Pressure-modulated magnetism and negative thermal expansion in the HoFe intermetallic compound

Cao, Y.*; Zhou, H.*; Khmelevskyi, S.*; Lin, K.*; Avdeev, M.*; Wang, C.-W.*; Wang, B.*; Hu, F.*; Kato, Kenichi*; Hattori, Takanori; et al.

Chemistry of Materials, 35(8), p.3249 - 3255, 2023/04

https://doi.org/10.1021/acs.chemmater.3c00158

Hydrostatic and chemical pressure are efficient stimuli to alter the crystal structure and are commonly used for tuning electronic and magnetic properties in materials science. However, chemical pressure is difficult to quantify and a clear correspondence between these two types of pressure is still lacking. Here, we study intermetallic candidates for a permanent magnet with a negative thermal expansion (NTE). Based on in situ synchrotron X-ray diffraction, negative chemical pressure is revealed in HoFe on Al doping and quantitatively evaluated by using temperature and pressure dependence of unit cell volume. A combination of magnetization and neutron diffraction measurements also allowed one to compare the effect of chemical pressure on magnetic ordering with that of hydrostatic pressure. Intriguingly, pressure can be used to control suppression and enhancement of NTE. Electronic structure calculations indicate that pressure affected the top of the majority band with respect to the Fermi level, which has implications for the magnetic stability, which in turn plays a critical role in modulating magnetism and NTE. This work presents a good example of understanding the effect of pressure and utilizing it to control properties of functional materials.

Spallation and fragmentation cross sections for 168 MeV/nucleon Xe ions on proton, deuteron, and carbon targets

Sun, X. H.*; Wang, H.*; Otsu, Hideaki*; Sakurai, Hiroyoshi*; Ahn, D. S.*; Aikawa, Masayuki*; Fukuda, Naoki*; Isobe, Tadaaki*; Kawakami, Shunsuke*; Koyama, Shumpei*; et al.

Physical Review C, 101(6), p.064623_1 - 064623_12, 2020/06

https://doi.org/10.1103/PhysRevC.101.064623

The spallation and fragmentation reactions of Xe induced by proton, deuteron and carbon at 168 MeV/nucleon were studied at RIKEN Radioactive Isotope Beam Factory via the inverse kinematics technique. The cross sections of the lighter products are larger in the carbon-induced reactions due to the higher total kinetic energy of carbon. The energy dependence was investigated by comparing the newly obtained data with previous results obtained at higher reaction energies. The experimental data were compared with the results of SPACS, EPAX, PHITS and DEURACS calculations. These data serve as benchmarks for the model calculations.

Neutron computed tomography of phase separation structures in solidified Cu-Co alloys and investigation of relationship between the structures and melt convection during solidification

Shoji, Eita*; Isogai, Shosei*; Suzuki, Rikuto*; Kubo, Masaki*; Tsukada, Takao*; Kai, Tetsuya; Shinohara, Takenao; Matsumoto, Yoshihiro*; Fukuyama, Hiroyuki*

Scripta Materialia, 175, p.29 - 32, 2020/01

https://doi.org/10.1016/j.scriptamat.2019.08.041

Assembly study for JT-60SA tokamak

Shibanuma, Kiyoshi; Arai, Takashi; Hasegawa, Koichi; Hoshi, Ryo; Kamiya, Koji; Kawashima, Hisato; Kubo, Hirotaka; Masaki, Kei; Saeki, Hisashi; Sakurai, Shinji; et al.

Fusion Engineering and Design, 88(6-8), p.705 - 710, 2013/10

https://doi.org/10.1016/j.fusengdes.2012.12.011

Microprocessing of arched bridge structures with epoxy resin by proton beam writing

Takano, Katsuyoshi*; Asano, Atsushi*; Maeyoshi, Yuta*; Marui, Hiromi*; Omichi, Masaaki*; Saeki, Akinori*; Seki, Shu*; Sato, Takahiro; Ishii, Yasuyuki; Kamiya, Tomihiro; et al.

Journal of Photopolymer Science and Technology, 25(1), p.43 - 46, 2012/07

https://doi.org/10.2494/photopolymer.25.43

Fabrication of poly(9,9'-dioctylfluorene)-based nano- and microstructures by proton beam writing

Maeyoshi, Yuta*; Takano, Katsuyoshi*; Asano, Atsushi*; Marui, Hiromi*; Omichi, Masaaki*; Sato, Takahiro; Kamiya, Tomihiro; Ishii, Yasuyuki; Okubo, Takeru; Koka, Masashi; et al.

