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論文

DC transport in a dissipative superconducting quantum point contact

Visuri, A.-M.*; Mohan, J.*; 内野 瞬; Huang, M.-Z.*; Esslinger, T.*; Giamarchi, T.*

Physical Review Research (Internet), 5(3), p.033095_1 - 033095_11, 2023/08

粒子ロスのある量子ポイントコンタクト系のカレント・バイアス特性を研究する。Keldysh形式を採用し、チャンネルの透過率を変化させた場合のカレントを計算した。透過率の低い場合は、散逸により低バイアス領域でのカレントの増大、散逸に対する非単調性、輸送特性における新しい構造の出現が見られる。粒子ロスによる散逸の効果は、熱浴内の有限温度効果や非弾性散乱効果とは定性的に異なることがわかった。

論文

Superfluid signatures in a dissipative quantum point contact

Huang, M.-Z.*; Mohan, J.*; Visuri, A.-M.*; Fabritius, P.*; Talebi, M.*; Wili, S.*; 内野 瞬; Giamarchi, T.*; Esslinger, T.*

Physical Review Letters, 130(20), p.200404_1 - 200404_8, 2023/05

 被引用回数:1 パーセンタイル:83.24(Physics, Multidisciplinary)

スピン依存の局所的な粒子損失を伴う量子ポイントコンタクトを通して、強く相互作用する2成分フェルミ超流動輸送を測定した。高次の多重アンドレーフ反射によって実現される特徴的な非オーミック型超流動輸送は、散逸強度が超流動ギャップを超えると過剰オーミック電流に遷移することを観測した。我々は、散逸のあるサイトへのトンネル過程のある2端子の平均場モデルを開発した。Keldysh形式による計算では、観測された非平衡粒子電流を再現したが、観測された損失率やスピン流を完全に説明することはできなかった。

論文

Tensile overload-induced texture effects on the fatigue resistance of a CoCrFeMnNi high-entropy alloy

Lam, T.-N.*; Chin, H.-H.*; Zhang, X.*; Feng, R.*; Wang, H.*; Chiang, C.-Y.*; Lee, S. Y.*; 川崎 卓郎; Harjo, S.; Liaw, P. K.*; et al.

Acta Materialia, 245, p.118585_1 - 118585_9, 2023/02

 被引用回数:2 パーセンタイル:73.49(Materials Science, Multidisciplinary)

The present study investigates the crystallographic-texture effects on the improved fatigue resistance in the CoCrFeMnNi high-entropy alloys (HEAs) with the full-size geometry of the ASTM Standards E647-99. We exploited X-ray nano-diffraction mapping to characterize the crystal-deformation levels ahead of the crack tip after stress unloading under both constant- and tensile overloaded-fatigue conditions. The crack-tip blunting-induced much higher deformation level was concentrated surrounding the crack-tip which delays the fatigue-crack growth immediately after a tensile overload. The predominant deformation texture orientation in the Paris regime was investigated, using electron backscatter diffraction and orientation distribution function analyses. The twinning formation-driven shear deformation gave rise to the development of the Goss-type texture within the plastic deformation regime under a tensile-overloaded-fatigue condition, which was attributed to enhance the crack deflection and thus the tensile induced crack-growth-retardation period in the CoCrFeMnNi HEA.

論文

Two-dimensional quantum universality in the spin-1/2 triangular-lattice quantum antiferromagnet Na$$_{2}$$BaCo(PO$$_{4}$$)$$_{2}$$

Sheng, J.*; Wang, L.*; Candini, A.*; Jiang, W.*; Huang, L.*; Xi, B.*; Zhao, J.*; Ge, H.*; Zhao, N.*; Fu, Y.*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 119(51), p.e2211193119_1 - e2211193119_9, 2022/12

Although considerable progress has been made in the theoretical understanding of the low-dimensional frustrated quantum magnets, experimental realizations of a well-established scaling analysis are still scarce. This is particularly true for the two-dimensional antiferromagnetic triangular lattices. Owing to the small exchange strength, the newly discovered compound Na$$_{2}$$BaCo(PO$$_{4}$$)$$_{2}$$ provides a rare opportunity for clarifying the quantum criticality in an ideal triangular lattice with quantum spin S=1/2. In addition to the establishment of the complete phase diagrams, the spin Hamiltonian with a negligible interplane interaction has been determined through the spin wave dispersion in the polarized state, which is consistent with the observation of a two-dimensional quantum critical point with the Bose-Einstein condensation of diluted free bosons.

