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Iwase, Akihiro*; Fukuda, Kengo*; Saito, Yuichi*; Okamoto, Yoshihiro; Semboshi, Satoshi*; Amekura, Hiroshi*; Matsui, Toshiyuki*
Journal of Applied Physics, 132(16), p.163902_1 - 163902_10, 2022/10
Times Cited Count：0 Percentile：0.00(Physics, Applied)Amorphous SiO
samples were implanted with 380 keV Fe ions at room temperature. After implantation, some of the samples were irradiated with 16 MeV Au ions. magnetic properties were investigated using a SQUID magnetometer, and the morphology of the Fe-implanted SiO samples was examined using transmission electron microscopy and X-ray absorption spectroscopy (EXAFS and XANES), which showed that the size of Fe nanoparticles was increasing The size of Fe nanoparticles increased with increasing Fe implantation amount; some of the Fe nanoparticles consisted of Fe oxides, and the valence and structure of Fe atoms became closer to that of metallic 
-Fe with increasing Fe injection amount. The magnetization-field curve of the sample implanted with a small amount of Fe was reproduced by Langevin's equation, suggesting that the Fe nanoparticles behave in a superparamagnetic manner. In addition, when a large amount of Fe was implanted, the magnetization-magnetic field curve shows a ferromagnetic state. These magnetic property results are consistent with the X-ray absorption results. Subsequent 16 MeV Au irradiation crushed the Fe nanoparticles, resulting in a decrease in magnetization.
pellets for Mo-99 production, 3Ishida, Takuya; Suzuki, Yoshitaka; Nishikata, Kaori; Yonekawa, Minoru; Kato, Yoshiaki; Shibata, Akira; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; et al.
KURRI Progress Report 2015, P. 64, 2016/08
no abstracts in English
pellets for Mo-99 production, 2Nishikata, Kaori; Ishida, Takuya; Yonekawa, Minoru; Kato, Yoshiaki; Kurosawa, Makoto; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.
KURRI Progress Report 2014, P. 109, 2015/07
As one of effective applications of the Japan Materials Testing Reactor (JMTR), JAEA has a plan to produce 
Mo by (n,
) method ((n,)Mo production), a parent nuclide of 
Tc. In this study, preliminary irradiation test was carried out with the high-density molybdenum trioxide (MoO) pellets in the hydraulic conveyer (HYD) of the Kyoto University Research Reactor (KUR) and the Tc solution extracted from Mo was evaluated. After the irradiation test of the high-density MoO pellets in the KUR, Tc was extracted from the Mo solution and the recovery rate of Tc achieved the target values. The Tc solution also got the value that satisfied the standard value for Tc radiopharmaceutical products by the solvent extraction method.
pellets for Mo-99 productionNishikata, Kaori; Ishida, Takuya; Yonekawa, Minoru; Kato, Yoshiaki; Kurosawa, Makoto; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.
KURRI Progress Report 2013, P. 242, 2014/10
As one of effective applications of the Japan Materials Testing Reactor (JMTR), JAEA has a plan to produce Mo-99 (Mo) by (n,) method ((n,)Mo production), a parent nuclide of Tc. In this study, preliminary irradiation tests were carried out with the high-density MoO pellets in the KUR and the Mo production amount was evaluated between the calculation results and measurement results.
Hemmi, Tsutomu; Matsui, Kunihiro; Kajitani, Hideki; Okuno, Kiyoshi; Koizumi, Norikiyo; Ishimi, Akihiro; Katsuyama, Kozo
IEEE Transactions on Applied Superconductivity, 24(3), p.4802704_1 - 4802704_4, 2014/06
Times Cited Count：1 Percentile：9.39(Engineering, Electrical & Electronic)Japan Atomic Energy Agency (JAEA), as Japan Domestic Agency, has responsibility to procure nine ITER Toroidal Field (TF) coils. The TF coil winding consists of a NbSn Cable-In-Conduit conductor, a pair of joints and a He-inlet. The current capacity of 68 kA is required at the magnetic field of 7 T around the He-inlet region in the TF coil winding. During reaction heat-treatment, the compressive residual strain in NbSn cable is induced by the difference in the thermal expansion coefficients between the NbSn cable and stainless steel jacket. The strands bending in the NbSn cable of the He-inlet is anticipated since there is the compressive residual strain and a gap between the NbSn cable and the He-inlet to introduce SHE flow. If the strand is bent, the variation of mechanical behaviors, such as the elongation of He-inlet during the reaction heat-treatment and the thermally induced residual strain on the jacket around the He-inlet, are expected. To investigate the strands bending in the NbSn cable of the He-inlet, the following items are performed; (1) elongation measurement during reaction heat-treatment, (2) residual longitudinal strain measurement using strain gauges by sample cuttings, (3) nondestructive inspection on the cable and strands using high resolution X-ray CT, Detail of test results and investigation of the strands bending in the NbSn cable of the He-inlet are reported and discussed.