Japanese Journal of Applied Physics, 51(4R), p.045201_1 - 045201_4, 2012/04

https://doi.org/10.1143/JJAP.51.045201

Characteristic heavy fermion properties in YbCuSi and YbTZn (T: Co, Rh, Ir)

Onuki, Yoshichika; Yasui, Shinichi*; Matsushita, Masaki*; Yoshiuchi, Shingo*; Oya, Masahiro*; Hirose, Yusuke*; Dung, N. D.*; Honda, Fuminori*; Takeuchi, Tetsuya*; Settai, Rikio*; et al.

Journal of the Physical Society of Japan, 80(Suppl.A), p.SA003_1 - SA003_6, 2011/12

https://doi.org/10.1143/JPSJS.80SA.SA003

Characterization of the microstructure of dual-phase 9Cr-ODS steels using a laser-assisted 3D atom probe

Nogiwa, Kimihiro; Nishimura, Akihiko; Yokoyama, Atsushi; Otsuka, Satoshi; Kaito, Takeji; Inoue, Masaki; Okubo, Tadakatsu*; Hono, Kazuhiro*

Journal of Nuclear Materials, 417(1-3), p.201 - 204, 2011/10

https://doi.org/10.1016/j.jnucmat.2010.12.053

Du se 9Cr-ODS (oxide dispersion-strengthened) steel consisting of residual- ferrite and prime martensite has excellent high-temperature strength. This study describes the microstructure of dual-phase 9Cr-ODS steels characterized by atom-probe tomography in order to compare oxide-particle dispersion states in each phase. This revealed that nano-size oxide particles were of the same chemical composition and that their mean size was about 3 nm in each phase. On the other hand, the number density in the residual- phase was about four times higher than that of the prime phase. These results indicate that the dense distribution of the oxide particles in the residual- phase contribute to the excellent high-temperature strength of 9Cr-ODS steel.

Evaluations of the new LiF-scintillator and optional brightness enhancement films for neutron imaging

Iikura, Hiroshi; Tsutsui, Noriaki*; Nakamura, Tatsuya; Katagiri, Masaki*; Kureta, Masatoshi; Kubo, Jun*; Matsubayashi, Masahito

Nuclear Instruments and Methods in Physics Research A, 651(1), p.100 - 104, 2011/09

https://doi.org/10.1016/j.nima.2011.01.010

Japan Atomic Energy Agency has developed the neutron scintillator jointly with Chichibu Fuji Co., Ltd. In this study, we evaluated the new ZnS(Ag):Al/LiF scintillator developed for neutron imaging. It was confirmed that the brightness increased by about double while maintaining equal performance for the spatial resolution as compared with a conventional scintillator. High frame-rate imaging using a high-speed video camera system and this new scintillator made it possible to image beyond 10000 frames per second while still having enough brightness. This technique allowed us to obtain a high-frame-rate visualization of oil flow in a running car engine. Furthermore, we devised a technique to increase the light intensity of reception for a camera by adding brightness enhancement films on the output surface of the scintillator. It was confirmed that the spatial resolution degraded more than double, but the brightness increased by about three times.

Achievement of 500 keV negative ion beam acceleration on JT-60U negative-ion-based neutral beam injector

Kojima, Atsushi; Hanada, Masaya; Tanaka, Yutaka*; Kawai, Mikito*; Akino, Noboru; Kazawa, Minoru; Komata, Masao; Mogaki, Kazuhiko; Usui, Katsutomi; Sasaki, Shunichi; et al.

Nuclear Fusion, 51(8), p.083049_1 - 083049_8, 2011/08

https://doi.org/10.1088/0029-5515/51/8/083049

Hydrogen negative ion beams of 490 keV, 3 A and 510 keV, 1 A have been successfully produced in the JT-60 negative ion source with three acceleration stages. These successful productions of the high-energy beams at high current have been achieved by overcoming the most critical issue, i.e., a poor voltage holding of the large negative ion sources with the grids of 2 m for JT-60SA and ITER. To improve voltage holding capability, the breakdown voltages for the large grids was examined for the first time. It was found that a vacuum insulation distance for the large grids was 6-7 times longer than that for the small-area grid (0.02 m). From this result, the gap lengths between the grids were tuned in the JT-60 negative ion source. The modification of the ion source also realized a significant stabilization of voltage holding and a short conditioning time. These results suggest a practical use of the large negative ion sources in JT-60SA and ITER.