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Journal Articles

Polarized and unpolarized neutron scattering for magnetic materials at the triple-axis spectrometer PONTA in JRR-3

Nakajima, Taro*; Saito, Hiraku*; Kobayashi, Naoki*; Kawasaki, Takuro; Nakamura, Tatsuya; Furukawa, Hazuki*; Asai, Shinichiro*; Masuda, Takatsugu*

Journal of the Physical Society of Japan, 93(9), p.091002_1 - 091002_5, 2024/09

Journal Articles

Experimental evidence for the significance of optical phonons in thermal transport of tin monosulfide

Wu, P.*; Murai, Naoki; Li, T.*; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Kofu, Maiko; Nakajima, Kenji; Xia, K.*; Peng, K.*; Zhang, Y.*; et al.

New Journal of Physics (Internet), 25(1), p.013032_1 - 013032_11, 2023/01

 Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)

Journal Articles

"Live-autoradiography" technique reveals genetic variation in the rate of Fe uptake by barley cultivars

Higuchi, Kyoko*; Kurita, Keisuke; Sakai, Takuro; Suzui, Nobuo*; Sasaki, Minori*; Katori, Maya*; Wakabayashi, Yuna*; Majima, Yuta*; Saito, Akihiro*; Oyama, Takuji*; et al.

Plants (Internet), 11(6), p.817_1 - 817_11, 2022/03

 Times Cited Count:2 Percentile:32.87(Plant Sciences)

Genetic diversity in the rate of Fe uptake by plants has not been broadly surveyed among plant species or genotypes, although plants have developed various Fe acquisition mechanisms. We adopted the "Live-autoradiography" technique with radioactive $$^{59}$$Fe to directly evaluate the uptake rate of Fe by barley cultivars from a nutrient solution containing a very low concentration of Fe. Our observations revealed that the ability to acquire Fe from the low Fe solution was not always the sole determinant of tolerance to Fe deficiency among the barley genotypes.

Journal Articles

Recent update of AMATERAS; A Cold-neutron disk-chopper spectrometer

Nakajima, Kenji; Kawamura, Seiko; Kofu, Maiko; Murai, Naoki; Inamura, Yasuhiro; Kikuchi, Tatsuya*; Wakai, Daisuke*

JPS Conference Proceedings (Internet), 33, p.011089_1 - 011089_7, 2021/03

The recent update of AMATERAS, a cold-neutron disk-chopper spectrometer at Japan Proton Accelerator Research Complex (J-PARC), is reported. AMATERAS has been operating for a decade. Since 2017, some updates have been done or are underway, which include installing new detectors, replacing the vacuum system of the scattering chamber, and other works. We are also working on the re-investigation of the resolution function. Demonstration measurements were carried out at 1MW test operations done in 2018 and 2019. Plans of upgrading the spectrometer are currently being considered.

Journal Articles

Freezable and unfreezable hydration water; Distinct contributions to protein dynamics revealed by neutron scattering

Yamamoto, Naoki*; Kofu, Maiko; Nakajima, Kenji; Nakagawa, Hiroshi; Shibayama, Naoya*

Journal of Physical Chemistry Letters (Internet), 12(8), p.2172 - 2176, 2021/03

 Times Cited Count:9 Percentile:66.28(Chemistry, Physical)

Hydration water plays a crucial role for activating the protein dynamics required for functional expression. Yet, the details are not understood about how hydration water couples with protein dynamics. A temperature hysteresis of the ice formation of hydration water is a key phenomenon to understand which type of hydration water, unfreezable or freezable hydration water, is crucial for the activation of protein dynamics. Using neutron scattering, we observed a temperature-hysteresis phenomenon in the diffraction peaks of the ice of freezable hydration water, whereas protein dynamics did not show any temperature hysteresis. These results show that the protein dynamics is not coupled with freezable hydration water dynamics, and unfreezable hydration water is essential for the activation of protein dynamics.

Journal Articles

Field-tuned magnetic structure and phase diagram of the honeycomb magnet YbCl$$_3$$

Hao, Y. Q.*; Wo, H. L.*; Gu, Y. M.*; Zhang, X. W.*; Gu, Y. Q.*; Zheng, S. Y.*; Zhao, Y.*; Xu, G. Y.*; Lynn, J. W.*; Nakajima, Kenji; et al.

