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草野 完也*; 一本 潔*; 石井 守*; 三好 由純*; 余田 成男*; 秋吉 英治*; 浅井 歩*; 海老原 祐輔*; 藤原 均*; 後藤 忠徳*; et al.
Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12
被引用回数：6 パーセンタイル：51.19(Geosciences, Multidisciplinary)PSTEPとは、2015年4月から2020年3月まで日本国内の太陽・地球惑星圏に携わる研究者が協力して実施した科研費新学術領域研究である。この研究枠組みから500以上の査読付き論文が発表され、様々なセミナーやサマースクールが実施された。本論文では、その成果をまとめて報告する。
吉田 寿雄*; 山本 旭*; 細川 三郎*; 山添 誠司*; 吉川 聡一*; 原 賢二*; 中村 充孝; 蒲沢 和也*; 田中 庸裕*
Topics in Catalysis, 64(9-12), p.660 - 671, 2021/08
被引用回数：2 パーセンタイル：11.54(Chemistry, Applied)Inelastic neutron scattering (INS) enables direct and selective observation of H species due to the extremely large incoherent neutron scattering cross section of a hydrogen atom. In the present study, the adsorbed H species on some heterogeneous precious metal catalysts supported by alumina and carbon black were investigated by in situ INS spectroscopy with a newly designed sample cell. Three alumina-supported metal catalysts having Pt, Pd, and Rh metal nanoparticles with different particle sizes exhibited different INS spectra in intensities and band distribution. Observation of the H species on the metal nanoparticles and the alumina surface revealed their properties. In addition, the H atoms stored in Pd nanoparticles were observed as palladium hydride. In contrast, the H species on a Pt catalyst supported by carbon black were found to be strongly adsorbed on the carbon support.
中西 利典*; 奥野 充*; 山崎 圭二*; Hong, W.*; 藤田 奈津子; 中村 俊夫*; 堀川 義之*; 佐藤 鋭一*; 木村 治夫*; 堤 浩之*
名古屋大学年代測定研究,5, p.38 - 43, 2021/03
雲仙火山の約13km西方にある唐比低地には泥炭層や泥層からなる湿地堆積物が厚く分布しており、それらの堆積物には千々石断層や雲仙火山の活動履歴が記録されていることが期待される。それらの履歴を精度よく検知するために、複数本のボーリングコアを掘削して放射性炭素年代値を測定した。それらの結果を地中レーダ探査断面と対比して湿地堆積物の形成過程を検討した。その結果得られたすべての
C年代値は層序関係と矛盾がなく、堆積曲線は若干のずれが認められるが概ね一致する結果となった。本研究の年代測定の一部はペレトロン年代測定装置による施設供用利用で行われたものである。
北里 宏平*; Milliken, R. E.*; 岩田 隆浩*; 安部 正真*; 大竹 真紀子*; 松浦 周二*; 高木 靖彦*; 中村 智樹*; 廣井 孝弘*; 松岡 萌*; et al.
Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03
被引用回数：43 パーセンタイル：96.93(Astronomy & Astrophysics)2019年4月「はやぶさ2」ミッションは、地球に近い炭素質の小惑星(162173)リュウグウの人工衝撃実験を成功させた。これは露出した地下物質を調査し、放射加熱の潜在的な影響をテストする機会を提供した。はやぶさ2の近赤外線分光器(NIRS3)によるリュウグウの地下物質の観測結果を報告する。発掘された材料の反射スペクトルは、表面で観測されたものと比較して、わずかに強くピークがシフトした水酸基(OH)の吸収を示す。これは、宇宙風化や放射加熱が最上部の表面で微妙なスペクトル変化を引き起こしたことを示している。ただし、このOH吸収の強度と形状は、表面と同様に、地下物質が300
Cを超える加熱を経験したことを示している。一方、熱物理モデリングでは、軌道長半径が0.344AUに減少しても、推定される掘削深度1mでは放射加熱によって温度が200Cを超えて上昇しないことが示されている。これは、リュウグウ母天体が放射加熱と衝撃加熱のいずれか、もしくは両方により熱変化が発生したという仮説を裏付けている。
S郷 慎太郎*; 井手口 栄治*; 横山 輪*; 青井 考*; Azaiez, F.*; 古高 和禎; 初川 雄一; 木村 敦; 木佐森 慶一*; 小林 幹*; et al.
