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Magnetic correlations in Ho$$_{x}$$Tb$$_{2-x}$$Ti$$_{2}$$O$$_{7}$$

Ho$$_{x}$$Tb$$_{2-x}$$Ti$$_{2}$$O$$_{7}$$の磁気相関

Chang, L.-J.; Schweika, W.*; Kao, Y.-J.*; Chou, Y. Z.*; Per${ss}$on, J.*; Br$"u$ckel, T.*; Yang, H. C.*; Chen, Y. Y.*; Gardner, J. S.*

Chang, L.-J.; Schweika, W.*; Kao, Y.-J.*; Chou, Y. Z.*; Per${ss}$on, J.*; Br$"u$ckel, T.*; Yang, H. C.*; Chen, Y. Y.*; Gardner, J. S.*

Polycrystalline samples of Ho$$_{x}$$Tb$$_{2-x}$$Ti$$_{2}$$O$$_{7}$$ (0 $$<$$ $$x$$ $$<$$ 2) have been prepared and characterized for their structural and magnetic properties. The parent compounds of this solid solution are the spin ice Ho$$_{2}$$Ti$$_{2}$$O$$_{7}$$ and the spin liquid Tb$$_{2}$$Ti$$_{2}$$O$$_{7}$$. The results of specific heat, elastic and inelastic neutron scattering measurements suggest that the very strong single-ion effects of Ho$$_{2}$$Ti$$_{2}$$O$$_{7}$$ and Tb$$_{2}$$Ti$$_{2}$$O$$_{7}$$ persist in the Ho$$_{x}$$Tb$$_{2-x}$$Ti$$_{2}$$O$$_{7}$$ (0 $$<$$ $$x$$ $$<$$ 2) solid solution, whereas the Tb-Ho correlations are weak, resulting in small shifts in the energy scales but with no dramatic effect on the bulk properties.

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パーセンタイル:81.32

分野:Materials Science, Multidisciplinary

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