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Measurements of neutron capture cross-section for nuclides of interest in decommissioning (III); $$^{170}$$Er(n,$$gamma$$)$$^{171}$$Er and $$^{180}$$Hf(n,$$gamma$$)$$^{181}$$Hf reactions

廃止措置に係る核種の中性子捕獲断面積測定,III; $$^{170}$$Er(n,$$gamma$$)$$^{171}$$Er反応と$$^{180}$$Hf(n,$$gamma$$)$$^{181}$$Hf反応

中村 詔司  ; 芝原 雄司*; 遠藤 駿典   ; Rovira Leveroni, G.   ; 木村 敦   

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Rovira Leveroni, G.; Kimura, Atsushi

In the decommissioning of nuclear facilities, large amounts of radioactive waste are generated due to neutron activation. In that case, neutron capture cross-sections of nuclides targeted in decommissioning are required to evaluate their radioactivities produced. The present study selected two nuclides, $$^{171}$$Er and $$^{181}$$Hf, among objective ones for decommissioning, and thermal-neutron capture cross-sections for their parent nuclides were measured by the neutron activation method at the Kyoto University Research Reactor under 1-MW operation. The thermal-neutron capture cross-sections were derived on the basis of Westcott's convention. The present study obtained the results as follows: 8.19$$pm$$0.35 barns for the $$^{170}$$Er(n,$$gamma$$)$$^{171}$$Er reaction and 13.57$$pm$$0.14 barns for the $$^{180}$$Hf(n,$$gamma$$)$$^{181}$$Hf reaction. As a by-product, the measurements of the Hf sample also yielded 0.427$$pm$$0.006 barns for the $$^{179}$$Hf(n,$$gamma$$)$$^{180m}$$Hf reaction. This study revealed that some experimental and data evaluations differ from the present results by more than the experimental uncertainties.

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分野:Nuclear Science & Technology

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