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Journal Articles

Strain-induced crystallization and phase separation used for fabricating a tough and stiff slide-ring solid polymer electrolyte

Hashimoto, Kei*; Shiwaku, Toru*; Aoki, Hiroyuki; Yokoyama, Hideaki*; Mayumi, Koichi*; Ito, Kozo*

Science Advances (Internet), 9(47), p.eadi8505_1 - eadi8505_8, 2023/11

 Times Cited Count:5 Percentile:86.76(Multidisciplinary Sciences)

Journal Articles

First observation of a nuclear $$s$$-state of a $$Xi$$ hypernucleus, $$^{15}_{Xi}{rm C}$$

Yoshimoto, Masahiro*; Fujita, Manami; Hashimoto, Tadashi; Hayakawa, Shuhei; Ichikawa, Yudai; Ichikawa, Masaya; Imai, Kenichi*; Nanamura, Takuya; Naruki, Megumi; Sako, Hiroyuki; et al.

Progress of Theoretical and Experimental Physics (Internet), 2021(7), p.073D02_1 - 073D02_19, 2021/07

 Times Cited Count:13 Percentile:79.65(Physics, Multidisciplinary)

Journal Articles

J-PARC E07; Systematic study of double strangeness system with hybrid emulsion method

Yoshida, Junya; Akaishi, Takaya; Fujita, Manami; Hasegawa, Shoichi; Hashimoto, Tadashi; Hosomi, Kenji; Ichikawa, Masaya; Ichikawa, Yudai; Imai, Kenichi*; Kim, S.; et al.

JPS Conference Proceedings (Internet), 33, p.011112_1 - 011112_8, 2021/03

Journal Articles

Observation of Coulomb-assisted nuclear bound state of $$Xi^-$$-$$^{14}$$N system

Hayakawa, Shuhei; Fujita, Manami; Hasegawa, Shoichi; Hashimoto, Tadashi; Hosomi, Kenji; Ichikawa, Yudai; Imai, Kenichi*; Nanamura, Takuya; Naruki, Megumi; Sako, Hiroyuki; et al.

Physical Review Letters, 126(6), p.062501_1 - 062501_6, 2021/02

 Times Cited Count:34 Percentile:94.71(Physics, Multidisciplinary)

Journal Articles

$$omega N$$ scattering length from $$omega$$ photoproduction on the proton near the reaction threshold

Ishikawa, Takatsugu*; Fujimura, Hisako*; Fukasawa, Hiroshi*; Hashimoto, Ryo*; He, Q.*; Honda, Yuki*; Hosaka, Atsushi; Iwata, Takahiro*; Kaida, Shun*; Kasagi, Jirota*; et al.

Physical Review C, 101(5), p.052201_1 - 052201_6, 2020/05

 Times Cited Count:4 Percentile:43.57(Physics, Nuclear)

Journal Articles

Observation of a Be double-Lambda hypernucleus in the J-PARC E07 experiment

Ekawa, Hiroyuki; Ashikaga, Sakiko; Hasegawa, Shoichi; Hashimoto, Tadashi; Hayakawa, Shuhei; Hosomi, Kenji; Ichikawa, Yudai; Imai, Kenichi; Kimbara, Shinji*; Nanamura, Takuya; et al.

Progress of Theoretical and Experimental Physics (Internet), 2019(2), p.021D02_1 - 021D02_11, 2019/02

 Times Cited Count:25 Percentile:83.09(Physics, Multidisciplinary)

Journal Articles

Electron-tracking Compton camera imaging of technetium-95m

Hatsukawa, Yuichi*; Hayakawa, Takehito*; Tsukada, Kazuaki; Hashimoto, Kazuyuki*; Sato, Tetsuya; Asai, Masato; Toyoshima, Atsushi; Tanimori, Toru*; Sonoda, Shinya*; Kabuki, Shigeto*; et al.

