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Ichikawa, Tsubasa*; Hakoshima, Hideaki*; Inui, Koji*; Ito, Kosuke*; Matsuda, Ryo*; Mitarai, Kosuke*; Miyamoto, Koichi*; Mizukami, Wataru*; Mizuta, Kaoru*; Mori, Toshio*; et al.
Nature Reviews Physics (Internet), 6(6), p.345 - 347, 2024/06
Times Cited Count:8 Percentile:99.15(Physics, Applied)Otsuka, Yusuke*; Kanazawa, Naoya*; Hirayama, Motoaki*; Matsui, Akira*; Nomoto, Takuya*; Arita, Ryotaro*; Nakajima, Taro*; Hanashima, Takayasu*; Ukleev, V.*; Aoki, Hiroyuki; et al.
Science Advances (Internet), 7(47), p.eabj0498_1 - eabj0498_9, 2021/11
Times Cited Count:16 Percentile:63.29(Multidisciplinary Sciences)Sato, Tetsuya; Asai, Masato; Borschevsky, A.*; Beerwerth, R.*; Kaneya, Yusuke*; Makii, Hiroyuki; Mitsukai, Akina*; Nagame, Yuichiro; Osa, Akihiko; Toyoshima, Atsushi; et al.
Journal of the American Chemical Society, 140(44), p.14609 - 14613, 2018/11
Times Cited Count:32 Percentile:69.40(Chemistry, Multidisciplinary)The first ionization potential (IP) yields information on valence electronic structure of an atom. IP
values of heavy actinides beyond einsteinium (Es, Z = 99), however, have not been determined experimentally so far due to the difficulty in obtaining these elements on scales of more than one atom at a time. Recently, we successfully measured IP
of lawrencium (Lr, Z = 103) using a surface ionization method. The result suggests that Lr has a loosely-bound electron in the outermost orbital. In contrast to Lr, nobelium (No, Z = 102) is expected to have the highest IP
among the actinide elements owing to its full-filled 5f and the 7s orbitals. In the present study, we have successfully determined IP
values of No as well as fermium (Fm, Z = 100) and mendelevium (Md, Z = 101) using the surface ionization method. The obtained results indicate that the IP
value of heavy actinoids would increase monotonically with filling electrons up in the 5f orbital like heavy lanthanoids.
Sako, Hiroyuki; Harada, Hiroyuki; Sakaguchi, Takao*; Chujo, Tatsuya*; Esumi, Shinichi*; Gunji, Taku*; Hasegawa, Shoichi; Hwang, S.; Ichikawa, Yudai; Imai, Kenichi; et al.
Nuclear Physics A, 956, p.850 - 853, 2016/12
Times Cited Count:14 Percentile:64.97(Physics, Nuclear)Sato, Nozomi; Sato, Tetsuya; Asai, Masato; Toyoshima, Atsushi; Tsukada, Kazuaki; Li, Z.*; Nishio, Katsuhisa; Nagame, Yuichiro; Schdel, M.; Haba, Hiromitsu*; et al.
Radiochimica Acta, 102(3), p.211 - 219, 2014/03
Times Cited Count:10 Percentile:57.48(Chemistry, Inorganic & Nuclear)Production cross-sections of the isotope Lr in the
Cf +
B,
Am +
O, and
Cm +
N reactions were measured using a He/KCl gas-jet transport system and a rotating wheel
-particle detection apparatus. The
-particle energy of
Lr was distributed from 8.3 to 8.7 MeV and its half-life,
, was measured to be
s. The maximum cross sections in the
Cf(
B, 4
)
Lr and
Am(
O, 5
)
Lr reactions were determined to be
nb at the beam energy of 63 MeV and
nb at 96 MeV, respectively. In the
Cm(
N, 6
)
Lr reaction, the cross section was measured to be
nb at 91 MeV.
Asai, Masato; Tsukada, Kazuaki; Sakama, Minoru*; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Ishii, Yasuo; Toyoshima, Atsushi; Ishii, Tetsuro; Nishinaka, Ichiro; Nagame, Yuichiro; et al.
Physical Review C, 87(1), p.014332_1 - 014332_6, 2013/01
Times Cited Count:6 Percentile:41.87(Physics, Nuclear)The spin-parity and neutron configuration of the ground state of No have been identified through
-decay spectroscopy. The
No is the nucleus with the largest neutron number whose spin-parities and single-particle configurations have ever been identified. The neutron 9/2
[615] configuration was assigned to the ground state of
No as well as to the 231.4 keV level in
Fm. This allowed us to establish energy spacings and order of the neutron single-particle orbitals in such heaviest nuclear region. The appearance of the 9/2
[615] ground state at
=157 implies that the order of the neutron orbitals between the
=152 and 162 deformed shell gaps should change considerably with increasing neutron number.
Sato, Nozomi; Sato, Tetsuya; Asai, Masato; Toyoshima, Atsushi; Tsukada, Kazuaki; Li, Z.*; Nishio, Katsuhisa; Nagame, Yuichiro; Schdel, M.; Haba, Hiromitsu*; et al.
