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Magnetic properties of single crystalline Lu$$_{2}$$Fe$$_{3}$$O$$_{7}$$

Yoshii, Kenji  ; Ikeda, Naoshi*; Fukuyama, Ryota*; Nagata, Tomoko*; Kambe, Takashi*; Yoneda, Yasuhiro   ; Fukuda, Tatsuo  ; Mori, Shigeo*

The rare-earth iron oxides R$$_{2}$$Fe$$_{3}$$O$$_{7}$$ (R=Yb and Lu) are materials closely related to a multiferroic system RFe$$_{2}$$O$$_{4}$$, which shows a new type of ferroelectiricy (i.e., electronic ferroelectiricy) at 330 K owing to real-space charge ordering of Fe ions. In this work, we have investigated detailed magnetic properties of a single crystalline LuFe$$_{3}$$O$$_{7}$$. It was found that this oxide shows the magnetic transition temperature of 270 K, which is higher than that of the corresponding RFe$$_{2}$$O$$_{4}$$ (LuFe$$_{2}$$O$$_{4}$$), 240-250 K. AC magnetic susceptibility measurements exhibited spin-glass behavior at around the magnetic transition temperature. In addition, exchange bias and magnetocaloric effect were observed at low temperatures, similarly to RFe$$_{2}$$O$$_{4}$$. These phenomena are explained in connection with several factors, such as a coexistence of ferromagnetic and antiferromagnetic interactions between Fe ions.

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