PLOS ONE (Internet), 13(12), p.e0208909_1 - e0208909_12, 2018/12

AA2018-0639.pdf:2.39MB

 Times Cited Count:3 Percentile:29.51(Multidisciplinary Sciences)

Imaging of $$^{95m}$$Tc radioisotope was conducted using an electron tracking-Compton camera (ETCC). $$^{95m}$$Tc emits 204, 582, and 835 keV $$gamma$$ rays, and was produced in the $$^{95}$$Mo(p,n)$$^{95m}$$Tc reaction with a $$^{95}$$Mo-enriched target. The recycling of the $$^{95}$$Mo-enriched molybdenum trioxide was investigated, and the recycled yield of $$^{95}$$Mo was achieved to be 70% - 90%. The images were obtained with each of the three $$gamma$$ rays. Results showed that the spatial resolution increases with increasing $$gamma$$-ray energy, and suggested that the ETCC with high-energy $$gamma$$-ray emitters such as $$^{95m}$$Tc is useful for the medical imaging of deep tissue and organs in the human body.

Journal Articles

Development of numerical analysis method for core thermal-hydraulics during natural circulation decay heat removal in SFR, 1; Validation of ASFRE code in estimation of radial heat transfer phenomena

Kikuchi, Norihiro; Doda, Norihiro; Hashimoto, Akihiko*; Yoshikawa, Ryuji; Tanaka, Masaaki; Ohshima, Hiroyuki

Dai-23-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (USB Flash Drive), 5 Pages, 2018/06

For the thermal-hydraulic design regarding a fuel assembly of sodium-cooled fast reactors, a subchannel analysis code ASFRE has been developed by JAEA. ASFRE was applied to numerical simulations of several kinds of water and sodium experiments as its validation studies and it was confirmed that pressure drops and temperature distributions measured in the experiments can be well reproduced. To enhance safety of sodium-cooled fast reactor, it is required to evaluate thermal-hydraulics in a core during decay heat removal by natural circulation. It is necessary to estimate radial heat transfer phenomena between fuel assemblies. In this study, a numerical simulation of a 37-pin bundle sodium experiment with radial heat flux was carried out and it was confirmed that ASFRE can be qualitatively reproduced temperature distributions in a fuel assembly affected by radial heat transfer.

Journal Articles

Shielding performance of newly developed boron-loaded concrete for DT neutrons

Sato, Satoshi*; Konno, Chikara; Nakashima, Hiroshi; Shionaga, Ryosuke*; Nose, Hiroyuki*; Ito, Yuji*; Hashimoto, Hirohide*

Journal of Nuclear Science and Technology, 55(4), p.410 - 417, 2018/04

 Times Cited Count:1 Percentile:11.24(Nuclear Science & Technology)

In order to enhance the neutron shielding performance, we developed concrete with boron of more than 10 wt%. We performed a neutron shielding experiment using the mockup of the newly developed boron-loaded concrete and DT neutrons at FNS in JAEA, and measured the reaction rates of the $$^{93}$$Nb(n,2n)$$^{92m}$$Nb and $$^{197}$$Au(n,$$gamma$$)$$^{198}$$Au reactions in the mockup. The calculations were conducted by using MCNP-5.14 and FENDL-2.1. The calculation results agreed well with the measured ones, and we confirmed that the accuracy was very good on the atomic composition data of the boron-loaded concrete and their nuclear data. In addition, we calculated effective dose rates and reaction rates of the $$^{59}$$Co(n,$$gamma$$)$$^{60}$$Co and $$^{151}$$Eu(n,$$gamma$$)$$^{152}$$Eu reactions in the boron-loaded concrete and other concretes. It is concluded that the boron-loaded concrete has much better shielding performance for DT neutrons than other concretes.

