Crystal structure and magnetic properties of the new ternary actinide compounds AnPdAl (An = U, Np)
Haga, Yoshinori ; Aoki, Dai*; Homma, Yoshiya*; Ikeda, Shugo; Matsuda, Tatsuma; Yamamoto, Etsuji ; Sakai, Hironori ; Tateiwa, Naoyuki ; Dung, N. D.*; Nakamura, Akio; Shiokawa, Yoshinobu*; Onuki, Yoshichika
We report the crystal structure and magnetic properties of new ternary actinide compounds UPdAl and NpPdAl. Both compounds crystallize in the body-center tetragonal ZrAlNi -type tetragonal structure (I 4/mmm). Although the magnetic susceptibility of both compounds follows the Curie-Weiss behavior at high temperature, no magnetic phase transition was observed. UPdAl has a nonmagnetic ground state where the magnetic susceptibility saturates at low temperature, while NpPdAl superconducts below 4.9 K as reported recently.