Koide, Tetsuya*; Sato, Takahiro; Koka, Masashi; Saito, Yuichi; Kamiya, Tomihiro; Okochi, Takuo*; Kotsugi, Masato*; Kinoshita, Toyohiko*; Nakamura, Tetsuya*; Iwase, Akihiro*; et al.
Japanese Journal of Applied Physics, 53(5S1), p.05FC06_1 - 05FC06_4, 2014/05
Times Cited Count：12 Percentile：46.80(Physics, Applied)We previously reported that the magnetic state of FeRh can be controlled by irradiation with ion beams. In this paper, we evaluate possibility of magnetic patterning on FeRh thin films using energetic light ion microbeam irradiation with various shapes and dimensions. Proton microbeam irradiation with 2 MeV was performed at JAEA-Takasaki to produce micron-sized magnetic patterns. XMCD-PEEM observation was performed at SPring8 to confirm the synthesized magnetic patterns. As a result, the XMCD-PEEM images of the various micrometer sized patters in FeRh film were observed using 2 MeV H ion beam. The observed bright regions are considered to have ferromagnetic spin orders, in contrast that the gray areas have anti-ferromagnetic spin order. Since the brightness of the PEEM images is strongly correlated with the magnetization of the samples, we reveal that the magnetic state in local regions of the FeRh thin films can be controlled by changing the ion fluences.
Aiko, Kazuma*; Toki, Atsushi*; Okuda, Shuichi*; Saito, Yuichi; Kamiya, Tomihiro; Nakamura, Tetsuya*; Kinoshita, Toyohiko*; Iwase, Akihiro*; Matsui, Toshiyuki*
Nuclear Instruments and Methods in Physics Research B, 314, p.99 - 102, 2013/11
Times Cited Count：5 Percentile：38.30(Instruments & Instrumentation)Tc production from (n,)Mo based on solvent extractionKimura, Akihiro; Awaludin, R.*; Shiina, Takayuki*; Tanase, Masakazu*; Kawauchi, Yukimasa*; Gunawan, A. H.*; Lubis, H.*; Sriyono*; Ota, Akio*; Genka, Tsuguo; et al.
Proceedings of 3rd Asian Symposium on Material Testing Reactors (ASMTR 2013), p.109 - 115, 2013/11
JP, 2011-173260 
Patent publication (In Japanese)
Tc is generated by decay of Mo. Production of Mo is carried out by (n,f) method with high enriched uranium targets, and the production are currently producing to meet about 95% of global supply. Recently, it is difficult to carry out a stable supply for some problems such as aging of reactors etc. Furthermore, the production has difficulties in nuclear proliferation resistance etc. Thus, (n,) method has lately attracted considerable attention. The (n,) method has several advantages, but the extremely low specific activity makes its uses less convenient than (n,f) method. We proposed a method based on the solvent extraction, followed by adsorption of Tc with alumina column. In this paper, a practical production of Tc was tried by the method with 1Ci of Mo produced in MPR-30. The recovery yields were approximately 70%. Impurity of Mo was less than 4.0
10
% and the radiochemical purity was over 99.2%.
Sano, Kenji*; Yamada, Arisa*; Matsui, Akihiro*; Tsuji, Hideyuki*; Hasegawa, Shin; Sawada, Shinichi; Maekawa, Yasunari
Desalination, 324, p.34 - 36, 2013/09
Times Cited Count：3 Percentile：14.09(Engineering, Chemical)Anchored osmotic pressure inducer was examined. Salt-containing filter paper attached to an osmotic membrane increased the water flux to more than 10% at 1 MPa. The salt-containing filter paper was fabricated via graft polymerization of acrylic acid onto a filter paper followed by alkaline treatment. The filter paper was characterized by thermo gravimetric analysis (TGA), attenuated total reflection Fourier transform infrared spectroscopy (ATR-FTIR), scanning electronic microscopy-energy dispersive X-ray spectrometry(SEM-EDS).