Physical Review C, 103(3), p.034327_1 - 034327_8, 2021/03
被引用回数：4 パーセンタイル：57.13(Physics, Nuclear)Excited states in S were investigated by in-beam 
-ray spectroscopy using the 
Mg(
O, 2
1
) fusion-evaporation reaction. The de-exciting -rays were measured with germanium detector arrays along with the measurement of evaporated charged particles in a 
segmented Si detector array. The level scheme was extended up to 12470 keV. The obtained level structure is compared with the large-scale shell-model calculations. The possibility of isoscalar-pair excited states is discussed for 
states with comparison between the experimental and theoretical results.
O
by 
inelastic neutron scattering and their reactivity with ethylene山添 誠司*; 山本 旭*; 細川 三郎*; 福田 良一*; 原 賢二*; 中村 充孝; 蒲沢 和也*; 佃 達哉*; 吉田 寿雄*; 田中 庸裕*
Catalysis Science & Technology, 11(1), p.116 - 123, 2021/01
被引用回数：6 パーセンタイル：34.43(Chemistry, Physical)Hydrogen (H) species adsorbed on catalyst surfaces are key intermediates in catalytic hydrogenation reactions over supported metal catalysts. However, individual identification of H species on the metal catalysts has not been established to date. Here, we elucidated the H species on Pt/AlO by the combination of inelastic neutron scattering (INS) and density functional theory (DFT). Several H species in the presence of H were successfully identified at different sites on the Pt surface and AlO support. The INS and FT-IR measurements revealed that the hydride/atop Pt-H, bridged perimeter/terrace Pt-H-Pt, and threefold Pt-H are active intermediates in the CH
hydrogenation reaction, whereas the edge Pt-H-Pt is a rather inert species. In addition, the measurements indicate that the AlO itself acts as hydrogen storage material by mediating AlO-H and Al-H-Al species, which serve H species in the CH hydrogenation reaction.
吉富 寛; 古渡 意彦; 萩原 雅之*; 長畔 誠司*; 中村 一*
Radiation Protection Dosimetry, 184(2), p.179 - 188, 2019/08
被引用回数：2 パーセンタイル：21.58(Environmental Sciences)To manage the equivalent doses for radiation workers, exposure inhomogeneity is an important factor in the decision-making process related to protection measures and additional monitoring. Our previous study proposed the methodology to evaluate the inhomogeneity of exposure quantitatively. In this study, we applied proposed method to five different types of actual exposure situations in the nuclear industry. Two of them were conventionally characterized as homogeneous exposure, but the other three as inhomogeneous exposure. The evaluation of homogeneity exposure was conducted using Monte Carlo calculations with two simplified models, which were then verified with phantom experiments. Consequently, all of the evaluations reproduced the experimental results, implying that our proposed method would be applicable for actual work conditions in the nuclear industry. Furthermore, the two presumed homogeneous exposure situations were found to be rather inhomogeneous because of the contribution of positrons and the limited source region. The investigation also implies that obtaining the information on the most probable posture of the exposed worker, as well as the existence of the weekly penetrating radiation such as 
ray as a main source of exposure would be the key for more precise estimation.
北里 宏平*; Milliken, R. E.*; 岩田 隆浩*; 安部 正真*; 大竹 真紀子*; 松浦 周二*; 荒井 武彦*; 仲内 悠祐*; 中村 智樹*; 松岡 萌*; et al.
Science, 364(6437), p.272 - 275, 2019/04
被引用回数：259 パーセンタイル：99.73(Multidisciplinary Sciences)小惑星探査機はやぶさ2のターゲット天体であるリュウグウは、始原的な炭素質物質で構成されていると考えられている。はやぶさ2に搭載された近赤外分光計(NIRS3)によって、天体の表面組成を得た。天体全体の観測で、弱く細い吸収が2.72ミクロンに確認され、OHを含む鉱物の存在を示している。弱いOH吸収と低いアルベドは熱やショックによって変質を受けた炭素質コンドライトに似ている。OHバンドの位置はほとんど一定であり、衝撃片の集合によって形成されたリュウグウは組成的に均質であることを示している。
末國 晃一郎*; Lee, C. H.*; 田中 博己*; 西堀 英治*; 中村 篤*; 笠井 秀隆*; 森 仁志*; 臼井 秀知*; 越智 正之*; 長谷川 巧*; et al.
