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Journal Articles

Development of an iron(II) complex exhibiting thermal- and photoinduced double proton-transfer-coupled spin transition in a short hydrogen bond

Nakanishi, Takumi*; Hori, Yuta*; Shigeta, Yasuteru*; Sato, Hiroyasu*; Kiyanagi, Ryoji; Munakata, Koji*; Ohara, Takashi; Okazawa, Atsushi*; Shimada, Rintaro*; Sakamoto, Akira*; et al.

Journal of the American Chemical Society, 145(35), p.19177 - 19181, 2023/08

 Times Cited Count:1 Percentile:39.98(Chemistry, Multidisciplinary)

Journal Articles

Observation of proton-transfer-coupled spin transition by single-crystal neutron-diffraction measurement

Nakanishi, Takumi*; Hori, Yuta*; Shigeta, Yasuteru*; Sato, Hiroyasu*; Wu, S.-Q.*; Kiyanagi, Ryoji; Munakata, Koji*; Ohara, Takashi; Sato, Osamu*

Physical Chemistry Chemical Physics, 25(17), p.12394 - 12400, 2023/05

 Times Cited Count:1 Percentile:44.88(Chemistry, Physical)

Journal Articles

Distribution and settling behavior of americium-241 in the tropical East Pacific

Kinoshita, Norikazu*; Nagaoka, Mika; Nakanishi, Takashi*

Science of the Total Environment, 753, p.142087_1 - 142087_10, 2021/01

 Times Cited Count:4 Percentile:32.67(Environmental Sciences)

The distribution of the anthropogenic radionuclide americium-241 ($$^{241}$$Am), a decay product of $$^{241}$$Pu discharged from atmospheric tests of nuclear weapons, was investigated to resolve its horizontal and vertical migration in the Tropical East Pacific. We analyzed $$^{241}$$Am concentrations in seawater samples collected in 2003. On comparing the $$^{241}$$Am concentrations with the previously determined concentrations of $$^{239+240}$$Pu in the same samples, the vertical profiles of $$^{241}$$Am were found to be similar to those of $$^{239+240}$$Pu. At some stations, the maximum concentration of $$^{241}$$Am occurred 100-200 m deeper than that of $$^{239+240}$$Pu. The $$^{241}$$Am/$$^{239+240}$$Pu ratios in the North Pacific and South Pacific were comparable to one another, and were typical of the ratio for the Pacific. The $$^{241}$$Am distribution was influenced by the water mass at depths below 400 m. The $$^{241}$$Am data support the view there is a current flowing at depths of 400-3000 m from the North Pacific through the equator to the South Pacific. In addition, the $$^{241}$$Am vertical profile was explained by using a box model that considers the decay of $$^{241}$$Pu and adsorption and scavenging by suspended particles. The different depths for the maximum concentrations of $$^{241}$$Am and $$^{239+240}$$Pu observed at some stations were well explained by the model and by the distribution of CaCO$$_{3}$$ particles. The residence time of $$^{241}$$Am in the Pacific was also estimated by using the model.

Journal Articles

The Operation status of the superconducting cavity for CERL main linac; Toward the deep understanding inside the superconducting cavity with high current beam

Numata, Naoto*; Asakawa, Tomoyuki*; Sakai, Hiroshi*; Umemori, Kensei*; Furuya, Takaaki*; Shinoe, Kenji*; Enami, Kazuhiro*; Egi, Masato*; Sakanaka, Shogo*; Michizono, Shinichiro*; et al.

Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.566 - 570, 2015/09

no abstracts in English

Journal Articles

Tackling contamination of farmland by using NaI(Tl) spectrometer and gamma camera

Yin, Y.-G.; Suzui, Nobuo; Kawachi, Naoki; Yamaguchi, Mitsutaka; Tanoi, Keitaro*; Ishii, Satomi; Nakanishi, Tomoko*; Chino, Mitsuo*; Nakamura, Shinichi*; Watabe, Hiroshi*; et al.

Hoshasen To Sangyo, (133), p.45 - 48, 2012/12

no abstracts in English

Journal Articles

A Simple method for selective measurement of cesium 134 and cesium 137 by NaI(Tl) scintillation spectrometer

Yin, Y.-G.; Suzui, Nobuo; Yamaguchi, Mitsutaka; Kawachi, Naoki; Tanoi, Keitaro*; Nakanishi, Tomoko*; Chino, Mitsuo*; Nakamura, Shinichi*; Fujimaki, Shu

Nihon Dojo Hiryo Gaku Zasshi, 83(3), p.296 - 300, 2012/06

no abstracts in English

Journal Articles

Recent progress in the energy recovery linac project in Japan

Sakanaka, Shogo*; Akemoto, Mitsuo*; Aoto, Tomohiro*; Arakawa, Dai*; Asaoka, Seiji*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; et al.

Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2338 - 2340, 2010/05

Future synchrotron light source using a 5-GeV energy recovery linac (ERL) is under proposal by our Japanese collaboration team, and we are conducting R&D efforts for that. We are developing high-brightness DC photocathode guns, two types of cryomodules for both injector and main superconducting (SC) linacs, and 1.3 GHz high CW-power RF sources. We are also constructing the Compact ERL (cERL) for demonstrating the recirculation of low-emittance, high-current beams using above-mentioned critical technologies.