Mn
)O
Shinoda, Ryoichi*; Ito, Masayoshi*; Sakurai, Yoshiharu*; Yamamoto, Hiroyuki; Hirao, Norie; Baba, Yuji; Iwase, Akihiro*; Matsui, Toshiyuki*
Journal of Applied Physics, 113(17), p.17E307_1 - 17E307_3, 2013/05
Times Cited Count：9 Percentile：37.75(Physics, Applied)We revealed that the Ba(CoMn)O (BCMO) ceramic samples exhibited ferromagnetic-dielectric behavior below the magnetic transition temperature of about 35 K. The origin of their magnetic ordering was expected to super-exchange coupling of Co
(
)-O
-Mn (
) with bonding angle of 180
. and/or Mn()-O-Mn () with bonding angle of 90. The magnetic spin momentum estimated by the magnetic Compton profiles (MCP) of the samples had similar temperature dependence as that determined by the SQUID measurement, which meant that the observed magnetic moments could be ascribed to the spin moment. The shapes of the MCPs of the samples were completely same regardless of the temperature measured. This result indicates that there are no changes of the momentum space distribution of spin density between ferromagnetic and paramagnetic states. So, this magnetic transition is simply caused by a thermal fluctuation of the spin.
Aiko, Kazuma*; Toki, Atsushi*; Matsui, Toshiyuki*; Iwase, Akihiro*; Sato, Takahiro; Takano, Katsuyoshi*; Koka, Masashi; Saito, Yuichi; Kamiya, Tomihiro
JAEA-Review 2012-046, JAEA Takasaki Annual Report 2011, P. 133, 2013/01
Shimizu, Hirotaka*; Kosugi, Shinya*; Tahara, Yuki*; Yasunaga, Kazufumi*; Kaneta, Yasunori*; Ishikawa, Norito; Hori, Fuminobu*; Matsui, Toshiyuki*; Iwase, Akihiro*
Nuclear Instruments and Methods in Physics Research B, 286, p.291 - 294, 2012/09
Times Cited Count：27 Percentile：87.31(Instruments & Instrumentation)We have studied the magnetic properties of pure CeO irradiated with swift heavy ions. Experiment a results showed that the ferromagnetism was induced even at room temperature by 200 MeV Xe ion irradiation. The value of saturation magnetization, Ms, systematically changes as a function of ion-fluence. The X-ray diffraction (XRD) spectra show that the lattice constant of CeO increases with increasing ion-fluence. This result and our previous XPS result show that the ion-irradiation produced oxygen vacancies. The present study implies that the ferromagnetic behavior of the ion-irradiated CeO is attributed to the magnetic moments of localized 4f electrons on Ce
atoms, which are related to oxygen vacancies.
Inoue, Shuichi; Omuro, Tadao; Nabeya, Hideaki; Matsui, Yoshinori; Iida, Kazuhiro; Ito, Kazuyuki; Kimura, Akihiro; Kanno, Masaru
JAEA-Technology 2010-010, 27 Pages, 2012/05
JAEA-Technology-2010-010.pdf:1.99MB
In fuel irradiation transient tests using a boiling water capsule, a dilution tube has been installed in the boiling water capsule in order to detect fission products (FP) from an irradiated fuel, in case of the fuel failure during the transient, by a radiation monitor located outside the reactor. When the fuel failure occurs, the released FP flows out from the capsule through the dilution tube. The dilution tube is designed to minimize the released FP that can be detected by the radiation monitor located outside the reactor. This report summarized the measurement results of the dilution tube installed in the boiling water capsule.
O
-doped CeO by means of synchrotron radiation X-ray spectroscopyTahara, Yuki*; Shimizu, Hirotaka*; Ishikawa, Norito; Okamoto, Yoshihiro; Hori, Fuminobu*; Matsui, Toshiyuki*; Iwase, Akihiro*
Nuclear Instruments and Methods in Physics Research B, 277, p.53 - 57, 2012/04
Times Cited Count：11 Percentile：63.06(Instruments & Instrumentation)To study the effects of GdO-doping and the irradiation with high energy fission products in the nuclear fuels (UO), GdO-doped CeO pellets were irradiated with 200 MeV Xe
ions. Effects of GdO-doping and the ion irradiation were estimated by using Extended X-ray Absorption Fine Structure (EXAFS) measurement. The interatomic distances between each Ce and the first nearest O atoms, and Ce and the second nearest Ce atoms increase by the irradiation and the effect of the ion irradiation on the atomic distances is more pronounced for higher amounts of dopant. The Debye-Waller factors for Ce-O and Ce-Ce pairs increase with increasing the amount of GdO dopant. These results suggest that the lattice binding energy is weakened by GdO-doping. The Debye-Waller factors increase also by the irradiation. The effect of ion irradiation on the Debye-Waller factors, however, becomes smaller for higher amounts of dopant.
