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Report No.

Production and detection of fission-induced neutrons following fast neutron direct interrogation to various dry materials containing $$^{235}$$U

Sakoda, Akihiro   ; Nakatsuka, Yoshiaki; Ishimori, Yuu  ; Nakashima, Shinichi ; Komeda, Masao   ; Ozu, Akira  ; Toh, Yosuke   

For better nuclear material accountancy, we had developed a non-destructive assay system dedicated to uranium waste drums (JAWAS-N: JAEA Waste Assay System at Ningyo-toge). The system is based on a fast neutron direct interrogation (FNDI) method. To clarify the characteristics of the FNDI method and the performance of JAWAS-N, experimental and computational mock-up tests were carried out using various dry materials that contained known amounts of natural uranium. As a result, linearity between the die-away time ($$tau$$$$_{2}$$) and the counts of fast neutrons attributed to $$^{235}$$U fission was confirmed experimentally and analytically. Moreover, the MCNP simulation was performed to discuss the radial and axial dependences of $$^{235}$$U fission probability, neutron detection efficiency, and sensitivity on uranium distributions in the drum. The simulation results agreed with the empirical results reported in a previous paper, providing valuable information on the practice of FNDI-based uranium determination. Furthermore, the nominal detection limits of natural uranium in JAWAS-N were estimated to be 15, 4, and 2 g for $$tau$$$$_{2}$$ = 0.2, 0.3, and 0.4 msec, respectively. The findings obtained here will contribute to the implementation of the FNDI method to assess the quantities of $$^{235}$$U in actual uranium waste drums.



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Category:Nuclear Science & Technology



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