RIKEN Accelerator Progress Report, Vol.46, P. 237, 2013/00
Due to the strong relativistic effects, the weakly-bound outermost electron results in a significantly low first ionization potential (IP) of Lr as compared with its neighboring heavy actinides. The isotope Lr, with a relatively long half-life of 27 s, is the suitable candidates for the IP measurement of Lr through the surface ionization method. In the present study, we measured the cross section of the
Cm(
N, 6
)
Lr reaction to evaluate the production rate of
Lr. A
Cm target with 960
60
g/cm
thickness was bombarded with a
N
beam from the RIKEN AVF Cyclotron. The beam energy was 91 MeV in the middle of the target. The average beam intensity was 1.2 particle-
A. Reaction products were transported to the rotating wheel
-particle detection system with a He/KCl gas-jet system. The
Lr cross section of 27
1 nb was calculated based on the
-particle events between 8.3 and 8.7 MeV.
Ichikawa, Shoichi; Haga, Hiroyuki; Katsuyama, Kozo; Uwaba, Tomoyuki; Maeda, Koji; Nishinoiri, Kenji
JAEA-Testing 2012-001, 36 Pages, 2012/07
The life of FBR (Fast Breeder Reactor) fuel assembly is restricted by BDI (Bundle-Duct Interaction). Therefore, it is very important to carry out the out pile bundle compressive tests which can imitate BDI, in order to evaluate BDI behavior. The target of the conventional BDI behavior was thin pins ( 6.5 mm) for fuel pellets which were used with the assembly of Monju (the Monju prototype fast breeder reactor) etc. Furthermore by an upgraded Monju core and a demonstration core, adoption of thick pins for the holler annular pellets is planned. Therefore, it was necessary to carry out BDI evaluation of a thick pin. Then, the plans for out of pile bundle compressive test for large diameter pins were are reported this time.
Hirayama, Yoshikazu*; Mihara, Mototsugu*; Watanabe, Yutaka*; Jeong, S. C.*; Miyatake, Hiroari*; Momota, Sadao*; Hashimoto, Takashi*; Imai, Nobuaki*; Matsuta, Kensaku*; Ishiyama, Hironobu*; et al.
European Physical Journal A, 48(5), p.54_1 - 54_10, 2012/05
Times Cited Count:2 Percentile:16.19(Physics, Nuclear)Ichikawa, Shoichi; Abe, Kazuyuki; Haga, Hiroyuki; Kajima, Hisashi*; Sakurai, Satoshi*; Katsuyama, Kozo; Maeda, Koji; Nishinoiri, Kenji
JAEA-Technology 2011-032, 46 Pages, 2012/01
The assembly technique to the capsular irradiation rig newly developed was established. In the irradiation examination, the assembling disassembling and reassembling to PFB110 "B11(1), B11(2)" and PFB140 "B14" that built in Am-MOX fuel pin was achieved. The reassembly technique by recycling the irradiation material was established in the assembly of B11(2). This time, the assembly and disassembly of B11 (1) were reported. Moreover, the assembly of B14 which improved the assembly technology of B11 (1) was reported.
Sato, Nozomi; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Kaji, Daiya*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Ozeki, Kazutaka*; Sumita, Takayuki*; Yoneda, Akira*; et al.
Journal of the Physical Society of Japan, 80(9), p.094201_1 - 094201_7, 2011/09
Times Cited Count:16 Percentile:65.60(Physics, Multidisciplinary)Decay properties of Hs and
Hs produced in the
Pb(
Fe,
) [
=1, 2] reactions were studied using a gas-filled recoil ion separator at the linear accelerator facility of RIKEN. A total of 6 decay chains were assigned to
Hs. Cross sections for the
Hs production in the
Pb(
Fe,
) and
Pb(
Fe,
) reactions were measured to be
pb and
pb, respectively. The isotope
Hs decayed with a half-life of
ms by
-particle emission and spontaneous fission. The
-particle energy of
Hs was observed at 10.61
0.04 and 10.80
0.08 MeV. The spontaneous fission branch of
Hs was found to be
.
Ichikawa, Shoichi; Haga, Hiroyuki; Kikukawa, Kiyohide*; Fukasaku, Hironobu*; Kurosawa, Yoichi*; Katsuyama, Kozo; Maeda, Koji; Nagamine, Tsuyoshi
JAEA-Technology 2011-020, 32 Pages, 2011/07
Disassembling technique of the driver fuel assembly irradiated in the experimental fast reactor JOYO has been established at Fuel Monitoring Facility in JAEA. This technique made it possible to remove the fuel pins from the driver fuel assembly without the fuel pin sectioning. After disassembling the fuel assembly, some selected fuel pins can be reassembled into the new irradiation vehicle for the continuous irradiation at JOYO. This technique enables us to obtain the irradiation data of high burn-up fuel and high neutron dose material.