Science China; Physics, Mechanics & Astronomy, 64(3), p.237411_1 - 237411_6, 2021/03

 Times Cited Count:6 Percentile:59.12(Physics, Multidisciplinary)

Journal Articles

Computational approach to the evaluation of fission product behaviors

Miwa, Shuhei; Nakajima, Kunihisa; Suzuki, Chikashi; Rizaal, M.; Suzuki, Eriko; Horiguchi, Naoki; Osaka, Masahiko

Proceedings of Joint International Conference on Supercomputing in Nuclear Applications + Monte Carlo 2020 (SNA + MC 2020), p.253 - 260, 2020/12

We have proceeded the fundamental study for the improvement of the evaluation of fission product (FP) chemistry and the treatment of fine space resolution which are main issues for the evaluation of FP behaviors in a severe accident (SA). We have been developing FP chemistry database named ECUME for the improvement of SA analysis codes. We prepared thermodynamic data for Cs compounds which is no experimental data available by computational approach. Regarding the space resolution issue, we have been developing analysis tool named CHASER based on 3D-CFD code with the model for FP chemistry. More accurate evaluation of FP behavior can be achieved by incorporating ECUME to the CHASER.

Journal Articles

Development of fission product chemistry database ECUME for the LWR severe accident

Miwa, Shuhei; Nakajima, Kunihisa; Miyahara, Naoya; Nishioka, Shunichiro; Suzuki, Eriko; Horiguchi, Naoki; Liu, J.; Miradji, F.; Imoto, Jumpei; Afiqa, B. M.; et al.

Mechanical Engineering Journal (Internet), 7(3), p.19-00537_1 - 19-00537_11, 2020/06

We constructed the fission product (FP) chemistry database named ECUME for LWR severe accident. This version of ECUME is equipped with dataset of the chemical reactions and their kinetics constants for the reactions of cesium(Cs)-iodine(I)-boron(B)-molybdenum(Mo)-oxygen(O)-hydrogen(H) system in gas phase, the elemental model for the high temperature chemical reaction of Cs with stainless steel applied as the structural material in a reactor, and thermodynamic data for CsBO$$_{2}$$ vapor species and solids of Cs$$_{2}$$Si$$_{4}$$O$$_{9}$$ and CsFeSiO$$_{4}$$ for these chemical reactions. The ECUME will provide estimation of Cs distribution due to the evaluation of effects of interaction with BWR control material B and stainless steel on Cs behavior in the Fukushima Daiichi Nuclear Power Station.

Journal Articles

$$q$$=0 long-range magnetic order in centennialite CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O; A Spin-$$frac{1}{2}$$ perfect kagome antiferromagnet with $$J_{1}$$-$$J_{2}$$-$$J_{d}$$

Iida, Kazuki*; Yoshida, Hiroyuki*; Nakao, Akiko*; Jeschke, H. O.*; Iqbal, Y.*; Nakajima, Kenji; Kawamura, Seiko; Munakata, Koji*; Inamura, Yasuhiro; Murai, Naoki; et al.

Physical Review B, 101(22), p.220408_1 - 220408_6, 2020/06

 Times Cited Count:22 Percentile:80.37(Materials Science, Multidisciplinary)

Crystal and magnetic structures of the mineral centennialite CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O are investigated by means of synchrotron X-ray diffraction and neutron diffraction measurements complemented by density functional theory (DFT) and pseudofermion functional renormalization group (PFFRG) calculations. In CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O, Cu$$^{2+}$$ ions form a geometrically perfect kagome network with antiferromagnetic $$J_{1}$$. No intersite disorder between Cu$$^{2+}$$ and Ca$$^{2+}$$ ions is detected. CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O enters a magnetic long-range ordered state below $$T_{rm N}$$ = 7.2 K, and the $$q$$=0 magnetic structure with negative vector spin chirality is obtained. The ordered moment at 0.3 K is suppressed to 0.58(2)$$mu$$B. Our DFT calculations indicate the presence of antiferromagnetic $$J_{2}$$ and ferromagnetic $$J_{d}$$ superexchange couplings of a strength which places the system at the crossroads of three magnetic orders (at the classical level) and a spin-$$frac{1}{2}$$ PFFRG analysis shows a dominance of $$q$$=0 type magnetic correlations, consistent with and indicating proximity to the observed $$q$$=0 spin structure. The results suggest that this material is located close to a quantum critical point and is a good realization of a $$J_{1}$$-$$J_{2}$$-$$J_{d}$$ kagome antiferromagnet.