論文

Estimating fine melt pool, coarse melt pool, and heat affected zone effects on the strengths of additive manufactured AlSi10Mg alloys

Lam, T.-N.*; Lee, A.*; Chiu, Y.-R.*; Kuo, H.-F.*; 川崎 卓郎; Harjo, S.; Jain, J.*; Lee, S. Y.*; Huang, E.-W.*

Materials Science & Engineering A, 856, p.143961_1 - 143961_9, 2022/10

 被引用回数:2 パーセンタイル:48.15(Nanoscience & Nanotechnology)

Fine melt pool (FMP), coarse melt pool (CMP), and heat affected zone (HAZ) are generally observed in the additive manufactured AlSi10Mg alloys. In this study, we demonstrated that the yield strength can be estimated by the combination of the sizes and volume fractions of FMP, CMP, HAZ together with the second-phase hardening. Two different AlSi10Mg alloys fabricated via powder bed fusion (PBF) process were prepared to examine the lattice strain evolution of constituent phases during uniaxial tensile loading via in-situ neutron diffraction measurements. The horizontally-built (Hz-built) exhibited a much better yield and tensile strength as well as elongation compared to the vertically-built (Vt-built) AlSi10Mg alloy. We reported empirical strength quantification based on the sizes and ratios of fine melt pool (FMP), coarse melt pool (CMP), and heat affected zone (HAZ) together with the possible failure mode to prevent early fracture in the additive manufactured alloys.

論文

First observation of the decay of the 13/2$$^+$$ isomer in $$^{183}$$Hg and $$B$$(${it M}$2) systematics of neutron transitions across the nuclear chart

Huang, H.*; Zhang, W. Q.*; Andreyev, A. N.; Liu, Z.*; Seweryniak, D.*; Li, Z. H.*; Guo, C. Y.*; Barzakh, A. E.*; Van Duppen, P.*; Andel, B.*; et al.

Physics Letters B, 833, p.137345_1 - 137345_8, 2022/10

 被引用回数:0 パーセンタイル:0.02(Astronomy & Astrophysics)

The decay of the 13/2$$^+$$ isomeric state in $$^{183}$$Hg was observed for the first time following the $$alpha$$ decay of the 13/2$$^+$$ isomer in $$^{187}$$Pb produced in the $$^{142}$$Nd$$(^{50}$$Cr$$, 2p3n)$$ reaction. Using $$alpha$$-$$gamma$$ delayed coincidence measurements, the half-life of this isomer was measured to be 290(30) $$mu$$s. This isomer is proposed to deexcite by an unobserved low-energy $$M$$2 transition to the known 9/2$$^-$$ member of a strongly prolate-deformed 7/2$$^-$$[514] band, followed by a 105-keV $$M$$1 transition to the bandhead. A lower limit of B($$M$$2)$$geq$$0.018 W.u. was deduced for the unobserved transition. The presumed retardation is proposed to be due to the notable shape change between the initial, nearly spherical, and the final, strongly deformed, states. A similar scenario is also considered for the 13/2$$^+$$ isomer in $$^{181}$$Hg, suggesting both are cases of shape isomers. The B($$M$$2) systematics of neutron transitions across the nuclear chart is discussed.

論文

Identification of excited states in $$^{188}$$Bi and $$^{188}$$Po

Zhang, W. Q.*; Andreyev, A. N.; Liu, Z.*; Seweryniak, D.*; Huang, H.*; 他37名*

Physical Review C, 106(2), p.024317_1 - 024317_11, 2022/08

 被引用回数:1 パーセンタイル:34.54(Physics, Nuclear)

The neutron-deficient $$^{188}$$Bi and $$^{188}$$Po isotopes have been studied by $$gamma$$-ray spectroscopy using the recoil-decay tagging technique with the Argonne Gas-Filled Analyzer. A new 0.25(5)-micro second isomeric state and a prompt cascade formed by 319-, 366-, and 462-keV $$gamma$$ rays have been established on top of the (10$$^{-}$$) $$alpha$$-decaying isomer in $$^{188}$$Bi. The first excited (2$$^{+}$$) state in $$^{188}$$Po was identified, its excitation energy of 242(2) keV continues the nearly constant trend for the first 2$$^{+}$$ states in $$^{190,192,194}$$Po. The state is most likely a member of a prolate rotational band built on the ground state, albeit mixing with other coexisting configurations cannot be excluded. The new results obtained in the present work provide new information to shape coexistence in bismuth and polonium isotopes near the neutron midshell at $$N$$ = 104. In this mass region, a reduction in the prompt $$gamma$$-ray yield obtained with recoil decay tagging was observed for a few nuclides, and the possible reasons are presented.