Asai, Masato; Tsukada, Kazuaki; Haba, Hiromitsu*; Ishii, Yasuo; Ichikawa, Takatoshi*; Toyoshima, Atsushi; Ishii, Tetsuro; Nagame, Yuichiro; Nishinaka, Ichiro; Kojima, Yasuaki*; et al.
Physical Review C, 83(1), p.014315_1 - 014315_12, 2011/01
Times Cited Count:29 Percentile:82.00(Physics, Nuclear)Excited states in Fm populated via the
decay of
No are studied in detail through
-
coincidence and
fine structure measurements. Spin-parities and neutron configurations of the excited states in
Fm as well as the ground state of
No are definitely identified on the basis of deduced internal conversion coefficients, lifetimes of
transitions, rotational-band energies built on one-quasiparticle states, and hindrance factors of
transitions. It is found that the excitation energy of the 1/2
[620] state in
=151 isotones increases with the atomic number, especially at
100, while that of the 1/2
[631] state decreases at
=100. Energy systematics of the one-quasiparticle states in the
=151 isotones are discussed in terms of the evolution of nuclear deformation involving the hexadecapole and hexacontatetrapole deformations.
Kobayashi, Yasuhiko; Kikuchi, Masahiro; Todoriki, Setsuko*; Saito, Kimie*; Katsura, Yoko*; Kameya, Hiromi*; Ichikawa, Mariko*; Iizuka, Tomoko*; Chiba, Etsuko*; Ukai, Mitsuko*
Shokuhin Shosha, 45(1-2), p.26 - 33, 2010/09
Effect of -irradiation on sprouting and rooting of garlic was investigated. Sprouting and rooting of garlic were inhibited by irradiation of bulbs at 2 months after harvest with doses more than 30 Gy. Four weeks-later irradiation requires higher doses to complete sprouting/rooting inhibition.
Ichikawa, Tatsuya*; Seito, Hajime; Sato, Yoshishige*; Takehisa, Masaaki*; Kojima, Takuji; Watanabe, Hiroshi*
Shokuhin Shosha, 45(1-2), p.1 - 3, 2010/09
Nagae, Daisuke*; Ishii, Tetsuro; Takahashi, Ryuta*; Asai, Masato; Makii, Hiroyuki; Osa, Akihiko; Sato, Tetsuya; Ichikawa, Shinichi; Shimizu, Yoshifumi*; Shoji, Takuya*
AIP Conference Proceedings 1224, p.156 - 160, 2010/04
Times Cited Count:2 Percentile:63.32(Physics, Nuclear)Seito, Hajime; Ichikawa, Tatsuya*; Hanaya, Hiroaki; Sato, Yoshishige*; Kaneko, Hirohisa; Haruyama, Yasuyuki; Watanabe, Hiroshi*; Kojima, Takuji
Radiation Physics and Chemistry, 78(11), p.961 - 965, 2009/11
Times Cited Count:5 Percentile:34.78(Chemistry, Physical)no abstracts in English
Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sato, Nozomi*; Sumita, Takayuki*; Yoneda, Akira*; Ichikawa, Takatoshi*; et al.
Journal of the Physical Society of Japan, 78(6), p.064201_1 - 064201_6, 2009/06
Times Cited Count:30 Percentile:77.45(Physics, Multidisciplinary)Decay properties of an isotope Bh and its daughter nucleus
Db produced by the
Cm(
Na,5
) reaction were studied by using a gas-filled recoil separator coupled with a position-sensitive semiconductor detector.
Bh was clearly identified from the correlation of the known nuclide,
Db. The obtained decay properties of
Bh and
Db are consistent with those observed in the
113 chain, which provided further confirmation of the discovery of
113.
Seito, Hajime; Ichikawa, Tatsuya*; Kaneko, Hirohisa; Sato, Yoshishige*; Watanabe, Hiroshi*; Kojima, Takuji
Radiation Physics and Chemistry, 78(5), p.356 - 359, 2009/05
Times Cited Count:6 Percentile:39.83(Chemistry, Physical)Kaji, Daiya*; Morimoto, Koji*; Sato, Nozomi*; Ichikawa, Takatoshi*; Ideguchi, Eiji*; Ozeki, Kazutaka*; Haba, Hiromitsu*; Koura, Hiroyuki; Kudo, Yuki*; Ozawa, Akira*; et al.
Journal of the Physical Society of Japan, 78(3), p.035003_1 - 035003_2, 2009/03
A new hassium isotopes Hs is directly produced for the first time. The experiment was performed at the linear accelerator (RILAC) facility in RIKEN (the Institute of Physical and Chemical Research) from Jun. 19 to 25. In the 25-h irradiation of
Fe on
Pb and 46-h irradiation of
Fe on
Pb, 8 decay chains and 1 decay chain, respectively, were observed. All decay chains were assigned to subsequent decays from
Hs. The half-life of
Hs is 0.60
ms. In this experiment, the total beam dose was
ions for
Fe and
ions for
Fe. The production cross section corresponding to 8 decay events and 1 decay chain was deduced to be 21
pb and 1.6
pb by assuming that the transmission of the system is 80%.