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Gate-tunable resistance drops related to local superconducting gaps in thin TaS$$_2$$ layers on SrTiO$$_3$$ substrates

SrTiO$$_3$$基板上の薄いTaS$$_2$$層における局所超伝導ギャップに関連したゲート調整可能な抵抗低下

小杉 美央子*; 齊藤 英治; 吉川 貴史*; 他11名*

Kosugi, Mioko*; Saito, Eiji; Kikkawa, Takashi*; 11 of others*

Strontium titanate [SrTiO$$_{3}$$ (STO)], a perovskite oxide with an extremely high gate-tunable dielectric constant ($$varepsilon$$) due to quantum paraelectric phases, is attracting considerable attention for yielding various physical phenomena when two-dimensional (2D) layers are integrated. Superconductivity is such a typical phenomenon. However, the influence of the STO substrates on enhancing transition temperatures ($$T$$$$_{rm c}$$) for (atomically) thin 2D flakes attached to them has been rarely investigated. Here, we report gate-tunable and gradual four-terminal resistance drops with critical onset $$T$$ ($$T$$$$_{rm CR}$$) and scanning tunneling spectroscopy (STS) spectra in devices comprising thin TaS$$_{2}$$ flakes attached on monolayer hexagonal boron nitride (hBN) spacer/STO substrates. Observation of STS spectra confirms the presence of local superconducting gaps. (similar to 1.5 meV) with transition $$T$$($$T_{Delta rm C})$$ three-times higher than previous reports of $$T$$$$_{rm c}$$ under absent pressure and strong position dependence of $${Delta}$$. Depending on $$Delta$$ on back gate voltages ($$V$$$$_{rm bg}$$) and magnetic fields, there is a strong correlation between $$T$$$$_{rm CR}$$ and the onset $$T$$$$_{rm c}$$ of superconductivity, implying an enhancement of approximately five times compared with the previous highest-onset $$T$$$$_{rm c}$$ values without pressure as the applied $$V$$$$_{rm bg}$$ increases. The high onset $$T$$$$_{rm c}$$ and. are discussed based on screening of the long-range Coulomb interaction (CI) due to the high-$$varepsilon$$ of SrTiO$$_{3}$$, while the short-ranged CI remains strong in the 2D limit, causing the superconductivity. Using a monolayer hBN/SrTiO$$_{3}$$ substrate with $$V$$$$_{rm bg}$$ opens doors to $$T$$$$_{rm c}$$ enhancement in thin superconducting layers integrated on it and wide application due to the solid-state high-$$varepsilon$$ substrates.

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パーセンタイル:15.21

分野:Nanoscience & Nanotechnology

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