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Chemical & atomic studies of the heaviest elements with JAEA-ISOL; Measurements of the first ionization potentials and study of thermochemical properties

Sato, Tetsuya   

The chemical and atomic properties of the heavy elements with atomic numbers Z $$>$$ 100, affected by strong relativistic effects, are studied at an-atom-at-a-time scale using the JAEA-ISOL. We successfully determined the first ionization potential (IP$$_1$$) values of heavy actinide elements from fermium (Fm, Z = 100) to lawrencium (Lr, Z = 103) by using a surface ion-source installed in the Isotope Separator On-Line (ISOL) at the JAEA tandem accelerator facility. The adsorption behavior of Lr is being studied by a newly developed method combining vacuum chromatography with surface ionization in a metallic column/ionizer of the ISOL as well.

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