecular scale, which was calculated by the molecular dynamics method.
Yokoyama, Kaoru; Sugitsue, Noritake; Ohara, Yoshiyuki; Takeda, Hiroshi*; Rong, D.*; Yanase, Shinichiro*; Kuwagi, Kenya*; Takami, Toshihiro*; Hyakutake, Toru*
no journal, ,
Some disaster wastes polluted with the radioactive cesium diffused in the accident of the Fukushima Daiichi Nuclear Power Plant are incinerated in the refuse incineration plant. It is thought that cesium is not emitted outside since cesium is coagulated to the refuse incineration ash and trapped by a bag filter or an electric dust collector. Therefore, we research concentration and particle size distribution of the refuse incineration ash. In this study, an introduction and a plan of study are reported.
Yokoyama, Kaoru; Sugitsue, Noritake; Ohara, Yoshiyuki; Takeda, Hiroshi*; Rong, D.*; Yanase, Shinichiro*; Kuwagi, Kenya*; Takami, Toshihiro*; Hyakutake, Toru*
no journal, ,
Some disaster wastes polluted with the radioactive cesium diffused in the accident of the Fukushima Daiichi Nuclear Power Plant are incinerated in the refuse incineration plant. It is thought that cesium is not emitted outside since cesium is coagulated to the refuse incineration ash and trapped by a bag filter or an electric dust collector. Therefore, we research concentration and particle size distribution of the refuse incineration ash. In this study, the combustion model is reported.
Yokoyama, Kaoru; Sugitsue, Noritake; Ohara, Yoshiyuki; Takeda, Hiroshi*; Rong, D.*; Yanase, Shinichiro*; Kuwagi, Kenya*; Takami, Toshihiro*; Hyakutake, Toru*
no journal, ,
Some disaster wastes polluted with the radioactive cesium diffused in the accident of the Fukushima Daiichi Nuclear Power Plant are incinerated in the refuse incineration plant. It is thought that cesium is not emitted outside since cesium is coagulated to the refuse incineration ash and trapped by a bag filter or an electric dust collector. Therefore, we report the results of analysis of the cesium concentration and specific surface area of the ash, for the evaluation of the status of adherence to the incinerated ash of cesium.
Yokoyama, Kaoru; Sugitsue, Noritake; Ohara, Yoshiyuki; Takeda, Hiroshi*; Rong, D.*; Yanase, Shinichiro*; Kuwagi, Kenya*; Takami, Toshihiro*; Hyakutake, Toru*
no journal, ,
Some disaster wastes polluted with the radioactive cesium diffused in the accident of the Fukushima Daiichi Nuclear Power Plant are incinerated in the refuse incineration plant. It is thought that cesium is not emitted outside since cesium is coagulated to the refuse incineration ash and trapped by a bag filter or an electric dust collector. Therefore, we report on simulation results incorporating the adhesion model of cesium in the combustion model of waste.
Yokoyama, Kaoru; Ohara, Yoshiyuki; Sugitsue, Noritake; Takahashi, Nobuo; Rong, D.*; Takeda, Hiroshi*; Kochi, Toshinori*; Yanase, Shinichiro*; Kuwagi, Kenya*; Takami, Toshihiro*; et al.
no journal, ,
Some disaster wastes polluted with the radioactive cesium diffused in the accident of the Fukushima Daiichi Nuclear Power Plant are incinerated in the refuse incineration plant. It is thought that cesium is not emitted outside since cesium is coagulated to the refuse incineration ash and trapped by a bag filter or an electric dust collector. Therefore, we report the simulation of the behavior of cesium in an incineration plant.
Takahashi, Nobuo; Sugitsue, Noritake; Yokoyama, Kaoru; Ohara, Yoshiyuki; Yanase, Shinichiro*; Kochi, Toshinori*; Takami, Toshihiro*; Kuwagi, Kenya*; Hyakutake, Toru*; Takeda, Hiroshi*; et al.
no journal, ,
As part of the cesium behavior analysis in the incineration plant, we carried out simulation by urban garbage of high cesium density incinerated. We chose plant having the results that burnt up contaminated urban garbage with radiocesium, as the object of the analysis.
Yanase, Shinichiro*; Sugitsue, Noritake; Ishimori, Yuu; Yokoyama, Kaoru; Ohara, Yoshiyuki; Takahashi, Nobuo; Rong, D.*; Takeda, Hiroshi*; Kochi, Toshinori*; Takami, Toshihiro*; et al.
no journal, ,
no abstracts in English