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Isotope production using novel MoO$$_{3}$$ targets; Contribution by vietnamese institutes, staffs and students

Suematsu, Hisayuki*; Ngo, M. C.*; Quach, N. M.*; Fujita, Yoshitaka   ; Do, T. M. D.*; Nakayama, Tadachika*; Suzuki, Tatsuya*; Nguyen, V. T.*; Niihara, Koichi*

Radiopharmacies have been used in various medical diagnoses/therapies and their market has been growing by ten times in fifteen years. In particular, $$^{99m}$$Tc has been widely used in gamma ray diagnoses. $$^{99}$$Mo, the raw material for $$^{99m}$$Tc, is currently produced as a fission product by irradiating highly enriched uranium in nuclear reactors. Efforts are being made worldwide to reduce the use of uranium from the perspective of nuclear non-proliferation. A $$^{98}$$Mo(n,$$gamma$$)$$^{99}$$Mo reaction in low enriched uranium reactors can be an alternative method. In this research, we revealed that $$beta$$-MoO$$_{3}$$, a low-temperature phase of MoO$$_{3}$$, as a neutron irradiation target promotes the diffusion of $$^{99}$$Mo from the target to water due to the hot atom effect. Utilizing this phenomenon can contribute to the stable supply of $$^{99}$$Mo and $$^{99m}$$Tc. The first nuclear reaction in/water dispersion experiments using an $$alpha$$-MoO$$_{3}$$ powder target was carried out in Dalat Nuclear Reactor, Vietnam Atomic Energy Institute to show the hot atom effect. Then, the water recovery efficiency was dramatically improved using a novel $$beta$$-MoO$$_{3}$$ whisker target by Vietnamese students and staffs. Their contributions to this research will be explained in the presentation.

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