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JAEA Reports

Decommissioning report for Wastewater Treatment Facility (Part 2); Chapter on contamination inspection section

Yamamoto, Keisuke; Nakagawa, Takuya; Shimojo, Hiroto; Kijima, Jun; Miura, Daiya; Onose, Yoshihiko*; Namba, Koji*; Uchida, Hiroaki*; Sakamoto, Kazuhiko*; Ono, Chika*; et al.

JAEA-Technology 2024-019, 211 Pages, 2025/02

JAEA-Technology-2024-019.pdf:35.35MB

The uranium enrichment facilities at the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency (JAEA) were constructed sequentially to develop uranium enrichment technology with centrifugal separation method. The developed technologies were transferred to Japan Nuclear Fuel Limited until 2001. And the original purpose has been achieved. Wastewater Treatment Facility, one of the uranium enrichment facilities, was constructed in 1976 to treat radioactive liquid waste generated at the facilities, and it finished the role in 2008. In accordance with the Medium/Long-Term Management Plan of JAEA Facilities, interior equipment installed in this facility had been dismantled and removed since November 2021 to August 2023. This report summarizes the findings obtained through the work related to the contamination inspection methods cancellation the controlled area of Wastewater Treatment Facility from September 2023 to March 2024.

Journal Articles

Development of a dissolution method for analyzing the elemental composition of fuel debris using sodium peroxide fusion technique

Nakamura, Satoshi; Ishii, Sho*; Kato, Hitoshi*; Ban, Yasutoshi; Hiruta, Kenta; Yoshida, Takuya; Uehara, Hiroyuki; Obata, Hiroki; Kimura, Yasuhiko; Takano, Masahide

Journal of Nuclear Science and Technology, 62(1), p.56 - 64, 2025/01

 Times Cited Count:1 Percentile:27.40(Nuclear Science & Technology)

A dissolution method for analyzing the elemental composition of fuel debris using the sodium peroxide (Na$$_{2}$$O$$_{2}$$) fusion technique has been developed. Herein, two different types of simulated debris materials (such as solid solution of (Zr,RE)O$$_{2}$$ and molten core-concrete interaction products (MCCI)) were taken. At various temperatures, these debris materials were subsequently fused with Na$$_{2}$$O$$_{2}$$ in crucibles, which are made of different materials, such as Ni, Al$$_{2}$$O$$_{3}$$, Fe, and Zr. Then, the fused samples are dissolved in nitric acid. Furthermore, the effects of the experimental conditions on the elemental composition analysis were evaluated using inductively coupled plasma-atomic emission spectroscopy (ICP-AES), which suggested the use of a Ni crucible at 923 K as an optimum testing condition. The optimum testing condition was then applied to the demonstration tests with Three Mile Island unit-2 (TMI-2) debris in a shielded concrete cell, thereby achieving complete dissolution of the debris. The elemental composition of TMI-2 debris revealed by the proposed dissolution method has good reproducibility and has an insignificant contradiction in the mass balance of the sample. Therefore, this newly developed reproducible dissolution method can be effectively utilized in practical applications by dissolving fuel debris and estimating its elemental composition.

Journal Articles

Temperature stability of PIN-PMN-PT ternary ceramics during pyroelectric power generation

Moro, Takuya*; Kim, J.*; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Nakayama, Tadachika*; Takeda, Masatoshi*; Yamada, Noboru*; Nishihata, Yasuo; Fukuda, Tatsuo; et al.

Journal of Alloys and Compounds, 768, p.22 - 27, 2018/11

 Times Cited Count:20 Percentile:61.68(Chemistry, Physical)

Journal Articles

Neutron irradiation effect of high-density MoO$$_{3}$$ pellets for Mo-99 production, 3

Ishida, Takuya; Suzuki, Yoshitaka; Nishikata, Kaori; Yonekawa, Minoru; Kato, Yoshiaki; Shibata, Akira; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; et al.