Journal Articles

Lattice dynamics in FeSe via inelastic X-ray scattering and first-principles calculations

Murai, Naoki; Fukuda, Tatsuo; Nakajima, Masamichi*; Kawamura, Mitsuaki*; Ishikawa, Daisuke*; Tajima, Setsuko*; Baron, A. Q. R.*

Physical Review B, 101(3), p.035126_1 - 035126_6, 2020/01

 Times Cited Count:5 Percentile:31.64(Materials Science, Multidisciplinary)

We report an inelastic X-ray scattering investigation of phonons in FeSe superconductor. Comparing the experimental phonon dispersion with density functional theory (DFT) calculations in the non-magnetic state, we found a significant disagreement between them. A better overall agreement was obtained by allowing for spin-polarization in DFT calculations, despite the absence of magnetic order in FeSe. This calculation gives a realistic approximation, at DFT level, of the disordered paramagnetic state of FeSe, in which strong spin fluctuations are present.

Journal Articles

Experimental investigation of the suppressed superconducting gap and double-resonance mode in Ba$$_{1-x}$$K$$_{x}$$Fe$$_{2}$$As$$_{2}$$

Ideta, Shinichiro*; Murai, Naoki; Nakajima, Masamichi*; Kajimoto, Ryoichi; Tanaka, Kiyohisa*

Physical Review B, 100(23), p.235135_1 - 235135_7, 2019/12

 Times Cited Count:3 Percentile:15.75(Materials Science, Multidisciplinary)

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:8 Percentile:55.27(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Development of fission product chemistry database ECUME for the LWR severe accident

Miwa, Shuhei; Miyahara, Naoya; Nakajima, Kunihisa; Nishioka, Shunichiro; Suzuki, Eriko; Horiguchi, Naoki; Liu, J.; Miradji, F.; Imoto, Jumpei; Afiqa, B. M.; et al.

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 8 Pages, 2019/05

We constructed the first version of fission product (FP) chemistry database named ECUME for LWR severe accident. The first version of ECUME is equipped with dataset of the chemical reactions and their kinetics constants for the reactions of cesium(Cs)-iodine(I)-boron(B)-molybdenum(Mo)-oxygen(O)-hydrogen(H) system in gas phase, the elemental model for the high temperature chemical reaction of Cs with stainless steel, and thermodynamic data for CsBO$$_{2}$$ vapor species and solids of Cs$$_{2}$$Si$$_{4}$$O$$_{9}$$ and CsFeSiO$$_{4}$$. The ECUME will provide more accurate estimation of Cs distribution due to the evaluation of effects of interaction with BWR control material B and stainless steel on Cs behavior in the Fukushima Daiichi Nuclear Power Station.

Journal Articles

Structure analysis of the defects generated by a thermal spike in single crystal CeO$$_{2}$$; A Molecular dynamics study

Sasajima, Yasushi*; Ajima, Naoki*; Kaminaga, Ryuichi*; Ishikawa, Norito; Iwase, Akihiro*

Nuclear Instruments and Methods in Physics Research B, 440, p.118 - 125, 2019/02

 Times Cited Count:2 Percentile:22.69(Instruments & Instrumentation)

In the present paper, we have extensively analyzed the atomic structures generated by supplying a thermal spike to the single crystal CeO$$_{2}$$. Our analysis results were compared with the atomic structures obtained by the microscope experiments. Our simulation reproduced the distribution of the numbers of oxygen atoms obtained from the analysis of microscope images. We found that the number of vacancies was increased abruptly immediately after the thermal spike, and the number subsequently dropped through a relaxation process within 3 ps.

Journal Articles

Status report of the chopper spectrometer 4SEASONS

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Inamura, Yasuhiro; Kamazawa, Kazuya*; Ikeuchi, Kazuhiko*; Iida, Kazuki*; Ishikado, Motoyuki*; Murai, Naoki; Kira, Hiroshi*; Nakatani, Takeshi; et al.

Journal of Physics; Conference Series, 1021(1), p.012030_1 - 012030_6, 2018/06

BB2016-1727.pdf:0.39MB

 Times Cited Count:3 Percentile:88.20(Nuclear Science & Technology)

Journal Articles

Effect of electron correlations on spin excitation bandwidth in Ba$$_{0.75}$$K$$_{0.25}$$Fe$$_{2}$$As$$_{2}$$ as seen via time-of-flight inelastic neutron scattering

Murai, Naoki; Suzuki, Katsuhiro*; Ideta, Shinichiro*; Nakajima, Masamichi*; Tanaka, Kiyohisa*; Ikeda, Hiroaki*; Kajimoto, Ryoichi

Physical Review B, 97(24), p.241112_1 - 241112_6, 2018/06

 Times Cited Count:5 Percentile:25.26(Materials Science, Multidisciplinary)

