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伊藤 孝; 門野 良典*
Journal of the Physical Society of Japan, 93(4), p.044602_1 - 044602_7, 2024/04
We propose a model to describe the fluctuations in the internal magnetic field due to ion dynamics observed in muon spin relaxation (
SR) by an Edwards-Anderson-type autocorrelation function that separates the quasi-static and dynamic components of the correlation by the parameter 
(where 
). Our Monte Carlo simulations for this model showed that the time evolution of muon spin polarization deviates significantly from the Kubo-Toyabe function. To further validate the model, the results of simulations were compared with the SR spectra observed in a hybrid organic-inorganic perovskite FAPbI
[with FA referring to HC(NH
)], where local field fluctuations associated with the rotational motion of FA molecules and quasi-static fields from the PbI lattice are presumed to coexist. The least-squares curve fitting showed reasonable agreement with the model with 
, and the fluctuation frequency of the dynamical component was obtained. This result opens the door to the possibility of experimentally distinguishing fluctuations due to the dynamics of ions around muons from those due to the self-diffusion of muons. On the other hand, it suggests the need to carefully consider the spin relaxation function when applying SR to the issue of ion dynamics.
inferred from muon study門野 良典*; 平石 雅俊*; 岡部 博孝*; 幸田 章宏*; 伊藤 孝
Journal of Physics; Condensed Matter, 35(28), p.285503_1 - 285503_13, 2023/07
被引用回数：0 パーセンタイル：0(Physics, Condensed Matter)Magnesium hydride has great potential as a solid hydrogen (H) storage material because of its high H storage capacity of 7.6 wt%. However, its slow hydrogenation and dehydrogenation kinetics and the high temperature of 300 
C required for decomposition are major obstacles to small-scale applications such as automobiles. The local electronic structure of interstitial H in MgH is an important fundamental knowledge in solving this problem, which has been studied mainly based on density functional theory (DFT). However, few experimental studies have been performed to assess the results of DFT calculations. We have therefore introduced muon (Mu) as pseudo-H into MgH and investigated the corresponding interstitial H states by analyzing their electronic and dynamical properties in detail. As a result, we observed multiple Mu states similar to those observed in wide-gap oxides, and found that their electronic states can be attributed to relaxed-excited states associated with donor/acceptor levels predicted by the recently proposed ambipolarity model. This provides an indirect support for the DFT calculations on which the model is based via the donor/acceptor levels. An important implication of the muon results for improved hydrogen kinetics is that dehydrogenation, serving as a reduction for hydrides, stabilises the interstitial H
state.
下村 浩一郎*; 幸田 章宏*; Pant, A. D.*; 名取 寛顕*; 藤森 寛*; 梅垣 いづみ*; 中村 惇平*; 反保 元伸*; 河村 成肇*; 手島 菜月*; et al.
Journal of Physics; Conference Series, 2462, p.012033_1 - 012033_5, 2023/03
被引用回数：0 パーセンタイル：0.2(Physics, Applied)At J-PARC MUSE, since the SR2017 conference and up to FY2022, there have been several new developments at the facility, including the completion of a new experimental area S2 at the surface muon beamline S-line and the first muon beam extraction to the H1 area in the H-line, mainly to carry out high-statistics fundamental physics experiments. Several new studies are also underway, such as applying negative muon non-destructive elemental analysis to the analysis of samples returned from the asteroid Ryugu in the D2 area of the D-line. This paper reports on the latest status of MUSE.
大熊 隆太郎*; 古府 麻衣子; 浅井 晋一郎*; Avdeev, M.*; 幸田 章宏*; 岡部 博孝*; 平石 雅俊*; 竹下 聡史*; 小嶋 健児*; 門野 良典*; et al.
