Mixing behavior of molten PbCl with alkali chlorides

Okamoto, Yoshihiro ; Yaita, Tsuyoshi; Minato, Kazuo

The structural change of molten PbCl by mixing with alkali chlorides was investigated by Pb L-edge XAFS measurements. By the mixing, the nearest neighbor Pb-Cl distance and its coordination number increased, while the Debye-Waller factor and the 3rd cumulant decreased. It is concluded that the coordination structure (PbCl) $^{4-}$ is enhanced by the mixing with alkali chlorides.

Language	:	English
Journal	:	Denki Kagaku Oyobi Kogyo Butsuri Kagaku
Volume	:	73
Number	:	8
Pages	:	p.745 - 747
Publication Year/Month	:	2005/08
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Paper URL	:	https://doi.org/10.5796/electrochemistry.73.745
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Keywords	:	溶融塩; 構造; XAFS; 混合効果; 放射光; 配位構造
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Registration No. : A20050013
JAEA Abstracts No. : 330921
Paper Submission No. : 6

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