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Quantum optimal control of the isotope-selective rovibrational excitation of diatomic molecules

Kurosaki, Yuzuru*; Yokoyama, Keiichi 

Electric field of laser pulses which gives maximum selectivity in the isotope-selective rovibrational excitation of lithium chloride molecules is calculated. Applying the optimal control theory, we calculate optimal electric field to produce mixture of LiCl-35 ($$nu$$=0, $$J$$=0) and LiCl-37 ($$nu$$=1, $$J$$=1) from molecular ensemble of LiCl-35 ($$nu$$=0, $$J$$=0) and LiCl-37 ($$nu$$=0, $$J$$=0). As a result, it is found that electric field which permit rotational excitations only gives high yield in the selective excitation compared to the electric field which permit both rotational and vibrational excitations.

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Category:Chemistry, Physical

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