Advanced Materials, 30(13), p.1706230_1 - 1706230_6, 2018/03
被引用回数：51 パーセンタイル：89.35(Chemistry, Multidisciplinary)高性能デバイスとしての熱電材料には、高い電気伝導度と低い熱伝導度という相反する要求を同時に満たす必要がある。本研究では、テトラへドライト(Cu,Zn)
(Sb,As)S
の結晶構造とフォノンダイナミクスを調べ、平面内に配位している銅原子のラットリング運動がフォノンを効率良く散乱することを見出した。これらの知見は、平面配位構造を有する高性能熱電材料の新たな開発指針を与えるものである。
and O/HO adsorption revealed by in situ XAFS and hard X-ray photoelectron spectroscopyCui, Y.*; 原田 慈久*; 畑中 達也*; 中村 直樹*; 安藤 雅樹*; 吉田 稔彦*; 池永 英司*; 石井 賢司*; 松村 大樹; Li, R.*; et al.
ECS Transactions, 72(8), p.131 - 136, 2016/10
被引用回数：1 パーセンタイル：48.91(Electrochemistry)The electronic structures of Pt and Pt-Co nanoparticles with O adsorption and O/HO co-adsorption were investigated by in situ hard X-ray photoelectron spectroscopy (HAXPES) and in situ high resolution fluorescence detection X-ray absorption spectroscopy (HERFD-XAS) to clarify the effects of water adsorption on fuel cell cathode catalysis surface. The experimental results suggest that under the pressure of 1 mbar, the adsorption of HO hinders the successive O adsorption on Pt surface, while under the pressure of 1 bar, the adsorption of HO enhances the adsorption of O on Pt surface. This water effect is found to be more significant on Pt surface than on Pt-Co surface. These results would be helpful to understand how the water affects the fuel cell performance and why Pt-Co nanoparticles show higher oxygen reduce reaction (ORR) activity than Pt nanoparticles.
S郷 慎太郎*; 井手口 栄治*; 横山 輪*; 小林 幹*; 木佐森 慶一*; 高木 基伸*; 宮 裕之*; 大田 晋輔*; 道正 新一郎*; 下浦 享*; et al.
JPS Conference Proceedings (Internet), 6, p.030005_1 - 030005_4, 2015/06
The high-spin states in S were investigated at Tandem-ALTO facility in Institut de Physique Nucl
aire d'Orsay The Mg(O, 21n)S fusion evaporation reaction was used to populate high-spin states in S. The germanium -ray detector array ORGAM was employed to measure rays from high-spin states and charged particles evaporated from the compound nuclei were detected by a segmented silicon detector, Si-Ball. A level scheme for S was deduced based on the gamma-gamma-coincidence analysis and -ray angular correlation analysis. The half-life of the transition in the superdeformed band was estimated by measuring the residual Doppler shift. The deduced half-life shows the large collectivity of the band.
山口 洋司*; 伊地知 亮*; 鈴木 善之*; 大岡 幸代*; 島田 啓二*; 高橋 直*; 鷲尾 英俊*; 中村 一世*; 高本 達也*; 今泉 充*; et al.
Proceedings of 42nd IEEE Photovoltaic Specialists Conference (PVSC-42) (CD-ROM), p.2407 - 2411, 2015/06
In order to develop high efficiency space solar cells with flexible and light weight, InGaP/GaAs/Ge Inverted Triple Junction (IMM-3J) solar cells mounted on film type sheet (film type space solar sheet) and glass type sheet (glass type space solar sheets) were fabricated and their reliability was investigated. As a result, no significant change in their characteristics (less than 1 % change) was observed for both types of space solar sheets after reliability tests, such as (1) thermal cycling (-180 to +120 C, 1000 cycles), (2) humidity and temperature (65 C, humidity 90 %, 720h), (3) high temperature under vacuum condition (160 C, less than 10
Torr, 168h), and (4) high temperature (150 C, 1000 h). Both type space solar sheets also showed high radiation resistance compared to current version of space 3J solar cells. Therefore, we can conclude that the space solar sheets have enough reliability in space environments.
Hwang, J.-G.*; Kim, E.-S.*; 宮島 司*; 本田 洋介*; 原田 健太郎*; 島田 美帆*; 高井 良太*; 久米 達哉*; 長橋 進也*; 帯名 崇*; et al.
