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Chemical reaction in intense laser fields explored by photoelectron-photoion coincidence momentum imaging

Itakura, Ryuji

In the present study, we observe the photoelectron momentum images for each reaction pathway of ethanol in intense laser fields. A photoelectron is detected in coincidence with a mass-selected product ion. Although a lot of reaction channels are opened in intense laser induced ionization, we can securely obtain 3D photoelectron momentum images correlated to a specific product ion. The intensity dependence, pulse-length dependence, and detailed structure of the photoelectron images are examined quantitatively for gaining the further insight into the electronic dynamics induced by intense laser fields.

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