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Report No.
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Oxygen potentials of transuranium oxides

Otobe, Haruyoshi  ; Akabori, Mitsuo; Arai, Yasuo; Minato, Kazuo 

The oxygen potentials of cubic zirconia containing Pu and americia have been measured by the electromotive force (EMF) method with a zirconia solid-electrolyte. The oxygen potentials of these oxides were reviewed. The phase relations, microstructure, equilibrium state of these oxides were discussed, referring to the isothermal curve of the oxygen potentials. It was found that the oxygen potentials are sensitive to the phase transitions. Moreover, the study on the microstructure around an element incorporated in oxide fuels as well as its phase is necessary to predict the effect of the element on the oxygen potentials of oxide fuels.

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