論文

Fine structure in the $$alpha$$ decay of the 8$$^{+}$$ isomer in $$^{216,218}$$U

Zhang, M. M.*; Tian, Y. L.*; Wang, Y. S.*; Zhang, Z. Y.*; Gan, Z. G.*; Yang, H. B.*; Huang, M. H.*; Ma, L.*; Yang, C. L.*; Wang, J. G.*; et al.

Physical Review C, 106(2), p.024305_1 - 024305_6, 2022/08

 被引用回数:1 パーセンタイル:34.54(Physics, Nuclear)

The extremely neutron-deficient even-even uranium isotopes $$^{216,218}$$U were produced in the complete-fusion reactions induced by impinging $$^{40}$$Ar and $$^{40}$$Ca ions on $$^{180,182,184}$$W targets. Fusion evaporation residues were separated in flight by the gas-filled recoil separator SHANS (Spectrometer for Heavy Atoms and Nuclear Structure) and subsequently identified using the recoil-$$alpha$$-correlation method. In this paper, we report on new $$alpha$$-decay activities with $$E_{alpha} = 10163(27)$$ keV for $$^{216}$$U and $$E_{alpha} = 10073(16)$$ keV for $$^{218}$$U, which decay from the 8$$^{+}$$ isomeric states of $$^{216,218}$$U into the 2$$^{+}$$ states of their daughter nuclei $$^{212,214}$$Th, respectively. The new results extend the systematics of the $$alpha$$-decay fine structure for the $$N$$ = 124 and 126 even-even isotones.

論文

First observation of a shape isomer and a low-lying strongly-coupled prolate band in neutron-deficient semi-magic $$^{187}$$Pb

Zhang, W. Q.*; Andreyev, A. N.; Liu, Z.*; Seweryniak, D.*; Huang, H.*; Li, Z. H.*; Li, J. G.*; Guo, C. Y.*; 他34名*

Physics Letters B, 829, p.137129_1 - 137129_7, 2022/06

 被引用回数:3 パーセンタイル:78.01(Astronomy & Astrophysics)

Prompt and delayed $$gamma$$-ray spectroscopy of the neutron-deficient, semi-magic isotope $$^{187}$$Pb has been performed at the Argonne Gas-Filled Analyzer. A new 5.15(15)-$$mu$$s isomeric state at only 308 keV above the spherical 3/2$$^{-}$$ ground state is identified and classified as a shape isomer. A strongly-coupled band is observed on top of the isomer, which is nearly identical to the one built on the prolate 7/2$$^{-}$$[514] Nilsson state in the isotone $$^{185}$$Hg. Based on this similarity and on the result of the potential-energy surface calculations, the new isomer in $$^{187}$$Pb is proposed to originate from the same configuration. The retarded character of the 308-keV transition can be well explained by the significant difference between the prolate parent and spherical daughter configurations, leading to the shape isomerism. The combined results of the present work and the previous $$alpha$$-decay and laser spectroscopy studies present evidence for triple shape coexistence at low energy in the negative-parity configurations of $$^{187}$$Pb, which is well reproduced by the potential-energy surface calculations.

論文

Grain-size-dependent microstructure effects on cyclic deformation mechanisms in CoCrFeMnNi high-entropy-alloys

Luo, M.-Y.*; Lam, T.-N.*; Wang, P.-T.*; Tsou, N.-T.*; Chang, Y.-J.*; Feng, R.*; 川崎 卓郎; Harjo, S.; Liaw, P. K.*; Yeh, A.-C.*; et al.

Scripta Materialia, 210, p.114459_1 - 114459_7, 2022/03

 被引用回数:7 パーセンタイル:92.51(Nanoscience & Nanotechnology)

The effect of grain size on strain-controlled low-cycle fatigue (LCF) properties in the CoCrFeMnNi high-entropy alloys (HEAs) was investigated towards the distinct microstructural developments during cyclic loading at a strain amplitude of $$pm$$ 1.0%. A much more prominent secondary cyclic hardening (SCH) behavior at the final deformation stage was observed in the fine-grained (FG) than in the coarse-grained (CG) CoCrFeMnNi. In-situ neutron-diffraction and microscopic examination, strongly corroborated by molecular dynamic (MD) simulations, indicated that dislocation activities from planar slip to wavy slip-driven subgrain structures within the grains acted as the primary cyclic-deformation behaviors in the FG CoCrFeMnNi. Differently observed in the cyclic behavior of the CG CoCrFeMnNi was due to a transition from the planar dislocation slip to twinning.

