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Inter-diffusion study of actinides in a MOX diffusion couple

Matsumoto, Taku; Arima, Tatsumi*; Inagaki, Yaohiro*; Idemitsu, Kazuya*; Kato, Masato   ; Morimoto, Kyoichi ; Uno, Hiroki*; Tamura, Tetsuya*

O/M ratio dependence of inter-diffusion coefficient of U and Pu at 1873 K was evaluated from MOX and UO$$_2$$ diffusion couple. The diffusion coefficient at O/M = 2.00 was about two orders of magnitude greater than that at O/M = 1.96. In addition, it was observed that grain boundary diffusion is so large compared to bulk one for O/M = 2.00. On the other hand, GB and bulk diffusions were not clearly observed for O/M = 1.96.

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