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Assessment of suspended sediment and $$^{137}$$Cs sources during the flood event in the Fukushima river using $$^{13}$$C and $$^{14}$$C

$$^{13}$$Cおよび$$^{14}$$Cを用いた福島県内河川における出水時の懸濁態$$^{137}$$Cs発生源の評価

中西 貴宏   ; 鶴田 忠彦  ; 舟木 泰智 

Nakanishi, Takahiro; Tsuruta, Tadahiko; Funaki, Hironori

本研究では、放射性炭素同位体比$$Delta$$$$^{14}$$Cを指標として、福島第一原子力発電所事故後に河川に流出した懸濁態$$^{137}$$Csの発生源を特定した。出水時と平水時に懸濁物質を採取し、$$^{137}$$Cs濃度、$$Delta$$$$^{14}$$C、安定炭素同位体比を測定した。その結果、出水ピーク時に森林表層土壌流出の寄与が増加することが示された。さらに、流域における$$^{137}$$Csの沈着分布は、出水時の懸濁態$$^{137}$$Cs濃度の時間的変化に反映された。この手法は、放射性セシウム、炭素それぞれの動態を理解するために有用である。

In this study, the radiocarbon isotope ratio, $$Delta$$$$^{14}$$C, was used to identify the sources of suspended sediment and $$^{137}$$Cs discharged into rivers after the Fukushima nuclear accident. Suspended sediments were collected during the flood event and under normal water conditions to determine $$^{137}$$Cs concentrations, $$Delta$$$$^{14}$$C, and stable carbon isotope ratios. The results indicated that the contribution of forest surface soil runoff increased during the flood peak. Furthermore, the distribution of $$^{137}$$Cs deposition in the watershed was reflected in temporal changes in suspended $$^{137}$$Cs concentration during the flood event. This approach provides a comprehensive understanding of both $$^{137}$$Cs and carbon dynamics.

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パーセンタイル:64.08

分野:Chemistry, Analytical

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