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Application of a novel gas phase synthesis approach to carbonyl complexes of accelerator-produced 5d transition metals

G$"o$tz, M.*; Yakushev, A.*; G$"o$tz, S.*; Di Nitto, A.*; D$"u$llmann, Ch. E.*; Asai, Masato  ; Kindler, B.*; Krier, J.*; Lommel, B.*; Nagame, Yuichiro* ; Sato, Tetsuya   ; Suzuki, Hayato*; Tomitsuka, Tomohiro; Tokoi, Katsuyuki*; Toyoshima, Atsushi*; Tsukada, Kazuaki  

The study of volatile superheavy element carbonyl complexes requires more efficient methods because the yield of transactinide elements decreases with increasing atomic number. This is achieved by using a newly developed double chamber system to separate the recoil chamber and the reaction one, thereby avoiding the decomposition of reactive molecules by the projectile ion beam, which hinders the synthesis of carbonyl complexes. The feasibility of this method was verified by synthesizing 5d metal short-lived isotopes as homologous element isotopes of the light transactinide elements Sg, Bh, Hs, and Mt at the Japan Atomic Energy Agency tandem accelerator and conducting model experiments.

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Category:Chemistry, Inorganic & Nuclear

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