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Thermal expansion measurement of (U,Pu)O$$_{2-x}$$ in oxygen partial pressure-controlled atmosphere

Kato, Masato   ; Ikusawa, Yoshihisa   ; Sunaoshi, Takeo*; Nelson, A. T.*; McClellan, K. J.*

Thermal expansion of (U$$_{0.7}$$Pu$$_{0.3}$$)O$$_{2-x}$$ (x = 0, 0.01, 0.02, 0.03) and (U$$_{0.52}$$Pu$$_{0.48}$$)O$$_{2.00}$$ was measured with a dilatometer in an oxygen partial pressure-controlled atmosphere. The oxygen partial pressure was controlled to hold a constant oxygen-to-metal ratio in the (U,Pu)O$$_{2-x}$$ during the measurement. Thermal expansion slightly increased with the decrease in oxygen-to-metal ratio. The relationship was derived to describe thermal expansion.

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Category:Materials Science, Multidisciplinary

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