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Strongly renormalized quasiparticles in UPt$$_3$$

Kawasaki, Ikuto  ; Takeuchi, Kazuharu*; Fujimori, Shinichi   ; Takeda, Yukiharu   ; Yamagami, Hiroshi; Yamamoto, Etsuji  ; Haga, Yoshinori   

We performed angle-resolved photoemission spectroscopy (ARPES) experiments using soft X rays to investigate the electronic structure of the heavy-fermion superconductor UPt$$_3$$. The overall band structure revealed by the present ARPES measurements is compared with density-functional calculations for UPt$$_3$$ and the non-$$5f$$ reference compound ThPt$$_3$$. We showed that the calculation for ThPt$$_3$$ gives a better description of the experimental band structure, except for the $$5f$$-derived heavy quasiparticle bands. This situation is reminiscent of Ce-based heavy-fermion systems, whose band structures are often very similar to those of non-$$4f$$ La-based compounds. The narrow heavy quasiparticle bands are located just below the Fermi level ($$E_{rm F}$$), and their band structure could not be resolved by the present energy resolution. We also showed that most of the U $$5f$$ spectral weight exists not as the coherent heavy-fermion bands but as incoherent components that distribute over a wide energy range, spanning from near $$E_{rm F}$$ to approximately 2 eV. This result indicates that the heavy quasiparticle bands are enormously renormalized by the electron correlation effect. Additionally, we showed that the spectral intensity of the heavy-fermion bands is almost temperature independent, at least up to 100 K, where the magnetic susceptibility follows a Curie-Weiss behavior.

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Category:Materials Science, Multidisciplinary

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