KURRI Progress Report 2015, P. 64, 2016/08

no abstracts in English

JAEA Reports

Performance tests of radiation detectors for inspection of $$^{99}$$Mo/$$^{99m}$$Tc solution, 1

Suzuki, Yumi*; Nakano, Hiroko; Suzuki, Yoshitaka; Ishida, Takuya; Shibata, Akira; Kato, Yoshiaki; Kawamata, Kazuo; Tsuchiya, Kunihiko

JAEA-Technology 2015-031, 58 Pages, 2015/11

JAEA-Technology-2015-031.pdf:14.57MB

Technetium-99m ($$^{99m}$$Tc) is one of the most commonly used radioisotopes in the field of nuclear medicine. In the Japan Atomic Energy Agency (JAEA), the research and development (R&D) have been carried out for production of molybdenum-99 ($$^{99}$$Mo) by (n, $$gamma$$) method, a parent nuclide of $$^{99m}$$Tc, with the Japan Material Testing Reactor (JMTR). On the other hand, the new project as "Domestic Production of Medical Radioisotope (Technetium preparation) in Japan" was adopted in the Tsukuba International Strategic Zone on October, 2013 and the demonstration tests will be planned for the domestic production of $$^{99}$$Mo/$$^{99m}$$Tc with the JMTR. Thus, new facilities and analysis devices were equipped in the JMTR Hot Laboratory in 2014 as the part of this project. As the part of the analytical device equipment, the $$gamma$$-TLC analyzer and the radiation detector connected with the High Performance Liquid Chromatography (HPLC) were installed for quality inspection of the $$^{99}$$Mo/$$^{99m}$$Tc solution and the extracted $$^{99m}$$Tc solution in the JMTR Hot Laboratory. The performance tests of these devices such as detection sensitivity, resolution, linearity and selectivity of energy range were carried out with $$^{137}$$Cs and $$^{152}$$Eu as alternative radionuclides of $$^{99}$$Mo and $$^{99m}$$Tc, respectively. In the results, bright prospects were obtained concerning the quality inspection of the $$^{99}$$Mo/$$^{99m}$$Tc and $$^{99m}$$Tc solutions using these devices. This report describes the results of those performance tests.

Journal Articles

Neutron irradiation effect of high-density MoO$$_{3}$$ pellets for Mo-99 production, 2

Nishikata, Kaori; Ishida, Takuya; Yonekawa, Minoru; Kato, Yoshiaki; Kurosawa, Makoto; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.

KURRI Progress Report 2014, P. 109, 2015/07

As one of effective applications of the Japan Materials Testing Reactor (JMTR), JAEA has a plan to produce $$^{99}$$Mo by (n,$$gamma$$) method ((n,$$gamma$$)$$^{99}$$Mo production), a parent nuclide of $$^{99m}$$Tc. In this study, preliminary irradiation test was carried out with the high-density molybdenum trioxide (MoO$$_{3}$$) pellets in the hydraulic conveyer (HYD) of the Kyoto University Research Reactor (KUR) and the $$^{99m}$$Tc solution extracted from $$^{99}$$Mo was evaluated. After the irradiation test of the high-density MoO$$_{3}$$ pellets in the KUR, $$^{99m}$$Tc was extracted from the Mo solution and the recovery rate of $$^{99m}$$Tc achieved the target values. The $$^{99m}$$Tc solution also got the value that satisfied the standard value for $$^{99m}$$Tc radiopharmaceutical products by the solvent extraction method.

Journal Articles

Neutron irradiation effect of high-density MoO$$_{3}$$ pellets for Mo-99 production

Nishikata, Kaori; Ishida, Takuya; Yonekawa, Minoru; Kato, Yoshiaki; Kurosawa, Makoto; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.

KURRI Progress Report 2013, P. 242, 2014/10

As one of effective applications of the Japan Materials Testing Reactor (JMTR), JAEA has a plan to produce Mo-99 ($$^{99}$$Mo) by (n,$$gamma$$) method ((n,$$gamma$$)$$^{99}$$Mo production), a parent nuclide of $$^{99m}$$Tc. In this study, preliminary irradiation tests were carried out with the high-density MoO$$_{3}$$ pellets in the KUR and the $$^{99}$$Mo production amount was evaluated between the calculation results and measurement results.

Journal Articles

Expansion control for cementation of incinerated ash

Nakayama, Takuya; Suzuki, Shinji; Hanada, Keiji; Tomioka, Osamu; Sato, Junya; Irisawa, Keita; Kato, Jun; Kawato, Yoshimi; Meguro, Yoshihiro

Proceedings of 2nd International Symposium on Cement-based Materials for Nuclear Wastes (NUWCEM 2014) (CD-ROM), 12 Pages, 2014/06

Journal Articles

Development of post-irradiation test facility for domestic production of $$^{99}$$Mo

Taguchi, Taketoshi; Yonekawa, Minoru; Kato, Yoshiaki; Kurosawa, Makoto; Nishikata, Kaori; Ishida, Takuya; Kawamata, Kazuo