Journal Articles

Development of a prototype module for the ERL superconducting main linac at KEK

Furuya, Takaaki*; Hara, Kazufumi*; Hosoyama, Kenji*; Kojima, Yuji*; Nakai, Hirotaka*; Nakanishi, Kota*; Sakai, Hiroshi*; Umemori, Kensei*; Sawamura, Masaru; Shinoe, Kenji*

Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2923 - 2925, 2010/05

A prototype module including a couple of 1.3 GHz superconducting 9-cell cavities has been designed as the main linac of cERL which is the test facility to establish the basic ERL technology at KEK. The shape of 9-cell Nb structure is optimized to accelerate a CW beam of 100 mA with sufficiently damped higher order modes (HOM) which is achieved by adopting an eccentric fluted beam pipe and a cylindrical beam pipe of a large diameter of 120 mm. Extracted HOMs are absorbed by the ferrite cylinders bonded on the copper beam pipes by HIP process. A power coupler with double disk-ceramics has been developed to transfer an RF of 20 kW CW to the cavity in full reflection. The test results of fabrication, cooling and RF performance for these components are integrated as the prototype module of the main linac for cERL facility.

Journal Articles

Partition coefficient of Ra in gypsum

Yoshida, Yasushi*; Nakazawa, Toshiyuki*; Yoshikawa, Hideki; Nakanishi, Takashi*

Journal of Radioanalytical and Nuclear Chemistry, 280(3), p.541 - 545, 2009/06

 Times Cited Count:12 Percentile:62.14(Chemistry, Analytical)

Coprecipitation experiment of Ra in gypsum was done with oversaturation method. Derived partition coefficient is,0.71$$pm$$0.53. Partition coefficient of Ra in gypsum was not reported. Comparing with that of Ra in barite and of Sr in gypsum, a value of partition coefficient in the present study is though to be reasonable.

Journal Articles

New system of nuclear education by network

Hasegawa, Makoto; Nakanishi, Takashi*; Fujii, Yasuhiko*; Odaka, Tomohiro*

Hosha Kagaku Nyusu, (17), p.29 - 35, 2008/03

no abstracts in English

Journal Articles

Partition coefficients of Ra and Ba in calcite

Yoshida, Yasushi*; Yoshikawa, Hideki; Nakanishi, Takashi*

Geochemical Journal, 42(3), p.295 - 304, 2008/00

 Times Cited Count:15 Percentile:37.55(Geochemistry & Geophysics)

Partition coefficients ($$D$$) of Ra and Ba in calcite were derived in an experiment of coprecipitation. Free Drift Method (FDM) was adopted. As a result of experiment, $$D$$ of Ra and Ba were 9.4e-3 and 4.7e-3, respectively. A saturation state is expected to be a low oversaturation in duration of experiment and according to an estimated saturation index, a composition of a final solution was close to equilibrium with calcite. The values of $$D$$$$_{rm Ra}$$ and $$D$$$$_{rm Ba}$$ showed the similar extent. It implies that difference of size of ionic radius does not affect incorporation behavior of Ra and Ba in calcite.

Journal Articles

MOX Co-deposition tests at RIAR for SF reprocessing optimization

Kofuji, Hirohide; Sato, Fuminori; Myochin, Munetaka; Nakanishi, Shigeyuki*; Kormilitsyn, M. V.*; Ishunin, V.*; Bychkov, A. V.*

Journal of Nuclear Science and Technology, 44(3), p.349 - 353, 2007/03

 Times Cited Count:8 Percentile:51.08(Nuclear Science & Technology)

The Oxide Electrowinning method has being studied as one of the candidate dry reprocessing concepts of future fuel cycle system. On the MOX co-deposition process, main process of that method, some fundamental experiments have been performed to confirm its feasibility. In the experiments, several parameters were set to study the suitable electrolysis condition to obtain desired granule of MOX. The concentrations of uranium, plutonium, FP simulators, and CP simulators were adopted as the parameters. The blowing gas composition during the electrolysis was also set as the variable condition. Through these experiments, it was clarified that the partial pressure of chlorine gas during electrolysis was important to obtain MOX granule with high Pu concentration without generating bottom precipitation in melt. Finally, adequacy of process control method for MOX co-electrolysis was confirmed through the test using spent FR fuel.