Nature Communications (Internet), 12, p.4382_1 - 4382_7, 2021/07
被引用回数：6 パーセンタイル：61.42(Multidisciplinary Sciences)Dimensionality is a critical factor in determining the properties of solids and is an apparent built- in character of the crystal structure. However, it can be an emergent and tunable property in geometrically frustrated spin systems. Here, we study the spin dynamics of the tetrahedral cluster antiferromagnet, pharmacosiderite, via muon spin resonance and neutron scattering. We find that the spin correlation exhibits a two-dimensional characteristic despite the isotropic connectivity of tetrahedral clusters made of spin 5/2 Fe
ions in the three-dimensional cubic crystal, which we ascribe to two-dimensionalisation by geometrical frustration based on spin wave calculations. Moreover, we suggest that even one-dimensionalisation occurs in the decoupled layers, generating low-energy and one-dimensional excitation modes, causing large spin fluctuation in the classical spin system.
Miao, P.*; Tan, Z.*; Lee, S. H.*; 石川 喜久*; 鳥居 周輝*; 米村 雅雄*; 幸田 章宏*; 小松 一生*; 町田 真一*; 佐野 亜沙美; et al.
Physical Review B, 103(9), p.094302_1 - 094302_18, 2021/03
被引用回数：2 パーセンタイル：17.84(Materials Science, Multidisciplinary)層状ペロブスカイトPrBaCo
O
は、熱膨張のない複合材料を作るために必要な負の熱膨張(NTE)を示す。NTEは、自発的な磁気秩序と密接に関連していることがわかっていた(磁気体積効果: MVE)。今回、われわれは、PrBaCoOの連続的な磁気体積効果が、本質的には不連続であり、大きな体積を持つ反強磁性絶縁体(AFILV)から、小さな体積をもつ強磁性卑絶縁体(FLISV)への磁気電気的相転移に起因することを明らかにした。また、磁気電気効果(ME)は、温度,キャリアドーピング,静水圧,磁場などの複数の外部刺激に対して高い感度を示した。これは、これまでよく知られている対称性の破れを伴う巨大磁気抵抗やマルチフェロイック効果などのMEとは対照的であり、輝コバルト鉱のMEは同一の結晶構造で起こる。われわれの発見は、MEとNTEを実現するための新しい方法を示しており、それは新しい技術に応用されるかもしれない。
D
measured with inelastic neutron spectroscopy山浦 淳一*; 平賀 晴弘*; 飯村 壮史*; 村場 善行*; Bang, J.*; 池内 和彦*; 中村 充孝; 稲村 泰弘; 本田 孝志*; 平石 雅俊*; et al.
Physical Review B, 99(22), p.220505_1 - 220505_6, 2019/06
被引用回数：3 パーセンタイル：16.31(Materials Science, Multidisciplinary)鉄系超伝導体LaFeAsODの非弾性中性子散乱実験により、超伝導転移温度26K以下において、5-15meVのエネルギー領域に新しい励起が生じることを見出した。なお、この励起は母物質であるLaFeAsOFでは現れない。14.5meVと11.1meVに現れる強い励起は水素の量子ラットリングまたはバンド運動に起因し、格子間サイトが2個以上のポテンシャル極小点を有する場合にのみ出現するものと結論付けた。
Mo
O
( = In, Sc)飯田 一樹*; 吉田 紘行*; 岡部 博孝*; 片山 尚幸*; 石井 裕人*; 幸田 章宏*; 稲村 泰弘; 村井 直樹; 石角 元志*; 門野 良典*; et al.
Scientific Reports (Internet), 9(1), p.1826_1 - 1826_9, 2019/02
被引用回数：9 パーセンタイル：59.53(Multidisciplinary Sciences)Molecular based spin-1/2 triangular lattice systems have attracted research interest. LiMoO
( = In or Sc) is such a compound where spin-1/2 MoO
clusters in place of Mo ions form the uniform triangular lattice. Here, we report exotic magnetisms in LiInMoO and LiScMoO investigated by muon spin rotation (SR) and inelastic neutron scattering (INS) spectroscopies. LiInMoO exhibits spin wave excitation which is quantitatively described by the nearest neighbor anisotropic Heisenberg model based on the 120
spin structure. In contrast, LiScMoO undergoes short-range magnetic order below 4 K with quantum-spin-liquid-like magnetic fluctuations down to the base temperature. Origin of the different ground states is discussed in terms of anisotropies of crystal structures and magnetic interactions.