We use inelastic neutron scattering (INS) to investigate the effect of electron correlations on spin dynamics in iron-based superconductor Ba$$_{0.75}$$K$$_{0.25}$$Fe$$_{2}$$As$$_{2}$$. Our INS data show a spin-wave-like dispersive feature, with a zone boundary energy of 200 meV. A first principles analysis of dynamical spin susceptibility, incorporating the mass renormalization factor of 3, as determined by angle-resolved photoemission spectroscopy, provides a reasonable description of the observed spin excitations. This analysis shows that electron correlations in the Fe-3d bands yield enhanced effective electron masses, and consequently, induce substantial narrowing of the spin excitation bandwidth. Our results highlight the importance of electron correlations in an itinerant description of the spin excitations in iron-based superconductors.

Journal Articles

Effect of magnetism on lattice dynamics in SrFe$$_2$$As$$_2$$ using high-resolution inelastic X-ray scattering

Murai, Naoki*; Fukuda, Tatsuo; Kobayashi, Tatsuya*; Nakajima, Masamichi*; Uchiyama, Hiroshi*; Ishikawa, Daisuke*; Tsutsui, Satoshi*; Nakamura, Hiroki; Machida, Masahiko; Miyasaka, Shigeki*; et al.

Physical Review B, 93(2), p.020301_1 - 020301_5, 2016/01

 Times Cited Count:7 Percentile:33.68(Materials Science, Multidisciplinary)

Journal Articles

JAEA-ISCN development programs of advanced NDA technologies of nuclear material

Seya, Michio; Kobayashi, Naoki; Naoi, Yosuke; Hajima, Ryoichi; Soyama, Kazuhiko; Kureta, Masatoshi; Nakamura, Hironobu; Harada, Hideo

Book of Abstracts, Presentations and Papers of Symposium on International Safeguards; Linking Strategy, Implementation and People (Internet), 8 Pages, 2015/03

JAEA-ISCN has been implementing basic development programs of the advanced NDA technologies for nuclear material (NM) since 2011JFY (Japanese Fiscal Year), which are (1) NRF (Nuclear resonance fluorescence) NDA technology using laser Compton scattered (LCS) $$gamma$$-rays (intense mono-energetic $$gamma$$-rays), (2) Alternative to $$^{3}$$He neutron detection technology using ZnS/B$$_{2}$$O$$_{3}$$ ceramic scintillator, and (3) NRD (Neutron resonance densitometry) using NRTA (Neutron resonance transmission analysis) and NRCA (Neutron resonance capture analysis). These programs are going to be finished in 2014JFY and have demonstration tests in February - March 2015.

Journal Articles

Basic technology development of advanced non-destructive detection / Measurement of nuclear material for nuclear security and nuclear nonproliferation

Seya, Michio; Naoi, Yosuke; Kobayashi, Naoki; Nakamura, Takahisa; Hajima, Ryoichi; Soyama, Kazuhiko; Kureta, Masatoshi; Nakamura, Hironobu; Harada, Hideo

Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-35-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2015/01

The Integrated Support Center for Nuclear Non-proliferation and Nuclear Security (ISCN) of Japan Atomic Energy Agency (JAEA) has been conducting (based on collaborations with JAEA other centers) the following basic technology development programs of advanced non-destructive detection/measurement of nuclear material for nuclear security and nuclear non-proliferation. (1) The demonstration test of the Pu-NDA system for spent fuel assembly using PNAR and SINRD (JAEA/USDOE(LANL) collaboration, completed in JFY2013), (2) Basic development of NDA technologies using laser Compton scattered $$gamma$$-rays (Demonstration of an intense mono-energetic $$gamma$$-ray source), (3) Development of alternative to He-3 neutron detection technology, (4) Development of neutron resonance densitometry (JAEA/JRC collaboration)This paper introduces above programs.

Journal Articles

Progress of manufacturing trials for the ITER toroidal field coil structures

Iguchi, Masahide; Morimoto, Masaaki; Chida, Yutaka*; Hemmi, Tsutomu; Nakajima, Hideo; Nakahira, Masataka; Koizumi, Norikiyo; Yamamoto, Akio*; Miyake, Takashi*; Sawa, Naoki*

IEEE Transactions on Applied Superconductivity, 24(3), p.3801004_1 - 3801004_4, 2014/06

 Times Cited Count:6 Percentile:35.46(Engineering, Electrical & Electronic)

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69 (Records 1-20 displayed on this page)