O-doped CeO by means of synchrotron radiation X-ray spectroscopyTahara, Yuki*; Shimizu, Hirotaka*; Ishikawa, Norito; Okamoto, Yoshihiro; Hori, Fuminobu*; Matsui, Toshiyuki*; Iwase, Akihiro*
Nuclear Instruments and Methods in Physics Research B, 277, p.53 - 57, 2012/04
In this study, to simulate such an environment, GdO-doped CeO samples were irradiated with 200 MeV Xe ions at room temperature using an ion beam accelerator at JAEA-Tokai. As CeO has the same fluorite structure as that of UO and several properties of CeO are similar to UO, in this study CeO was used as a simulation material of UO. To study the effects of the ion irradiation on GdO-doped CeO, extended X-ray absorption fine structure (EXAFS) and X-ray photoelectron spectroscopy (XPS) were used at the Photon Factory of High Energy Accelerator Research Organization (KEK) as well as conventional X-ray diffraction (XRD) measurement. The EXAFS and XRD spectra show that the effects of the ion irradiation are more pronounced for higher amount of GdO dopant.
Aiko, Kazuma*; Toki, Atsushi*; Matsui, Toshiyuki*; Iwase, Akihiro*; Sato, Takahiro; Takano, Katsuyoshi*; Koka, Masashi; Saito, Yuichi; Kamiya, Tomihiro; Okochi, Takuo*; et al.
Journal of Synchrotron Radiation, 19(2), p.223 - 226, 2012/03
Times Cited Count：7 Percentile：36.52(Instruments & Instrumentation)
Mn)O thin filmMatsui, Toshiyuki*; Iwase, Akihiro*; Yamamoto, Hiroyuki; Hirao, Norie; Baba, Yuji
Photon Factory Activity Report 2011, Part B, P. 243, 2012/00
no abstracts in English
Al cable-in-conduit conductorKoizumi, Norikiyo; Matsui, Kunihiro; Hemmi, Tsutomu; Nakajima, Hideo; Takeuchi, Takao*; Banno, Nobuya*; Kikuchi, Akihiro*
Teion Kogaku, 46(8), p.495 - 499, 2011/08
JAEA and NIMS has been collaborating in development of high performance Rapid-Heating-Quenching-Transformation (RHQT) NbAl CIC conductor, aiming at the application of this conductor to DEMO plant. The technical issue of the RHQT NbAl strand in the application to a fusion magnet is stabilization against perturbation. NIMS developed technique to attach copper stabilizer by using electroplating and a sub-scale CIC conductor is developed using this conductor. JAEA performed stability test of the developed CIC conductor to demonstrate efficiency of this copper stabilization technique. The measured stability margin is sufficiently high compared to the one of similar NbTi CIC conductor previously tested by the authors. Then, it can be concluded that the copper stabilizer works efficiently from view point of stability, resulting in solving the remained technical issues in the RHQT CIC conductor. Therefore, we can say that the RHQT NbAl CIC conductor is the most promising candidate for application to magnet in DEMO plant.
Kosugi, Shinya*; Fujita, Naoki*; Matsui, Toshiyuki*; Hori, Fuminobu*; Saito, Yuichi; Ishikawa, Norito; Okamoto, Yoshihiro; Iwase, Akihiro*
Nuclear Instruments and Methods in Physics Research B, 269(9), p.869 - 872, 2011/05
Times Cited Count：10 Percentile：60.56(Instruments & Instrumentation)Effects of thermal annealing on ion-irradiation induced ferromagnetism of FeRh bulk alloy and the related structural change were investigated by means of superconducting quantum interference device (SQUID) and extended X-ray absorption fine structure (EXAFS), respectively. Depending on the annealing temperature from 100 to 500 C, the magnetization induced by 10 MeV iodine ion irradiation and the lattice structure of the alloy were remarkably changed. After 500 C annealing, the magnetization and the lattice ordering of the alloy become similar to the states before the irradiation. The experimental result indicates that the thermal relaxation of irradiation-induced atomic disordering dominates the magnetic state of ion-irradiated FeRh alloy.
doped with GdOTahara, Yuki*; Zhu, B.-L.*; Kosugi, Shinya*; Ishikawa, Norito; Okamoto, Yoshihiro; Hori, Fuminobu*; Matsui, Toshiyuki*; Iwase, Akihiro*
Nuclear Instruments and Methods in Physics Research B, 269(9), p.886 - 889, 2011/05
Times Cited Count：16 Percentile：75.56(Instruments & Instrumentation)CeO pellets doped with GdO were irradiated with 200-MeV Xe ions, and the effects of GdO-doping and irradiation on the lattice structure were measured using XRD and EXAFS. The lattice constant decreases with increasing GdO-doping and the local structure near the Gd atoms is more disordered with increasing amounts of GdO-dopant. The irradiation induces an expansion of the lattice and disordering of the atomic arrangement around Gd atoms. The effect of high-energy ion irradiation becomes more pronounced with increasing amounts of GdO-dopant.
