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Time-resolved CARS study of vibrational coherence in solid phase

Kumada, Takayuki   ; Karavitis, M.*; Goldschleger, I.*; Apkarian, A.*

We studied time-resolved CARS study of vibrational coherence in solid phase using iodine molecules in solid krypton. We observed the vibrational coherence of iodine molecules for 200 ps corresponding to about 1000 oscillations at 7 K. The rate of decoherence increases with increasing temperature and the number of vibrational quantum state.

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