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Uranium-plutonium-americium cation interdiffusion in polycrystalline (U,Pu,Am)O$$_{2 pm x}$$ mixed oxides

Vauchy, R.  ; Matsumoto, Taku; Hirooka, Shun ; Uno, Hiroki*; Tamura, Tetsuya*; Arima, Tatsumi*; Inagaki, Yaohiro*; Idemitsu, Kazuya*; Nakamura, Hiroki  ; Machida, Masahiko  ; Murakami, Tatsutoshi ; Kato, Masato   

Diffusion couples made of dense polycrystalline (U,Pu,Am)O$$_{2 pm x}$$ oxides were annealed in various thermodynamic conditions (temperature, oxygen partial pressure), and for different durations. The associated actinide redistribution was quantified using Electron Probe Micro-Analysis (EPMA). Average diffusion profiles were obtained from elemental U, Pu, and Am X-ray maps and the resulting interdiffusion coefficients were calculated, then analyzed at the light of our model of point defect chemistry.

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