Strasser, P.*; 阿部 充志*; 青木 正治*; Choi, S.*; 深尾 祥紀*; 東 芳隆*; 樋口 嵩*; 飯沼 裕美*; 池戸 豊*; 石田 勝彦*; et al.
EPJ Web of Conferences, 198, p.00003_1 - 00003_8, 2019/01
被引用回数：13 パーセンタイル：99.06(Quantum Science & Technology)High precision measurements of the ground state hyperfine structure (HFS) of muonium is a stringent tool for testing bound-state quantum electrodynamics (QED) theory, determining fundamental constants of the muon magnetic moment and mass, and searches for new physics. Muonium is the most suitable system to test QED because both theoretical and experimental values can be precisely determined. Previous measurements were performed decades ago at LAMPF with uncertainties mostly dominated by statistical errors. At the J-PARC Muon Science Facility (MUSE), the MuSEUM collaboration is planning complementary measurements of muonium HFS both at zero and high magnetic field. The new high-intensity muon beam that will soon be available at H-Line will provide an opportunity to improve the precision of these measurements by one order of magnitude. An overview of the different aspects of these new muonium HFS measurements, the current status of the preparation for high-field measurements, and the latest results at zero field are presented.
上野 恭裕*; 青木 正治*; 深尾 祥紀*; 東 芳隆*; 樋口 嵩*; 飯沼 裕美*; 池戸 豊*; 石田 勝彦*; 伊藤 孝; 岩崎 雅彦*; et al.
Hyperfine Interactions, 238(1), p.14_1 - 14_6, 2017/11
被引用回数：3 パーセンタイル：86.59(Physics, Atomic, Molecular & Chemical)MuSEUM is an international collaboration aiming at a new precise measurement of the muonium hyperfine structure at J-PARC (Japan Proton Accelerator Research Complex). Utilizing its intense pulsed muon beam, we expect a ten-fold improvement for both measurements at high magnetic field and zero magnetic field. We have developed a sophisticated monitoring system, including a beam profile monitor to measure the 3D distribution of muonium atoms to suppress the systematic uncertainty.
髭本 亘; 門野 良典*; 河村 成肇*; 幸田 章宏*; 小嶋 健児*; 牧村 俊助*; 的場 史朗*; 三宅 康博*; 下村 浩一郎*; Strasser, P.*
Quantum Beam Science (Internet), 1(1), p.11_1 - 11_24, 2017/06
ミュオン科学実験施設はJ-PARCにおいて中性子, ハドロン, ニュートリノ各施設と並ぶ利用施設である。ミュオン施設では、物質生命科学実験棟において中性子実験施設と共有している高エネルギーの陽子により発生させたミュオンを用いて様々な科学研究に用いている。本レビューではミュオン科学実験施設の現状について報告する。
Strasser, P.*; 青木 正治*; 深尾 祥紀*; 東 芳隆*; 樋口 嵩*; 飯沼 裕美*; 池戸 豊*; 石田 勝彦*; 伊藤 孝; 岩崎 雅彦*; et al.
Hyperfine Interactions, 237(1), p.124_1 - 124_9, 2016/12
被引用回数：7 パーセンタイル：90.97(Physics, Atomic, Molecular & Chemical)At the Muon Science Facility (MUSE) of J-PARC (Japan Proton Accelerator Research Complex), the MuSEUM collaboration is planning new measurements of the ground state hyperfine structure (HFS) of muonium both at zero field and at high magnetic field. The previous measurements were performed both at LAMPF (Los Alamos Meson Physics Facility) with experimental uncertainties mostly dominated by statistical errors. The new high intensity muon beam that will soon be available at MUSE H-Line will provide an opportunity to improve the precision of these measurements by one order of magnitude. An overview of the different aspects of these new muonium HFS measurements, the current status of the preparation, and the results of a first commissioning test experiment at zero field are presented.
足立 泰平*; 池戸 豊*; 西山 樟生*; 薮内 敦*; 長友 傑*; Strasser, P.*; 伊藤 孝; 髭本 亘; 小嶋 健児*; 牧村 俊助*; et al.
