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Report No.
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Study on radiation induced reactions in groundwater,2

not registered

Since a chloride ion is assumed to be one of the predominant solutes dissolved in groundwater, a study of the radiolysis of chloride ion and oxychlorides in aqueous solutions has been carried out in order to obtain the reliable and predictable data for the understanding the radiation induced reactions taking place in groundwater, relevant to the geological radioactive waste repository. The rate constants of the reactions between water decomposition products and different oxychlorides were determined by means of pulse radiolysis and laser photolysis methods. By using the techniques of photometry and ion-chromatography, the products formed by irradiation were analyzed and the overall reactions were summarized. After the comparison between the simulation and the experimental results, the redox reactions of the oxychloride compounds in aqueous solution were summarized and future work to be done has been pointed out.

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