Nuclear Instruments and Methods in Physics Research A, 753, p.97 - 104, 2014/07
被引用回数：7 パーセンタイル：48.36(Instruments & Instrumentation)For a future synchrotron light source based on a linac, e.g. an X-ray free electron laser and an energy recovery linac (ERL), an injector is a key component to generate a high brightness electron beam. For the acceleration and transportation of the electron beam in the injector, the adjustment of beam orbit inside the cavity is important to avoid the deterioration of the beam quality due to the transverse electric field of it, which causes the transverse emittance growth. To adjust the beam orbit, an investigation of the electromagnetic center of the cavity is required in the beam operation. This paper shows a new method for measuring the electromagnetic center of the cavity, and describes an analytical model of emittance growth due to a combination of transverse electric field and orbit offset. The validation of the method was confirmed by the emittance measurement in the compact ERL (cERL) injector at KEK.
宮本 斉児; 杉原 正芳*; 新谷 吉郎*; 中村 幸治*; 利光 晋一*; Lukash, V. E.*; Khayrutdinov, R. R.*; 杉江 達夫; 草間 義紀; 芳野 隆治*
Fusion Engineering and Design, 87(11), p.1816 - 1827, 2012/11
被引用回数：15 パーセンタイル：71.22(Nuclear Science & Technology)Vertical displacement events (VDEs) and disruptions usually take place under intervention of vertical stability (VS) control and the vertical electromagnetic force induced on vacuum vessels is potentially influenced. This paper presents assessment of the force that arises from the VS control in ITER VDEs using a numerical simulation code DINA. The focus is on a possible malfunctioning of the VS control circuit: radial magnetic field is unintentionally applied to the direction of enhancing the vertical displacement further. Since this type of failure usually causes the largest forces (or halo currents) observed in the present experiments, this situation must be properly accommodated in the design of the ITER vacuum vessel. DINA analysis shows that although the VS control modifies radial field, it does not affect plasma motion and current quench behavior including halo current generation because the vacuum vessel shields the field created by the VS control coils. Nevertheless, the VS control modifies the force on the vessel by directly acting on the eddy current carried by the conducting structures of the vessel. Although the worst case was explored in a range of plasma inductance and pattern of VS control, the result confirmed that the force is still within the design margin.
Z nucleus, 
Ar and high-spin states in A = 30 
40 nuclei井手口 栄治*; 大田 晋輔*; 森川 恒安*; 大島 真澄; 小泉 光生; 藤 暢輔; 木村 敦; 原田 秀郎; 古高 和禎; 中村 詔司; et al.
Progress of Theoretical Physics Supplement, (196), p.427 - 432, 2012/10
A rotational band with five cascade -ray transitions was newly found in Ar. The deduced transition quadrupole moment of 
eb has demonstrated this band as having a superdeformed shape of 
0.5. The structure of the band was discussed in the framework of cranked Hartree-Fock-Bogoliubov calculations and the assignment of multiparticle-multihole configuration has been made.
桐原 明宏*; 内田 健一*; 梶原 瑛祐*; 石田 真彦*; 中村 泰信*; 眞子 隆志*; 齊藤 英治; 萬 伸一*
Nature Materials, 11(8), p.686 - 689, 2012/08
被引用回数：239 パーセンタイル：98.59(Chemistry, Physical)Energy harvesting technologies, which generate electricity from environmental energy, have been attracting great interest because of their potential to power ubiquitously deployed sensor networks and mobile electronics. Of these technologies, thermoelectric (TE) conversion is a particularly promising candidate, because it can directly generate electricity from the thermal energy that is available in various places. Here we show a novel TE concept based on the spin Seebeck effect, called "spin-thermoelectric (STE) coating", which is characterized by a simple film structure, convenient scaling capability, and easy fabrication. The STE coating, with a 60-nm-thick bismuth-substituted yttrium iron garnet (Bi:YIG) film, is applied by means of a highly efficient process on a non-magnetic substrate. Notably, spin-current-driven TE conversion is successfully demonstrated under a temperature gradient perpendicular to such an ultrathin STE-coating layer (amounting to only 0.01% of the total sample thickness). We also show that the STE coating is applicable even on glass surfaces with amorphous structures. Such a versatile implementation of the TE function may pave the way for novel applications making full use of omnipresent heat.
