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Report No.

Simultaneous observation of volatility of Zr, Hf, and Rf chlorides

Sato, Tetsuya; Tsukada, Kazuaki; Asai, Masato; Akiyama, Kazuhiko*; Haba, Hiromitsu*; Toyoshima, Atsushi; Ono, Sawako*; Hirai, Toshiyuki*; Goto, Shinichi*; Ichikawa, Shinichi; Nagame, Yuichiro; Kudo, Hisaaki*

$$^{85}$$Zr, $$^{169}$$Hf, and $$^{261}$$Rf were produced simultaneously from $$^{rm nat}$$Ge($$^{18}$$, ${it x}$n), $$^{rm nat}$$Gd($$^{18}$$O, ${it x}$n), and $$^{248}$$Cm($$^{18}$$O, 5n) reactions, respectively, and the volatility of their chlorides was examined using an isothermal gas chromatographic system. The observed gas chromatogram indicated that ZrCl$$_4$$, HfCl$$_4$$, and RfCl$$_4$$ had almost similar volatility.



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