Journal Articles

Production of iodine radionuclides using $$^{7}$$Li ion beams

Nishinaka, Ichiro*; Yokoyama, Akihiko*; Washiyama, Koshin*; Makii, Hiroyuki; Hashimoto, Kazuyuki*

Journal of Radioanalytical and Nuclear Chemistry, 314(3), p.1947 - 1965, 2017/12

 Times Cited Count:2 Percentile:19.24(Chemistry, Analytical)

Production cross sections of iodine, tellurium and antimony radionuclides in the 24-59 MeV $$^{7}$$Li + $$^{nat}$$Sn reaction have been measured by the conventional stacked foil technique with $$gamma$$-ray spectrometry. Excitation functions of the production cross sections were compared with a statistical model calculation. The contributions of complete and incomplete fusion in the production of observed radionuclides are discussed from the view points of production routes in the nuclide chart and decays for iodine, tellurium and antimony nuclides. The integral yields of $$^{123,124,125,126}$$I were deduced from the calculated excitation functions in the $$^{7}$$Li induced reactions on Sn isotopes in view of the production of medically important $$^{123,124}$$I. The results are discussed by comparing with literature values in the other reactions.

Journal Articles

Development of thermal hydraulics analysis code ASFRE for fuel assembly of sodium-cooled fast reactor; Modification of distributed resistance model and validation analysis

Kikuchi, Norihiro; Ohshima, Hiroyuki; Tanaka, Masaaki; Hashimoto, Akihiko*

Dai-21-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (USB Flash Drive), 4 Pages, 2016/06

For the thermal-hydraulic design and safety assessment regarding a fuel assembly of sodium-cooled fast reactors, a subchannel analysis code ASFRE has been and is continuously developed in JAEA. In the numerical simulation of ASFRE confirmed that the tendency to overestimate the maximum coolant temperature in a fuel assembly still remains. In this study, Distributed Resistance Model (DRM), which deals with wire-spacer wrap volumetric effect in subchannels on peripheral and axial directions, was modified and its calibration factor was optimized in order to improve the prediction accuracy of the maximum coolant temperature. A numerical simulation of a 37-pin bundle sodium experiment was also carried out and the result showed the validity of the modified DRM.

Journal Articles

Development of numerical simulation system for thermal-hydraulic analysis in fuel assembly of sodium-cooled fast reactor

Ohshima, Hiroyuki; Uwaba, Tomoyuki; Hashimoto, Akihiko*; Imai, Yasutomo*; Ito, Masahiro*

AIP Conference Proceedings 1702, p.040011_1 - 040011_4, 2015/12

A numerical simulation system, which consists of a deformation analysis program and three kinds of thermal-hydraulics analysis programs, is being developed in Japan Atomic Energy Agency in order to offer methodologies to clarify thermal-hydraulic phenomena in fuel assemblies of sodium-cooled fast reactors under various operating conditions including fuel deformation. This paper gives a summary of numerical methods of component programs of the system and their validation studies.

Journal Articles

Optics tuning for beam collimation in the J-PARC 3-50 beam transport line

Harada, Hiroyuki; Meigo, Shinichiro; Shirakata, Masashi*; Sato, Yoichi*; Tamura, Fumihiko; Tejima, Masaki*; Hashimoto, Yoshinori*; Igarashi, Susumu*; Koseki, Tadashi

JPS Conference Proceedings (Internet), 8, p.012010_1 - 012010_6, 2015/09

The J-PARC 3-50BT line is the beam transport line from 3-GeV rapid-cycling synchrotron (RCS) to 50-GeV main ring (MR). The RCS is the high-intensity proton accelerator, where designed beam power is 1 MW, and has the complex source of space charge effect, etc. Therefore, the uncontrolled emittance growth and beam halo increase nonlinearly with the increasing the beam power. Additionally, the physical aperture of MR with 81 $$pi$$ mm mrad is smaller than that of RCS with 486 $$pi$$ mm mrad. Therefore, the 3-50BT line has the collimators in order to remove the tail or halo of the extracted beam from the RCS. The designed collimator aperture is 54 $$pi$$ mm mrad. It is required to measure and optimize the optics parameters in the collimator area for taking full advantage of the beam collimation. Especially, it is very important to make the dispersion functions free in the collimator area and optimize the beta function. This paper will introduce the method of optics measurement and report the result of the measurement and optimization based on the simulation.