UTNL-R-0483, p.10_5_1 - 10_5_13, 2013/03

JMTR focus on the activation method. By carrying out the preliminary tests using irradiation facilities existing, and verification tests using the irradiation facility that has developed in the cutting-edge research and development strategic strengthening business, as irradiation tests towards the production of $$^{99}$$Mo, we have been conducting research and development that can contribute to supply about 25% for $$^{99}$$Mo demand in Japan and the stable supply of radiopharmaceutical. This report describes a summary of the status of the preliminary tests for the production of $$^{99}$$Mo: Maintenance of test equipment in the facility in JMTR Hot Laboratory in preparation for research and development for the production of $$^{99}$$Mo in JMTR and using MoO$$_{3}$$ pellet irradiated at Kyoto University Research Reactor Institute (KUR).

Journal Articles

X-ray spectroscopy diagnoses of clusters surviving under prepulses of ultra-intense femtosecond laser pulse irradiation

Faenov, A. Ya.*; Skobelev, I. Yu.*; Pikuz, T. A.; Pikuz, S. A.*; Fortov, V. E.*; Fukuda, Yuji; Hayashi, Yukio; Pirozhkov, A. S.; Kotaki, Hideyuki; Shimomura, Takuya; et al.

Laser and Particle Beams, 30(3), p.481 - 488, 2012/09

 Times Cited Count:11 Percentile:41.10(Physics, Applied)

Journal Articles

The Spectra of the multicharged argon hollow ions; Observation, modeling and using for diagnostics of the early stage of the heating of clusters by a supper high contrast femtosecond laser pulses

Pikuz, T. A.; Faenov, A.*; Skobelev, I.*; Fortov, V. E.*; Boldarev, A.*; Gasilov, V.*; Chen, L. M.*; Zhang, L.*; Yan, W.*; Yuan, D.*; et al.

AIP Conference Proceedings 1465, p.181 - 201, 2012/07

 Times Cited Count:0 Percentile:0.00(Physics, Applied)

Journal Articles

Effects of the self-absorption of X-ray spectral lines in the presence of the laser-cluster interaction

Skobelev, I. Yu.*; Faenov, A. Ya.*; Pikuz, T. A.; Pikuz, S. A. Jr.*; Fortov, V. E.*; Fukuda, Yuji; Hayashi, Yukio; Pirozhkov, A. S.; Kawase, Keigo*; Kotaki, Hideyuki; et al.

JETP Letters, 94(4), p.270 - 276, 2011/10

 Times Cited Count:2 Percentile:19.18(Physics, Multidisciplinary)

Journal Articles

Observation and modeling of high resolution spectral features of the inner-shell X-ray emission produced by 10$$^{-10}$$ contrast femtosecond-pulse laser irradiation of argon clusters

Colgan, J.*; Abdallah, J. Jr.*; Faenov, A. Ya.*; Pikuz, T. A.*; Skobelev, I. Yu.*; Fukuda, Yuji; Hayashi, Yukio; Pirozhkov, A. S.; Kawase, Keigo*; Shimomura, Takuya; et al.

High Energy Density Physics, 7(2), p.77 - 83, 2011/06

 Times Cited Count:21 Percentile:62.64(Physics, Fluids & Plasmas)

A study is made of the ultra-short laser pulse irradiation of Ar cluster targets. Experiments have been performed with large cluster sizes and using very high laser contrasts, which have allowed clear and unambiguous observation of exotic inner-shell transitions in near-neutral Ar ions. The interaction of the main laser pulse with the unperturbed target is a necessary requirement for observing these lines. Our measurements are supported by kinetics calculations in which a very detailed atomic model is used. The calculations predict all of the spectral features found experimentally, and support the notion that the X-ray emission arises from many ion stages of the Ar plasma, from near-neutral through He-like ions, and from a range of plasma temperatures and densities.

Journal Articles

Incommensurate structures of intermediate phase and martensite phase in Ni$$_{2}$$MnGa

Kushida, Hiroaki*; Fukuda, Kodai*; Terai, Tomoyuki*; Fukuda, Takashi*; Kakeshita, Tomoyuki*; Oba, Takuya*; Osakabe, Toyotaka; Kakurai, Kazuhisa; Kato, Kenichi*

Journal of Physics; Conference Series, 165, p.012054_1 - 012054_4, 2009/06

Journal Articles

Extrinsic sensors and external signal generator for advanced transparency framework

Katsumura, Soichiro; Kitabata, Takuya; Irie, Tsutomu; Suzuki, Mitsutoshi; Hashimoto, Yu; Kato, Keiji*

