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論文

Fabrication of (Bi$$_2$$)$$_m$$(Bi$$_2$$Te$$_3$$)$$_n$$ superlattice films by Te desorption from a pristine Bi$$_2$$Te$$_3$$ film

日下 翔太郎*; 佐々木 泰祐*; 角田 一樹; 一ノ倉 聖*; 出田 真一郎*; 田中 清尚*; 宝野 和博*; 平原 徹*

Applied Physics Letters, 120(17), p.173102_1 - 173102_5, 2022/04

 被引用回数:2 パーセンタイル:34.67(Physics, Applied)

We fabricated superlattice films composed of Bi$$_2$$ bilayers (BLs) and Bi$$_2$$Te$$_3$$ quintuple layers (QLs) by annealing pure Bi$$_2$$Te$$_3$$ films. It was found that Te desorbs from the QL to form the BL with an activation energy of 2.7 eV. Eventually two distinct stoichiometric phases were formed, Bi$$_1$$Te$$_1$$ (QL-BL-QL) and Bi$$_4$$Te$$_3$$ (QL-BL), as evidenced by scanning transmission emission microscopy measurements. The surface-state dispersion was measured with angle-resolved photoemission spectroscopy and the topological nature of each sample is discussed. Our method offers a convenient and simple way to fabricate superlattice films with different topological properties.

論文

Absence of ferromagnetism in MnBi$$_2$$Te$$_4$$/Bi$$_2$$Te$$_3$$ down to 6 K

深澤 拓朗*; 日下 翔太郎*; 角田 一樹; 橋爪 瑞葵*; 一ノ倉 聖*; 竹田 幸治; 出田 真一郎*; 田中 清尚*; 清水 亮太*; 一杉 太郎*; et al.

Physical Review B, 103(20), p.205405_1 - 205405_6, 2021/05

 被引用回数:9 パーセンタイル:66.35(Materials Science, Multidisciplinary)

We successfully fabricated a MnBi$$_2$$Te$$_4$$/Bi$$_2$$Te$$_3$$ heterostructure by incorporating Mn and Te inside the topmost quintuple layer of Bi$$_2$$Te$$_3$$, as unambiguously confirmed by LEED I-V scanning transmission electron microscopy measurements. The surface-state Dirac cone of the heterostructure showed little change compared to that of the pristine Bi$$_2$$Te$$_3$$ and X-ray magnetic circular dichroism measurements showed that the system was paramagnetic down to 5.6 K. These results are in contrast to the previous works on related materials that showed magnetic order around 10 K as well as theoretical predictions and suggests the intricacy of the magnetic properties of two-dimensional van der Waals magnets.

論文

Fabrication of a novel magnetic topological heterostructure and temperature evolution of its massive Dirac cone

平原 徹*; Otrokov, M. M.*; 佐々木 泰祐*; 角田 一樹*; 友弘 雄太*; 日下 翔太郎*; 奥山 裕磨*; 一ノ倉 聖*; 小林 正起*; 竹田 幸治; et al.

Nature Communications (Internet), 11, p.4821_1 - 4821_8, 2020/09

 被引用回数:41 パーセンタイル:93.11(Multidisciplinary Sciences)

We fabricate a novel magnetic topological heterostructure Mn$$_{4}$$Bi$$_{2}$$Te$$_{7}$$/Bi$$_{2}$$Te$$_{3}$$ where multiple magnetic layers are inserted into the topmost quintuple layer of the original topological insulator Bi$$_{2}$$Te$$_{3}$$. A massive Dirac cone (DC) with a gap of 40-75 meV at 16 K is observed. By tracing the temperature evolution, this gap is shown to gradually decrease with increasing temperature and a blunt transition from a massive to a massless DC occurs around 200-250 K. Magnetic measurements show that there are two distinct Mn components in the system that corresponds to the two heterostructures; MnBi$$_{2}$$Te$$_{4}$$/Bi$$_{2}$$Te$$_{3}$$ is paramagnetic at 6 K while Mn$$_{4}$$Bi$$_{2}$$Te$$_{7}$$/Bi$$_{2}$$Te$$_{3}$$ is ferromagnetic with a negative hysteresis (critical temperature 20 K). This novel heterostructure is potentially important for future device applications.

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