Journal Articles

Production and separation of astatine isotopes in the $$^7$$Li + $$^{nat}$$Pb reaction

Nishinaka, Ichiro; Yokoyama, Akihiko*; Washiyama, Koshin*; Maeda, Eita*; Watanabe, Shigeki; Hashimoto, Kazuyuki; Ishioka, Noriko; Makii, Hiroyuki; Toyoshima, Atsushi; Yamada, Norihiro*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 304(3), p.1077 - 1083, 2015/06

 Times Cited Count:9 Percentile:60.04(Chemistry, Analytical)

Production cross sections of astatine isotopes $$^{207-211}$$At in the 29-57 MeV $$^7$$Li induced reaction with $$^{nat}$$Pb target have been measured by $$alpha$$- and $$gamma$$-ray spectrometry. Excitation functions of production cross sections have been compared with a statistical model calculation to study the reaction mechanism of $$^7$$Li + $$^{nat}$$Pb. Considerably small experimental cross sections of $$^{210}$$At and $$^{209}$$At compared with the calculation were clearly observed at incident energies higher than 44 MeV, indicating that the effects of breakup reaction play a role. A chemical separation of astatine from an irradiated lead target has been studied with a dry-distillation method. A complementary way to produce astatine isotopes has been developed.

Journal Articles

Beam instrumentation at the 1 MW Proton beam of J-PARC RCS

Yamamoto, Kazami; Hayashi, Naoki; Okabe, Kota; Harada, Hiroyuki; Saha, P. K.; Yoshimoto, Masahiro; Hatakeyama, Shuichiro; Hotchi, Hideaki; Hashimoto, Yoshinori*; Toyama, Takeshi*

Proceedings of 54th ICFA Advanced Beam Dynamics Workshop on High-Intensity, High Brightness and High Power Hadron Beams (HB 2014) (Internet), p.278 - 282, 2015/03

Rapid Cycling Synchrotron (RCS) of Japan Proton Accelerator Complex (J-PARC) is providing more than 300 kW of proton beam to Material and Life science Facility (MLF) and Main Ring (MR). Last summer shutdown, a new ion source was installed to increase output power to 1 MW. In order to achieve reliable operation of 1 MW, we need to reduce beam loss as well. Beam quality of such higher output power is also important for users. Therefore we developed new monitors that can measure the halo with higher accuracy. We present beam monitor systems for these purposes.

Journal Articles

Production of $$^{rm 95m}$$Tc for Compton camera imaging

Hatsukawa, Yuichi; Hashimoto, Kazuyuki; Tsukada, Kazuaki; Sato, Tetsuya; Asai, Masato; Toyoshima, Atsushi; Nagai, Yasuki; Tanimori, Toru*; Sonoda, Shinya*; Kabuki, Shigeto*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1283 - 1285, 2015/02

 Times Cited Count:2 Percentile:17.42(Chemistry, Analytical)

Technetium-99m ($$^{rm 99m}$$Tc) is used in radioactive medical diagonostic tests, for example as a radioactive tracer that medical equipment can detect in the human body. It is well suited to the role because it emits readily detectable 141 keV $$gamma$$ rays, and its half-life is 6.01 hours (meaning that about 94% of it decays to technetium-99 in 24 hours). There are at least 31 commonly used radiopharmaceuticals based on technetium-99m for imaging and functional studies of the brain, myocardium, thyroid, lungs, liver, gallbladder, kidneys, skeleton, blood, and tumors. Recent years, with the develop-ment of the Compton camera which can realize high position resolution, technetium isotopes emitting high energy $$gamma$$-rays are required. In this study, technetium-95m which emits some $$gamma$$ rays around 800 keV was produced by the $$^{95}$$Mo(p,n)$$^{rm 95m}$$Tc reaction.