JPS Conference Proceedings (Internet), 8, p.036017_1 - 036017_4, 2015/09
We report on the tuning of the ultra-slow muon beam line at J-PARC MUSE using Li impurities in a tungsten muonium production target in place of positive muons. Li ions were evaporated from the tungsten target by heating it up to 2000K and were transported in the ultra-slow muon beam line. The Li ion beam was monitored by micro channel plates installed at several points in the beam line. The Li beam was successfully transported to the end of the beam line after optimization of beam line parameters.
平石 雅俊*; 飯村 壮史*; 小嶋 健児*; 山浦 淳一*; 平賀 晴弘*; 池田 一貴*; Miao, P.*; 石川 喜久*; 鳥居 周輝*; 宮崎 正範*; et al.
Nature Physics, 10(4), p.300 - 303, 2014/04
被引用回数：103 パーセンタイル：95.46(Physics, Multidisciplinary)High-temperature (high-
) superconductivity appears as a consequence of the carrier-doping of an undoped parent compound exhibiting antiferromagnetic order; thereby, ground-state properties of the parent compound are closely relevant to the superconducting state. On the basis of the concept, a spin-fluctuation has been addressed as an origin of pairing of the superconducting electrons in cuprates. Whereas, there is growing interest in the pairing mechanism such as an unconventional spin-fluctuation or an advanced orbital-fluctuation due to the characteristic multi-orbital system in iron-pnictides. Here, we report the discovery of an antiferromagnetic order as well as a unique structural transition in electron-overdoped LaFeAsO
H
(
), whereby another parent phase was uncovered, albeit heavily doped. The unprecedented two-dome superconducting phases observed in this material can be interpreted as a consequence of the carrier-doping starting from the original at 
and advanced at parent phases toward the intermediate region. The bipartite parent phases with distinct physical properties in the second magnetic phase provide us with an interesting example to illustrate the intimate interplay among the magnetic interaction, structural change and orbital degree of freedom in iron-pnictides.
Ru)
Sb
and Pr
La
OsSbShu, L.*; 髭本 亘; 青木 勇二*; Hillier, A. D.*; 大石 一城*; 石田 憲二*; 門野 良典*; 幸田 章宏*; Bernal, O. O.*; MacLaughlin, D. E.*; et al.
Physical Review B, 83(10), p.100504_1 - 100504_4, 2011/03
被引用回数：34 パーセンタイル：77.76(Materials Science, Multidisciplinary)時間反転対称性(TRS)の破れた超伝導状態について調べるため、Pr(OsRu)SbとPrLaOsSb合金において零磁場ミュオンスピン緩和測定を行った。TRSは自発的な局所磁場の発生で知ることができる。両合金において磁場は最初は減少したが、Ru置換系ではLa置換系に比べて50%速い現象がみられた。この結果から、TRSは
で抑制されるが、La置換系ではすべての濃度において残ることが明らかになった。この結果は結晶場励起子によるクーパー対形成によるTRSの破れた超伝導機構を支持するものである。
三宅 康博*; 下村 浩一郎*; 河村 成肇*; Strasser, P.*; 牧村 俊助*; 幸田 章宏*; 藤森 寛*; 中原 一隆*; 竹下 聡史*; 小林 庸男*; et al.
Journal of Physics; Conference Series, 225, p.012036_1 - 012036_7, 2010/06
被引用回数：9 パーセンタイル：92.71(Physics, Applied)The science facility (MUSE) along with the neutron, hadron and neutrino facilities is one of the experimental areas PF the J-PARC project, which was approved for construction in a period from 2001 to 2008. Construction of the MLF building was started in the beginning of 2004, and was completed at the end of the 2006 fiscal year. On September 19th, 2008, the graphite target for muon production was placed into the 3 GeV proton beam line. On September 26th, 2008, we finally succeeded to extract surface muon beams. We also succeeded in the extraction of the decay muons on December 25th, 2008.
