Mass-spectrometric study of PuCd $_{2}$

Nakajima, Kunihisa ; Arai, Yasuo; Yamashita, Toshiyuki

PuCd $_{2}$ intermetallic compound was prepared by heating pure Pu and Cd metals at about 950K. PuCd $_{2}$ was found to be a prototype of CdI $_{2}$ by means of powder X-ray diffractometry. Mass-spectrometric experiment was performed in the temperature range of 650-770K. It was found that the vapor pressures of Cd over PuCd $_{2}$ +Pu were three to five orders of magnitude lower than those over Cd in this temperature range. From these vapor pressures, Gibbs free energy of formation of PuCd $_{2}$ was evaluated.

Language	:	English
Journal	:	Journal of Physics and Chemistry of Solids
Volume	:	66
Number	:	2-4
Pages	:	p.639 - 642
Publication Year/Month	:	2005/02
Meeting title	:	11th International IUPAC Conference on High Temperature Materials Chemistry (HTMC-11)
Held date	:	2003/05
Location (city)	:	Tokyo
Location (country)	:	Japan
Patent information	:
PDF	:
Paper URL	:	https://doi.org/10.1016/j.jpcs.2004.06.072
DOI for research data	:
Keywords	:	Pu; Cd; Intermetallic Compound; Mass Spectrometry; Knudsen Cell; PuCd $_{2}$
Research Facility	:
Press Release	:
Article of JAEA R&D Review	:
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Registration No. : B20022225
JAEA Abstracts No. : 330375
Paper Submission No. : 21715

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