論文

Tensile response of as-cast CoCrFeNi and CoCrFeMnNi high-entropy alloys

Lam, T.-N.*; Luo, M.-Y.*; 川崎 卓郎; Harjo, S.; Jain, J.*; Lee, S.-Y.*; Yeh, A.-C.*; Huang, E.-W.*

Crystals (Internet), 12(2), p.157_1 - 157_9, 2022/02

 被引用回数:3 パーセンタイル:88.59(Crystallography)

In this research, we systematically investigated equiatomic CoCrFeNi and CoCrFeMnNi high-entropy alloys (HEAs). Both of these HEA systems are single-phase, face-centered-cubic (FCC) structures. Specifically, we examined the tensile response in as-cast quaternary CoCrFeNi and quinary CoCrFeMnNi HEAs at room temperature. Compared to CoCrFeNi HEA, the elongation of CoCrFeMnNi HEA was 14% lower, but the yield strength and ultimate tensile strength were increased by 17% and 6%, respectively. The direct real-time evolution of structural defects during uniaxial straining was acquired via in situ neutron-diffraction measurements. The dominant microstructures underlying plastic deformation mechanisms at each deformation stage in as-cast CoCrFeNi and CoCrFeMnNi HEAs were revealed using the Convolutional Multiple Whole Profile (CMWP) software for peak-profile fitting. The possible mechanisms are reported.

論文

Solving the puzzles of the decay of the heaviest known proton-emitting nucleus $$^{185}$$Bi

Doherty, D. T.*; Andreyev, A. N.; Seweryniak, D.*; Woods, P. J.*; Carpenter, M. P.*; Auranen, K.*; Ayangeakaa, A. D.*; Back, B. B.*; Bottoni, S.*; Canete, L.*; et al.

Physical Review Letters, 127(20), p.202501_1 - 202501_6, 2021/11

 被引用回数:4 パーセンタイル:66.91(Physics, Multidisciplinary)

$$^{185}$$Bi is the heaviest known proton emitting isotope. Its decay had been observed, but the assumed ground-state lifetime ($$sim$$$$60~mu$$s) was incorrect, leading to unexplained hindrance. With two new experiments at Argonne National Laboratory, two states were clearly identified. One is the proton-emitting ground-state (spin 1/2$$^+$$, half-life: 2.8$$^{+2.3}_{-1.0}$$ $$mu$$s), the second is a 58(2) $$mu$$s $$gamma$$-decaying isomer. The new data show the inversion of the ground and isomeric states compared to neighboring Bi isotopes. This is the only known example of a ground-state proton decay to a daughter nucleus ($$^{184}$$Pb) with a major shell closure.

論文

Development of a reference database for beta-delayed neutron emission

Dimitriou, P.*; Dillmann, I.*; Singh, B.*; Piksaikin, V.*; Rykaczewski, K. P.*; Tain, J. L.*; Algora, A.*; Banerjee, K.*; Borzov, I. N.*; Cano-Ott, D.*; et al.

Nuclear Data Sheets, 173, p.144 - 238, 2021/03

 被引用回数:16 パーセンタイル:96.48(Physics, Nuclear)

核分裂の発見以降、核分裂片から放出される遅発中性子の存在には、数多くの関心が集められてきた。原子力発電では、遅発中性子は原子炉動特性の計算や炉の安全運転において非常に重要な役割を演じている。それに加え、遅発中性子は、核構造や天体核、特に新世代のRIビーム施設の中心課題である安定線から離れた原子核でも、大きなインパクトをもっている。現在、ベータ崩壊半減期と遅発中性子分岐比に関するいくつかの文献が利用可能であるが、測定と評価によって実施されるべき十分な考証は、それらの文献ではしばしば抜けている。この欠落部に注目し、遅発中性子の核データ評価とそれに関する新しい文献作成の作業が、国際原子力機関(IAEA)の援助の基に着手され、「ベータ遅発中性子用データベースの開発」に関するCoordinated Research Project (CRP)が結成された。本論文では、CRPで行われたこれまでの結果について報告をする。

論文

Enhancement of fatigue resistance by overload-induced deformation twinning in a CoCrFeMnNi high-entropy alloy

Lam, T.-N.*; Lee, S. Y.*; Tsou, N.-T.*; Chou, H.-S.*; Lai, B.-H.*; Chang, Y.-J.*; Feng, R.*; 川崎 卓郎; Harjo, S.; Liaw, P. K.*; et al.