Strasser, P.*; 下村 浩一郎*; 幸田 章宏*; 河村 成肇*; 藤森 寛*; 牧村 俊助*; 小林 庸男*; 中原 一隆*; 加藤 峯夫*; 竹下 聡史*; et al.
Journal of Physics; Conference Series, 225, p.012050_1 - 012050_8, 2010/06
被引用回数：12 パーセンタイル：95.21(Physics, Applied)The new Muon Science Facility (MUSE) that is now under construction at J-PARC in the Materials and Life Sciences Facility (MLF) building will comprise four types of muon channels. In the first stage, a conventional superconducting decay muon channel (D-Line) was constructed, which can extract surface (positive) muons with an expected muon yield of 
/s and decay positive/negative muon up to 120 MeV/c, with an expected muon yield of a few 
/s at 60 MeV/c for both positive and negative muons. This channel will be used for various kinds of muon experiments like SR, muon catalyzed fusion and nondestruction elements analysis.
Pb
Sr
CuO
平賀 晴弘*; 林 陽一郎*; 脇本 秀一; 武田 全康; 加倉井 和久; 足立 匡*; 小池 洋二*; 山田 幾也*; 宮崎 正範*; 平石 雅俊*; et al.
Physical Review B, 81(14), p.144501_1 - 144501_6, 2010/04
被引用回数：15 パーセンタイル：55.02(Materials Science, Multidisciplinary)Spin correlations in the overdoped region of BiPbSrCuO have been explored with Fe-doped single crystals characterized by neutron scattering, muon-spin-rotation spectroscopy, and magnetic-susceptibility measurements. The incommensurability 
is unexpectedly large (
0.2 r.l.u.), as compared with the overdoped La
Sr
CuO
. However, this large is close to the hole concentration 
. While our findings in Fe-doped BiPbSrCuO support the commonality of incommensurate spin correlations in high-
cuprate superconductors, they also suggest that the magnetic response might be dominated by a distinct mechanism in the overdoped region.
三宅 康博*; 下村 浩一郎*; 河村 成肇*; Strasser, P.*; 牧村 俊助*; 幸田 章宏*; 藤森 寛*; 中原 一隆*; 門野 良典*; 加藤 峯夫*; et al.
Physica B; Condensed Matter, 404(5-7), p.957 - 961, 2009/04
被引用回数：12 パーセンタイル：47.84(Physics, Condensed Matter)ミュオン科学実験施設(MUSE)はJ-PARCの実験施設の一つである、MUSEは中性子とミュオン利用の実験施設である物質生命科学実験施設(MLF)の中にある。MLFの建屋建設は2004年にはじまり、2006年度末に完了した。われわれはそこにビームライン機器の設置を行っており、最初のミュオンビームが2008年の秋に発生する予定である。
佐藤 英行*; 青木 勇二*; 菊地 大輔*; 菅原 仁*; 髭本 亘; 大石 一城; 伊藤 孝; Heffner, R. H.; Saha, S. R.*; 幸田 章宏*; et al.
Physica B; Condensed Matter, 404(5-7), p.749 - 753, 2009/04
被引用回数：5 パーセンタイル：25.59(Physics, Condensed Matter)充填スクッテルダイト構造を持つ物質における強い電子相関に基づく現象は多岐に渡る。特に、複数の4f電子が含まれる場合は軌道の自由度が新たな非磁性又は弱磁性を伴う現象に大きな役割を果たす。Pr系及びSm系充填スクッテルダイト構造物質においてさまざまな例が見いだされており、これらとミュオンスピン緩和実験の関連を紹介する。
藤井 保彦; 新井 正敏; 門野 良典*; 金谷 利治*; 神山 崇*; 新村 信雄*; 野尻 浩之*; 野田 幸男*; 八木 健彦*; 山田 和芳*
固体物理, 43(7), p.441 - 450, 2008/07
平成20年12月から利用を開始するJ-PARC/MLF(中性子,ミュオン)において、凝縮系科学分野で計画している新しい科学を切り拓く研究を各分野の専門家がそれぞれの夢も交えて紹介している。
