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JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-3, JRR-4 and JRTF facilities

Tobita, Minoru*; Konda, Miki; Omori, Takeshi*; Nabatame, Tsutomu*; Onizawa, Takashi*; Kurosawa, Katsuaki*; Haraga, Tomoko; Aono, Ryuji; Mitsukai, Akina; Tsuchida, Daiki; et al.

JAEA-Data/Code 2022-007, 40 Pages, 2022/11

JAEA-Data-Code-2022-007.pdf:1.99MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete, ash, ceramic and brick samples generated from JRR-3, JRR4 and JRTF facilities. In this report, we summarized the radioactivity concentrations of 24 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{41}$$Ca, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{99}$$Tc, $$^{rm 108m}$$Ag, $$^{129}$$I, $$^{137}$$Cs, $$^{133}$$Ba, $$^{152}$$Eu, $$^{154}$$Eu, $$^{rm 166m}$$Ho, $$^{234}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{243}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2020-2021.

Journal Articles

Study on oxidation model for Zircalloy-2 cladding in SFP accident condition

Nemoto, Yoshiyuki; Kaji, Yoshiyuki; Onizawa, Takashi*; Kanazawa, Toru*; Nakashima, Kazuo*; Tojo, Masayuki*

Proceedings of Annual Congress of the European Federation of Corrosion (EUROCORR 2018) (USB Flash Drive), 8 Pages, 2018/09

The authors proposed oxidation models based on oxidation data which previously obtained in high temperature oxidation tests on small sample of Zircalloy-2 (Zry2) cladding in dry air and in air/steam mixture environment. The oxidation models were implemented in computational fluid dynamics (CFD) code to analyse oxidation behavior of long cladding sample in hypothetical spent fuel pool (SFP) accident conditions. The oxidation tests were conducted using Zry2 cladding sample 500 mm in length. The oxide layer growth in dry air was well reproduced in the calculation using the oxidation model, meanwhile which in air/steam mixture was overestimated atmosphere composition change anticipated in the spent fuel rack during the accident, and its influence on the oxidation behaviour of the cladding were discussed in consideration of the oxidation model improvement.

Journal Articles

Development of separation technique of sodium nitrate from low-level radioactive liquid waste using electrodialysis with selective ion-exchange membranes

Irisawa, Keita; Nakagawa, Akinori; Onizawa, Takashi*; Kogawara, Takafumi*; Hanada, Keiji; Meguro, Yoshihiro

Proceedings of 15th International Conference on Environmental Remediation and Radioactive Waste Management (ICEM 2013) (CD-ROM), 5 Pages, 2013/09

 Times Cited Count:1 Percentile:60.76(Engineering, Environmental)

Journal Articles

Manufacturability and strength assessment of modified 9Cr-1Mo steel products for Japan sodium cooled fast reactor components, 2; Long thin-walled tubes with small diameter

Wakai, Takashi; Onizawa, Takashi; Obara, Satoshi; Nakashima, Takashi*; Yokoyama, Tetsuo*; Iseda, Atsuro*; Ogumo, Shinya*; Futagami, Satoshi*

Tainetsu Kinzoku Zairyo Dai-123-Iinkai Kenkyu Hokoku, 52(2), p.171 - 181, 2011/07

To enhance the economic competitiveness, high-Cr ferritic steels are adopted as the structural materials for JSFR, because the steels have both excellent high temperature strength and thermal properties. Among the high-Cr ferritic steels, modified 9Cr-1Mo steel (compatible to ASTM A213 T91) is a candidate of the structural material for the demonstration facility of JSFR, because the steel has superior microstructure stability at elevated temperature for long time. As for the steam generator tubes, to enhance the safety, straight double-walled tubes will be employed. In this study, the following technical issues were investigated; (1) Industrial manufacturability of thin-walled small bore tubes made of modified 9Cr-1Mo steel, (2) performance demonstration of the thin-walled small bore tubes, (3) industrial manufacturability of double-walled tubes using the thin-walled small bore tubes and (4) extraction of technical problems to manufacture the double-walled tubes for the JSFR steam generator. As a result, thin-walled small bore tubes made of modified 9Cr-1Mo steel were successfully manufactured by using the existing industrial facilities, up to 17m in length. The mechanical properties of the tubes satisfy the requirements from plant designing, as well as those from the material strength standards. Further, double walled tubes were also manufactured, up to 15m in length. The surface conditions of the tubes and the contact pressure between inner and outer tubes should be optimized.

Oral presentation

Evaluation of radiation resistance of activated sludge used for nitrate ion decomposition

Nakagawa, Akinori; Kogawara, Takafumi; Onizawa, Takashi*; Hanada, Keiji; Nakayama, Takuya; Meguro, Yoshihiro

no journal, , 

no abstracts in English

Oral presentation

Development of membrane separation method of sodium nitrate from radioactive liquid waste, 5; Engineering test of sodium nitrate separation by electrodialysis with membrane

Nakagawa, Akinori; Kogawara, Takafumi; Onizawa, Takashi; Meguro, Yoshihiro

no journal, , 

Engineering test of high concentrated sodium nitrate separation by electrodialysis with membrane was conducted. In this test, transferation efficiency, electric power consumption, ion selectivity and composition of separated solution were researched.

Oral presentation

Study on improvement of safety for accident conditions in spent fuel pool, 21; Investigation of cladding oxidation model

Nemoto, Yoshiyuki; Onizawa, Takashi*; Kaji, Yoshiyuki; Nakashima, Kazuo*; Kanazawa, Toru*; Tojo, Masayuki*

no journal, , 

Cladding oxidation model construction and its validation is necessary for the upgrading of severe accidentcode which will be utilized for analysis of the spent fuel pool (SFP) accident. Cladding oxidation tests and analyses using the proposed oxidation model were coducted in the simulated SFP accident condition, and their results were compared. Modification of the oxidation model will be discussed in the lecture.

Oral presentation

Development of membrane separation method of sodium nitrate from radioactive liquid waste, 4; Engineering test apparatus building and its performance test

Meguro, Yoshihiro; Nakagawa, Akinori; Kogawara, Takafumi; Onizawa, Takashi

no journal, , 

Based on basic experiments of sodium nitrate separation by electrodialysis with membrane, an apparatus concept was established and an engineering scale equipment was built. A designed separation ability was showed in a performance test.

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