Acta Materialia, 201, p.412 - 424, 2020/12

 被引用回数:31 パーセンタイル:91.93(Materials Science, Multidisciplinary)

We examined fatigue-crack-growth behaviors of CoCrFeMnNi high-entropy alloys (HEAs) under as-fatigued and tensile-overloaded conditions using neutron-diffraction measurements coupled with diffraction peak-profile analyses. We applied both high-resolution transmission electron microscopy (HRTEM) and neutron-diffraction strain mapping for the complementary microstructure examinations. Immediately after a single tensile overload, the crack-growth-retardation period was obtained by enhancing the fatigue resistance, as compared to the as-fatigued condition. The combined mechanisms of the overload-induced larger plastic deformation, the enlarged compressive residual stresses and plastic-zone size, the crack-tip blunting ahead of the crack tip, and deformation twinning governed the pronounced macroscopic crack-growth-retardation behavior following the tensile overload.

論文

International network of nuclear structure and decay data evaluators

Dimitriou, P.*; Basunia, S*; Bernstein, L.*; Chen, J.*; Elekes, Z.*; Huang, X.*; Hurst, A.*; 飯村 秀紀; Jain, A. K.*; Kelley, J.*; et al.

EPJ Web of Conferences, 239, p.15004_1 - 15004_4, 2020/09

BB2020-0008.pdf:0.34MB

 被引用回数:0 パーセンタイル:0.1

評価済み核構造データファイル(Evaluated Nuclear Structure Data File: ENSDF)は、原子核構造と崩壊に関する様々な実験データを全ての核種について集めて、それらの実験データの評価値を与えてある世界唯一のデータファイルである。ENSDFは定期的に更新されており、そのための評価作業は各国の評価者で分担している。評価作業を速やかに行うために、IAEAの援助の下に評価者の国際的なネットワークが組織されている。この発表では、ネットワークの最近の活動のうち、ENSDFの処理コードの開発、測定が必要とされているデータのリストの作成、インターネット版核図表の利用の拡充などについて報告する。また、核構造・崩壊データの需要が増大しているにもかかわらず、評価者が減っている問題についても述べる。

論文

Signatures of the vortical quark-gluon plasma in hadron yields

田屋 英俊*; Park, A.*; Cho, S.*; Gubler, P.; 服部 恒一*; Hong, J.*; Huang, X.-G.*; Lee, S. H.*; 門内 明彦*; 大西 明*; et al.

Physical Review C, 102(2), p.021901_1 - 021901_6, 2020/08

AA2020-0306.pdf:0.47MB

 被引用回数:7 パーセンタイル:70.75(Physics, Nuclear)

We investigate the hadron production from the vortical quark-gluon plasma created in heavy-ion collisions. Based on the quark-coalescence and statistical hadronization models, we show that total hadron yields summed over the spin components are enhanced by the local vorticity with quadratic dependence. The enhancement factor amounts to be a few percent and may be detectable within current experimental sensitivities. We also show that the effect is stronger for hadrons with larger spin, and thus propose a new signature of the local vorticity, which may be detected by the yield ratio of distinct hadron species having different spins such as $$phi$$ and $$eta'$$. The vorticity dependence of hadron yields seems robust, with consistent predictions in both of the hadron production mechanisms for reasonable values of the vorticity strength estimated for heavy-ion collisions.

論文

Electronic structure of a (3$$times$$3)-ordered silicon layer on Al(111)

佐藤 祐輔*; 深谷 有喜; Cameau, M.*; Kundu, A. K.*; 志賀 大亮*; 湯川 龍*; 堀場 弘司*; Chen, C.-H.*; Huang, A.*; Jeng, H.-T.*; et al.