Journal Articles

Optics tuning at the J-PARC 3-50BT line

Harada, Hiroyuki; Meigo, Shinichiro; Shirakata, Masashi*; Sato, Yoichi*; Tamura, Fumihiko; Tejima, Masaki*; Hashimoto, Yoshinori*; Igarashi, Susumu*; Koseki, Tadashi

Proceedings of 10th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.39 - 43, 2014/06

The J-PARC 3-50 BT line is the beam transport line of extracted beam from 3-GeV rapid-cycling synchrotron (RCS) to 50-GeV main ring (MR). The RCS is the high-intensity proton accelerator, which designed beam power is 1 MW, and has the complex source of space charge effect, etc. Therefore, the uncontrolled emittance growth and beam halo increase nonlinearly with the increasing the beam power. Additionally, physical aperture of MR with 81 $$pi$$ mm mrad is smaller than that of RCS with 486 $$pi$$ mm mrad. Therefore, the 3-50 BT line has the collimators in order to scrape the tail/halo of extracted beam from the RCS. The designed collimator aperture is 54 $$pi$$ mm mrad. It is required to measure and optimize the optics parameter in the collimator area for taking full advantage of beam collimation. This paper will introduce the method of optics measurement and report the result of the measurement and optimization based on the simulation.

Journal Articles

Surrogate reactions research at JAEA/Tokyo Tech

Chiba, Satoshi; Nishio, Katsuhisa; Makii, Hiroyuki; Aritomo, Yoshihiro*; Nishinaka, Ichiro; Ishii, Tetsuro; Tsukada, Kazuaki; Asai, Masato; Furutaka, Kazuyoshi; Hashimoto, Shintaro; et al.

Nuclear Data Sheets, 119, p.229 - 232, 2014/05

 Times Cited Count:0 Percentile:0.02(Physics, Nuclear)

Journal Articles

Theoretical study of sodium-water surface reaction mechanism

Kikuchi, Shin; Kurihara, Akikazu; Ohshima, Hiroyuki; Hashimoto, Kenro*

Journal of Power and Energy Systems (Internet), 6(2), p.76 - 86, 2012/06

In a sodium-cooled fast reactor (SFR), liquid sodium is used as heat transfer fluid to carry the energy from the reactor core to the steam generation (SG) system for power generation. If the heat transfer tube in the SG is failed, high pressurized water vapor blows into the liquid sodium and the sodium-water reaction (SWR) takes place. The extremely high-temperature reaction jet formed by the SWR, causes damage to the surface of the neighboring heat transfer tubes by thermal and chemical effects. Therefore, it is important to clearly understand the SWR for safety assessment of SG. In this study, we investigated the surface reaction mechanism in the SWR by ab initio method. The potential energy profiles of the dissociations of H$$_{2}$$O and OH were obtained. The estimated rate constant of the former was much larger than the latter.

Journal Articles

Reactivity of a water molecule at the liquid sodium surface

Kikuchi, Shin; Kurihara, Akikazu; Ohshima, Hiroyuki; Hashimoto, Kenro*

Nihon Genshiryoku Gakkai Wabun Rombunshi, 11(2), p.147 - 157, 2012/06

A breach of the heat transfer tube in a steam generator (SG) of a sodium-cooled fast reactor results in sodium-water reaction (SWR) by direct contact between liquid sodium and water vapor, which generates high temperature reaction jet. This reaction jet causes damage to the surface of neighboring heat transfer tubes by thermal and chemical effects. Therefore, it is important to clearly understand the SWR for safety assessment of SG. Regarding chemical effect, the surface and gas-phase reaction model are considered. As for the surface reaction, the water vapor encounters the liquid sodium, and the reaction occurs at their interface. Subsequently, the chemical reaction heating vaporizes the liquid sodium, causing the gas-phase reaction. However, there is limited knowledge on surface reaction because of extremely rapid-reaction. Therefore, in this study, ab-initio calculation was performed to evaluate the reaction path on surface reaction in SWR. The reaction path on dissociation of a water molecule at the liquid sodium surface was obtained. In addition, we also confirmed the generation mechanism of hydrogen in the liquid sodium.

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