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Measurements of neutron capture cross-sections for nuclides of interest in decommissioning (IV); $$^{165}$$Ho(n,$$gamma$$)$$^{rm 166m,166g}$$Ho reactions

中村 詔司  ; 芝原 雄司*; 遠藤 駿典   ; Rovira Leveroni, G.   ; 木村 敦   

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Rovira Leveroni, G.; Kimura, Atsushi

During the decommissioning of nuclear facilities, large amounts of radioactive wastes are generated from structural materials. When considering the disposal or reuse of such wastes, accurate neutron capture cross-sections are required to evaluate the amounts of radioactive nuclides among the wastes. The present work selected $$^{165}$$Ho among nuclides included in the list for clearance levels in decommissioning, and measured the thermal-neutron capture cross-sections for the $$^{165}$$Ho(n,$$gamma$$)$$^{rm 166m}$$Ho, $$^{rm 166g}$$Ho reactions by the neutron activation method. The thermal cross-section measurements were performed with the graphite thermal column of the Kyoto University Research Reactor under the 5-MW operation and the thermal-neutron capture cross-sections were derived on the basis of Westcott's convention. In this work, a value of 2.79$$pm$$0.04 barn was obtained for the $$^{165}$$Ho(n,$$gamma$$)$$^{rm 166m}$$Ho reaction, and 61.2$$pm$$0.6 barn for the $$^{165}$$Ho(n,$$gamma$$)$$^{rm 166g}$$Ho reaction. The combination of these cross-sections presented 64.0$$pm$$0.6 barn, which supports the recent evaluated data of 64.69 barn and 64.4$$pm$$1.2 barn within the limit of uncertainties.

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分野:Nuclear Science & Technology

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