Physical Review Materials (Internet), 4(6), p.064005_1 - 064005_6, 2020/06

 被引用回数:6 パーセンタイル:31.82(Materials Science, Multidisciplinary)

本研究では、放射光角度分解光電子分光を用いて、Al(111)表面上の3$$times$$3周期を持つSi層の電子バンド構造を解明した。実験では、線形のエネルギー分散に起因する閉じたフェルミ面を観測した。ハニカム状のシリセンをモデル構造とした第一原理計算の結果、これは基板との混成状態を起源としたディラックコーン様の金属バンドと考えられる。Al(111)表面上のSi層は、基板との相互作用によりディラック電子を発現し、いわゆるXeneと呼ばれる2次元物質群のモデルシステムになりうることを示唆する。

論文

Fine structure in the $$alpha$$ decay of $$^{223}$$U

Sun, M. D.*; Liu, Z.*; Huang, T. H.*; Zhang, W. Q.*; Andreyev, A. N.; Ding, B.*; Wang, J. G.*; Liu, X. Y.*; Lu, H. Y.*; Hou, D. S.*; et al.

Physics Letters B, 800, p.135096_1 - 135096_5, 2020/01

 被引用回数:10 パーセンタイル:80.2(Astronomy & Astrophysics)

Fine structure in the $$alpha$$ decay of $$^{223}$$U was observed in the fusion-evaporation reaction $$^{187}$$Re($$^{40}$$Ar,p3n) by using fast digital pulse processing technique. Two $$alpha$$-decay branches of $$^{223}$$U feeding the ground state and 244 keV excited state of $$^{219}$$Th were identified by establishing the decay chain $$^{223}$$U$$rightarrow$$$$^{219}$$Th$$rightarrow$$$$^{215}$$Ra$$rightarrow$$$$^{211}$$Rn. The $$alpha$$-particle energy for the ground-state to ground-state transition of $$^{223}$$U was determined to be 8993(17) keV, 213 keV higher than the previous value, the half-life was updated to be 62$$^{+14}_{-10} mu$$s. Evolution of nuclear structure for $$N$$=131 even-$$Z$$ isotones from Po to U was discussed in the frameworks of nuclear mass and reduced $$alpha$$-decay width, a weakening octupole deformation in the ground state of $$^{223}$$U relative to its lighter isotones $$^{219}$$Ra and $$^{211}$$Th was suggested.

論文

Comparing cyclic tension-compression effects on CoCrFeMnNi high-entropy alloy and Ni-based superalloy

Lam, T.-N.*; Chou, Y.-S.*; Chang, Y.-J.*; Sui, T.-R.*; Yeh, A.-C.*; Harjo, S.; Lee, S. Y.*; Jain, J.*; Lai, B.-H.*; Huang, E.-W.*

Crystals (Internet), 9(8), p.420_1 - 420_8, 2019/08

AA2019-0503.pdf:1.06MB

 被引用回数:9 パーセンタイル:68.5(Crystallography)

An equal-molar CoCrFeMnNi, face-centered-cubic (fcc) high-entropy alloy (HEA) and a nickel-based superalloy are studied using in situ neutron diffraction experiments. With continuous measurements, the evolution of diffraction peaks is collected for microscopic lattice strain analyses. Cyclic hardening and softening are found in both metallic systems. However, as obtained from the diffraction-peak-width evolution, the underneath deformation mechanisms are quite different. The CoCrFeMnNi HEA exhibits distinct lattice strain and microstructure responses under tension-compression cyclic loadings.

論文

Super-absorbent polymer valves and colorimetric chemistries for time-sequenced discrete sampling and chloride analysis of sweat via skin-mounted soft microfluidics

Kim, S. B.*; Zhang, Y.*; Won, S. M.*; Bandodkar, A. J.*; 関根 由莉奈; Xue, Y.*; Koo, J.*; Harshman, S. W.*; Martin, J. A.*; Park, J. M.*; et al.

Small, 14(12), p.1703334_1 - 1703334_11, 2018/03

 被引用回数:86 パーセンタイル:95.48(Chemistry, Multidisciplinary)

This paper introduces super absorbent polymer valves and colorimetric sensing reagents as enabling components of soft, skin-mounted microfluidic devices designed to capture, store and chemically analyze sweat released from eccrine glands. The valving technology enables robust means for guiding the flow of sweat from an inlet location into a collection of isolated reservoirs, in a well-defined sequence. Analysis in these reservoirs involves a color responsive indicator of chloride concentration with a formulation tailored to offer stable operation with sensitivity optimized for the relevant physiological range. Evaluations on human subjects with comparisons against ex situ analysis illustrate the practical utility of these advances.

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