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Development of a phoswich detector for alpha, beta, and gamma-ray emitting radionuclide identification for decommissioning

Tateishi, Dai; Terasaka, Yuta   ; Morishita, Yuki   ; Sato, Yuki  

To ensure the safe decommissioning of the Fukushima Daiichi Nuclear Power Station, we developed a spectrum analysis method for the phoswich detector that can identify alpha-, beta-, and gamma-ray-emitting radionuclides, even in the presence of high gamma-ray backgrounds. The detector uses ZnS(Ag) and plastic scintillators to distinguish radionuclides by energy spectrum analysis. Tests with $$^{241}$$Am, $$^{90}$$Sr, $$^{57}$$Co, $$^{137}$$Cs ($$beta+gamma$$), $$^{137}$$Cs ($$gamma$$) revealed distinct spectral shapes and slopes, facilitating successful radionuclide identification of $$^{241}$$Am, $$^{90}$$Sr, $$^{137}$$Cs ($$beta$$),and $$^{137}$$Cs ($$gamma$$). However, we found no observable difference in the energy spectral shapes between $$^{57}$$Co and $$^{137}$$Cs gamma-ray emissions, which limited our spectral analysis method's ability to distinguish between these two radionuclides. This method improves upon previous smear-based techniques by detecting fixed contamination and differentiating between beta and gamma sources. The approach holds promise for applications in the characterization and treatment of radioactive waste.

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