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Mott gap excitations in twin-free YBa$$_2$$Cu$$_3$$O$$_{7-delta}$$ ($$T_{c}$$ = 93 K) studied by resonant inelastic X-ray scattering

Ishii, Kenji; Tsutsui, Kenji*; Endo, Yasuo*; Toyama, Takami*; Kuzushita, Kaori; Inami, Toshiya; Owada, Kenji; Maekawa, Sadamichi*; Masui, Takahiko*; Tajima, Setsuko*; Murakami, Yoichi; Mizuki, Junichiro

Mott gap excitations in the optimally doped high-$$T_{c}$$ superconductor YBa$$_2$$Cu$$_3$$O$$_{7-delta}$$ ($$T_{c}$$ = 93 K) have been studied by the resonant inelastic X-ray scattering method. Anisotropic spectra in the $$ab$$-plane are observed in a twin-free crystal. The excitation from the one-dimensional CuO chain is enhanced at 2 eV near the zone boundary of the $$b^{*}$$ direction, while the excitation from the CuO$$_2$$ plane is broad at 1.5-4 eV and almost independent of the momentum transfer. Theoretical calculation based on the one-dimensional and two-dimensional Hubbard model reproduces the observed spectra when different values of the on-site Coulomb energy are assumed. The Mott gap of the CuO chain site is found to be much smaller than that of the CuO$$_2$$ plane site.

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Category:Physics, Multidisciplinary

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