Journal Articles

Reaction analysis of MOX co-deposition in oxide electrowinning process

Sato, Fuminori; Mizuguchi, Koji; Nakanishi, Shigeyuki; Myochin, Munetaka

Nihon Genshiryoku Gakkai Wabun Rombunshi, 5(4), p.268 - 281, 2006/12

MOX co-deposition process, which is one of the main parts of oxide electrowinning process, was studied by both sides of examination and analysis. Parameter tests using U and Pu were performed as basic examination, and fundamental data of the process such as polarization property of molten salt including U and Pu, current efficiency of electrolysis and PuO$$_{2}$$ concentration in recovered deposit, etc. were acquired. In addition, to analyze the process behavior, especially polarization property at electrolysis, a reaction model considering Pu$$^{4+}$$, Pu$$^{3+}$$, UO$$_{2}$$$$^{2+}$$, UO$$_{2}$$$$^{+}$$, PuO$$_{2}$$$$^{2+}$$ and PuO$$_{2}$$$$^{+}$$in molten NaCl-2CsCl salt was developed. The validity of this model was confirmed by comparison of the experimental and analytical results. Using this model behavior of chemical species in the process was studied and control factors of MOX co-deposition process were discussed.

Journal Articles

Half-life of $$^{184}$$Re populated by the $$(gamma,n)$$ reaction from laser Compton scattering $$gamma$$ rays at the electron storage ring NewSUBARU

Hayakawa, Takehito; Miyamoto, Shuji*; Hayashi, Yukio; Kawase, Keigo*; Horikawa, Ken*; Chiba, Satoshi; Nakanishi, Kosuke*; Hashimoto, Hisanobu*; Ota, Takeshi*; Kando, Masaki; et al.

Physical Review C, 74(6), p.065802_1 - 065802_5, 2006/12

 Times Cited Count:29 Percentile:82.68(Physics, Nuclear)

We report a half-life of the ground state of $$^{184}$$Re populated by the $$^{185}$$Re$$(gamma,n)$$$$^{184}$$Re reaction with the laser Compton scattering $$gamma$$-rays generated through relativistic engineering. The $$gamma$$-rays are provided at the electron storage ring NewSUBARU. The previous experiment using deuteron-induced reactions has yielded a recommended half-life of the 3$$^-$$ ground state of $$^{184}$$Re to be 38.0 $$pm$$ 0.5 d, including a possible contribution from the 8$$^{+}$$ isomer ($$T_{1/2}$$ = 169 $$pm$$ 8 d) of $$^{184}$$Re since the presence of the isomer was not known at that time. In contrast, the $$(gamma,n)$$ reaction has an advantage to selectively populate the ground state because this reaction does not bring large angular momentum. The measured half-life of 35.4 $$pm$$ 0.7 d is shorter than the previous half-life by about 7%. This difference is crucial for applications using the activation method.

Journal Articles

Excitation and decay of the isovector spin-flip giant monopole resonance via the $$^{208}$$Pb($$^{3}$$He,${it tp}$) reaction at 410 MeV

Zegers, R. G. T.*; Abend, H.*; Akimune, Hidetoshi*; Van den Berg, A. M.*; Fujimura, Hisako*; Fujita, Hirohiko*; Fujita, Yoshitaka*; Fujiwara, Mamoru; Gal$`e$s, S.*; Hara, Keigo*; et al.

Nuclear Physics A, 731, p.121 - 128, 2004/02

 Times Cited Count:11 Percentile:56.77(Physics, Nuclear)

no abstracts in English

Journal Articles

Microscopic structure of the Gamow-Teller resonance in $$^{58}$$Cu

Hara, Keigo*; Adachi, Takeshi*; Akimune, Hidetoshi*; Daito, Izuru*; Fujimura, Hisako*; Fujita, Yoshitaka*; Fujiwara, Mamoru; Fushimi, Kenichi*; Hara, Kaoru*; Harakeh, M. N.*; et al.

Physical Review C, 68(6), p.064612_1 - 064612_9, 2003/12

 Times Cited Count:11 Percentile:57.99(Physics, Nuclear)

no abstracts in English

Journal Articles

Excitation and decay of the Isovector giant monopole resonances via the $$^{208}$$Pb($$^{3}$$He,${it tp}$) reaction at 410 MeV

Zegers, R. G. T.; Abend, H.*; Akimune, Hidetoshi*; Van den Berg, A. M.*; Fujimura, Hisako*; Fujita, Hirohiko*; Fujita, Yoshitaka*; Fujiwara, Mamoru; Gal$`e$s, S.*; Hara, Keigo*; et al.

Physical Review Letters, 90(20), p.202501_1 - 202501_4, 2003/05

 Times Cited Count:49 Percentile:84.91(Physics, Multidisciplinary)

no abstracts in English

Journal Articles

Effects of Pb depositon on pre-covered Ag/Ni(111) surface; Manipulation of growth mode and growth orientation

Ito, Takahiko*; Nakanishi, Shigemitsu*; Umezawa, Kenji*; Yamamoto, Shunya; Narumi, Kazumasa; Naramoto, Hiroshi

JAERI-Review 99-025, TIARA Annual Report 1998, p.182 - 184, 1999/10

no abstracts in English

Journal Articles

The Largest DC generator with a capacity of 51,300kW

;

Denki Gakkai-Shi, 118(2), p.108 - 111, 1998/00

no abstracts in English

Journal Articles

Control characteristics of DC generator-motors with flywheels for toroidal field coil power source

; ; ; ;

Denki Gakkai Rombunshi, D, 117-D(5), p.579 - 588, 1997/05

no abstracts in English

47 (Records 1-20 displayed on this page)