Short communication: Inverse correlation between radiation damage and fission-track etching time on monazite

Nakajima, Toru   ; Fukuda, Shoma   ; Sueoka, Shigeru   ; Niki, Sota*; Kawakami, Tetsuo*; Danhara, Toru*; Tagami, Takahiro*

In this study, we explored the impacts of radiation damage and chemical composition on the etching time of fission tracks in monazite. Despite the potential of monazite fission-track (MFT) dating as an ultralow-temperature thermochronology, the comprehensive effects of radiation damage and non-formula elements, especially on the etching rate of MFTs, remain unexplored, and established analytical procedures are lacking. We quantified the degree of radiation damage (dFHWM) in Cretaceous to Quaternary monazites distributed in the Japan arc through Raman spectroscopy and chemical composition analyses. Subsequently, MFT etching was performed to examine the correlation between these parameters and the etching time. Estimation of the degree of radiation damage showed an increase in radiation damage corresponding to the cooling age of each geological unit. For example, the Toya ignimbrite (ca. 0.1 Ma) and the Kurobegawa granodiorite (0.8 Ma), both of which are types of monazite from Quaternary geological units, have dFHWM values of 0.27 and 0.55 cm, respectively. In contrast, the Muro ignimbrite (ca. 15 Ma) has a dFHWM value of 4.01 cm, while the Kibe granite and the Sagawa granite, both of which are Cretaceous granitoids, yielded 7.35 and 6.31 cm, respectively. MFT etching of these samples according to the existing recipe (6M HCl at 90C for 60-90 min) was completed at 1200, 860, 210, 120, and 90 min for the Toya ignimbrite, Kurobegawa granodiorite, Muro ignimbrite, Sagawa granite, and Kibe granite, respectively.