Transactions of the American Nuclear Society, 99(1), P. 780, 2008/11

Journal Articles

Crystal structure of martensite and intermediate phases in Ni$$_{2}$$MnGa studied by neutron diffraction

Kushida, Hiroaki*; Fukuda, Kodai*; Terai, Tomoyuki*; Fukuda, Takashi*; Kakeshita, Tomoyuki*; Oba, Takuya*; Osakabe, Toyotaka; Kakurai, Kazuhisa; Kato, Kenichi*

European Physical Journal; Special Topics, 158(1), p.87 - 92, 2008/05

 Times Cited Count:22 Percentile:70.89(Physics, Multidisciplinary)

Journal Articles

A Cu NQR study in a $$d$$-electron heavy-fermion system, CaCu$$_{3}$$Ru$$_{4}$$O$$_{12}$$

Kato, Harukazu*; Tsuruta, Takuya*; Nishioka, Takashi*; Matsumura, Masahiro*; Sakai, Hironori; Kambe, Shinsaku

Journal of Physics and Chemistry of Solids, 68(11), p.2187 - 2190, 2007/11

 Times Cited Count:8 Percentile:37.21(Chemistry, Multidisciplinary)

Cu nuclear quadrupole resonance (NQR) studies have been carried out for CaCu$$_{3}$$Ru$$_{4}$$O$$_{12}$$,which has been suggested to show a heavy-fermion-like behavioral though it possess no f electron. A Lorentzian shape of the Cu NQR line with a narrow width implies that no magnetic ordering appears, at least, down to 5 K. The spin-lattice relaxation rate of the Cu nuclei probes a change of the Cu 3$$d$$ electron nature, resulting in the Fermi liquid state at a low temperature. These facts strongly support that the heavy fermion picture is available in the concerned compound.

Journal Articles

Cu NMR study in a heavy-electron system, CaCu$$_3$$Ru$$_4$$O$$_{12}$$

Kato, Harukazu*; Tsuruta, Takuya*; Nishioka, Takashi*; Matsumura, Masahiro*; Sakai, Hironori; Kambe, Shinsaku

Journal of Magnetism and Magnetic Materials, 310(2, Part1), p.251 - 253, 2007/03

Cu NMR measurements have been carried out for CaCu$$_3$$Ru$$_4$$O$$_{12}$$, which shows a heavy-fermion-like behavior although it posseses no f electron moment. The field-sweep spectrum observed can be understood as a powder pattern of a Cu nucleus affected by the quadrupole interaction with no axial symmetry. The quadrupole parameters and the Knight shift of Cu are evaluated.

JAEA Reports

Development of module for TRU high temperature chemistry (Joint research)

Minato, Kazuo; Akabori, Mitsuo; Tsuboi, Takashi; Kurobane, Shiro; Hayashi, Hirokazu; Takano, Masahide; Otobe, Haruyoshi; Misumi, Masahiro*; Sakamoto, Takuya*; Kato, Isao*; et al.

JAERI-Tech 2005-059, 61 Pages, 2005/09

JAERI-Tech-2005-059.pdf:20.67MB

An experimental facility called the Module for TRU High Temperature Chemistry (TRU-HITEC) was installed in the Back-end Cycle Key Elements Research Facility (BECKY) of the Nuclear Fuel Cycle Safety Engineering Research Facility (NUCEF) for the basic studies of the behavior of the transuranium elements (TRU) in pyrochemical reprocessing and oxide fuels. TRU-HITEC consists of three alpha/gamma cells shielded by steel and polyethylene and a glove box shielded by leaded acrylic resin, where experimental apparatuses have been equipped and a high purity argon gas atmosphere is maintained. In the facility 10 g of $$^{241}$$Am as well as the other TRU of Np, Pu and Cm can be handled. This report summarizes the outline, structure, performance and interior apparatuses of the facility, and is the result of the joint research between the Japan Atomic Energy Research Institute and three electric power companies of Tokyo Electric Power Co., Tohoku Electric Power Co. and the Japan Atomic Power Co.

Oral presentation

High-resolution X-ray spectroscopy diagnostics of early heating stage of clusters by high contrast femtosecond laser pulse

Faenov, A.*; Pikuz, T. A.; Skobelev, I.*; Fortov, V.*; Colgan, J.*; Abdallah, J. Jr.*; Fukuda, Yuji; Hayashi, Yukio; Pirozhkov, A. S.; Kawase, Keigo*; et al.

no journal, , 

47 (Records 1-20 displayed on this page)