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Journal Articles

France-Japan collaboration on thermodynamic and kinetic studies of core material mixture in severe accidents of sodium-cooled fast reactors

Quaini, A.*; Goss$'e$, S.*; Payot, F.*; Suteau, C.*; Delacroix, J.*; Saas, L.*; Gubernatis, P.*; Martin-Lopez, E.*; Yamano, Hidemasa; Takai, Toshihide; et al.

Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Sustainable Clean Energy for the Future (FR22) (Internet), 10 Pages, 2022/04

CEA and JAEA defined new sub-tasks under the current implementing arrangement: Kinetics of interaction in core material mixtures- Physical properties of core material mixtures, High temperature thermodynamic data for the UO$$_{2}$$-Fe-B$$_{4}$$C system, Experimental studies on B$$_{4}$$C-SS kinetics and B$$_{4}$$C-SS eutectic material relocation (freezing), B$$_{4}$$C/SS eutectic and kinetics models for SIMMER code systems, Methodology for the modelling of mixtures liquefaction kinetics. The paper describes major R&D results obtained in the France-Japan collaboration under the previous implementing arrangement as well as experimental and analytical roadmaps under the current arrangement.

Journal Articles

Experimental determination of the photooxidation of aqueous I$$^{-}$$ as a source of atmospheric I$$_{2}$$

Watanabe, Kosuke*; Matsuda, Shohei; Cuevas, C. A.*; Saiz-Lopez, A.*; Yabushita, Akihiro*; Nakano, Yukio*

ACS Earth and Space Chemistry (Internet), 3(4), p.669 - 679, 2019/04

https://doi.org/10.1021/acsearthspacechem.9b00007
 Times Cited Count：8 Percentile：42.10(Chemistry, Multidisciplinary)

The photooxidation of aqueous iodide ions (I$$^{-}$$$$_{(aq)}$$) at sea surface results in the emission of gaseous iodine molecules (I$$_{2}$$$$_{(g)}$$) into the atmosphere. It plays a certain role in the transport of iodine from ocean to the atmosphere in the natural cycle of iodine. In this study, we determined the photooxidation parameters, the molar absorption coefficient ($$varepsilon$$$$_{iodide}$$($$lambda$$)) and the photooxidative quantum yields ($$Phi$$$$_{iodide}$$($$lambda$$)) of I$$^{-}$$$$_{(aq)}$$, in the range of 290-500 nm. Through the investigation of the influence of pH and dissolved oxygen (DO) on $$Phi$$$$_{iodide}$$($$lambda$$), the subsequent emission rates of I$$_{2}$$$$_{(g)}$$ following the photooxidation of I$$^{-}$$$$_{(aq)}$$ in deionized water solution (pH 5.6, DO 7.8 mg L$$^{-1}$$) and artificial seawater solution (pH 8.0, DO 7.0 mg L$$^{-1}$$) were estimated. A global chemistry-climate model employed herein to assess the I$$_{2}$$$$_{(g)}$$ ocean emission on a global scale indicated that the photooxidation of I$$^{-}$$$$_{(aq)}$$ by solar light can enhance the atmospheric iodine budget by up to $$sim$$8% over some oceanic regions.

Journal Articles

Monte Carlo modelling for the ${it in vivo}$ lung monitoring of enriched uranium; Results of an international comparison

Broggio, D.*; Bento, J.*; Caldeira, M.*; Cardenas-Mendez, E.*; Farah, J.*; Fonseca, T.*; Konvalinka, C.*; Liu, L.*; Perez, B.*; Capello, K.*; et al.

Radiation Measurements, 47(7), p.492 - 500, 2012/07

https://doi.org/10.1016/j.radmeas.2012.04.020
 Times Cited Count：23 Percentile：83.76(Nuclear Science & Technology)

Oral presentation

Numerical simulation of coupled THM behavior of full-scale EBS in backfilled experimental gallery, Horonobe, Japan

Sugita, Yutaka; Ono, Hirokazu; Beese, S.*; Pan, P.*; Kim, M.*; Lee, C.*; Jove-Colon, C.*; M Lopez, C.*; Liang, S.-Y.*

no journal, , 

This paper presents the results of analytical simulations of in-situ test of engineered barriers system conducted at the Horonobe Underground Research Laboratory. This results is one of the tasks of the current phase "DECOVALEX-2023" of the international joint project DECOVALEX in which JAEA participates. Research teams from 6 countries or region, including JAEA, are participating in this task, Different analytical approaches and their effects on the analytical results are introduced, as well as the factors that affect the evaluation of coupled phenomena in engineered barrier system obtained through the task.

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