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The Magnetic structure of NpTGa$$_5$$ by neutron scattering

Jonen, Shintaro; Metoki, Naoto   ; Honda, Fuminori; Kaneko, Koji   ; Aoki, Dai*; Yamamoto, Etsuji  ; Haga, Yoshinori   ; Shiokawa, Yoshinobu*; Onuki, Yoshichika

The magnetic structure of antiferromagnetic NpPtGa$$_5$$ have been clarified by neutron scattering measurements. For temperature below $$T_N$$ = 27 K, the NpPtGa$$_5$$ exhibits an antiferromagnetic structure with propagation vector q=(0 0 1/2), namely the Np moment of 0.4 $$mu_B$$ is parallel to the $$<$$100$$>$$ direction in the basal plane. The neutron scattering measurements under application of magnetic field parallel to the [100] direction, revealed that the field induced phase transition is due a change of antiferromagnetic domain structure from multi-domain to single-domain state. The most intrigued result in this study is the necessity of high magnetic field above 10T at T = 1 K, observed in the magnetic susceptibility. Similar results was observed in NpRhGa$$_5$$, with magnetic moment is parallel to the basal plane at low temperature. The coexistence of ferroquadrupolar order with antiferromagnetic order in NpRhGa$$_5$$, predicted theoretically, might be the hint to understand this problem.

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