金村 卓治; 近藤 浩夫; 鈴木 幸子*; 帆足 英二*; 山岡 信夫*; 堀池 寛*; 古川 智弘; 井田 瑞穂; 中村 和幸; 松下 出*; et al.
Fusion Science and Technology, 62(1), p.258 - 264, 2012/07
被引用回数：4 パーセンタイル：31.96(Nuclear Science & Technology)本論文は、核融合炉候補材料の中性子照射試験施設である国際核融合材料照射施設(IFMIF)の研究開発にかかわるものである。現在幅広いアプローチ(BA)活動の1つである、IFMIFの工学実証・工学設計活動(EVEDA)プロジェクトが日欧協力で進められている。本プロジェクトの枠組みで大洗研究開発センターに製作されたEVEDA液体Li試験ループ(ELTL)は、Liターゲットの安定性評価等に供する。ELTLにおいて、Liターゲットを模擬した液体Li噴流の表面変動の計測に供する機器として、触針式液面計を開発した。本液面計は、触針と液面との接触を電圧降下として検知し、噴流の平均厚さや振幅の分布などの変動特性を取得するものである。開発の要点は、10
Paの真空下で触針を0.1mmの分解能、0.01mmの位置決め精度で動作させることである。この条件を満たすため、モーメント荷重とセンサーの自重荷重を計算し、その計算結果に基づいて、装置内外での1気圧の差圧に耐えて位置決めできるモータと摩擦を低減したボールねじを選定し、強固な構造を適用することとした。以上の結果、所定の性能を満たす設計を完了した。
細井 卓治*; 桐野 嵩史*; 上西 悠介*; 池口 大輔*; Chanthaphan, A.*; 吉越 章隆; 寺岡 有殿; 箕谷 周平*; 中野 佑紀*; 中村 孝*; et al.
Workshop digest of 2012 Asia-Pacific Workshop on Fundamentals and Applications of Advanced Semiconductor Devices (AWAD 2012), p.22 - 25, 2012/06
SiC is a promising material for high-power electronic devices. Although SiO film can be grown on SiC by thermal oxidation, low channel mobility and poor gate oxide reliability are the critical issues for SiC power MOSFETs. In this work, we investigated the fundamental aspects of thermally-grown SiO/4H-SiC structures such as an energy band alighnment and flatband voltage instability. Both electrical characterization and XPS study revealed that a conduction band offset between SiO and SiC is extrinsically increased. High temperature annealing in H could passivate mobile ions existing in as-oxidized SiO/SiC structures. Post-oxidation annealing in Ar eliminates the mobile ions, but they are generated again by subsequent high-temperature hydrogen annealing. These features were not observed for SiO/Si structures, and thus considered to be inherent to thermally grown SiO/SiC structures.
渡部 平司*; 細井 卓治*; 桐野 嵩史*; 上西 悠介*; Chanthaphan, A.*; 吉越 章隆; 寺岡 有殿; 箕谷 周平*; 中野 佑紀*; 中村 孝*; et al.
Materials Science Forum, 717-720, p.697 - 702, 2012/05
被引用回数：2 パーセンタイル：73.92(Materials Science, Multidisciplinary)We investigated the interface between oxide and 4H-SiC(0001) Si-face or (000-1) C-face by synchrotron radiation photoelectron spectroscopy. The Si 2p
spectra were fitted with bulk SiC and SiO together with intermediate oxides (Si
, Si
, Si
). The total amount of intermediate states was sufficiently small compared with that of the remaining oxides. This implies that the transition layer in the oxide is as thin as a few atomic layers. Moreover, the chemical composition in the bulk region was found to be almost identical to that of the initial SiC surface. These results indicate formation of a near-perfect SiO/SiC interface.
/4H-SiC interface細井 卓治*; 桐野 嵩史*; Chanthaphan, A.*; 上西 悠介*; 池口 大輔*; 吉越 章隆; 寺岡 有殿; 箕谷 周平*; 中野 佑紀*; 中村 孝*; et al.
Materials Science Forum, 717-720, p.721 - 724, 2012/05
被引用回数：5 パーセンタイル：91.62(Materials Science, Multidisciplinary)The energy band alignments of thermally grown SiO/SiC structures were investigated by means of synchrotron radiation photoelectron spectroscopy (SR-PES) and electrical characterization of SiC-MOS capacitors. In order to determine the energy band alignments of SiO/SiC, band gaps of the thermal oxides and valence band offsets at the interface were examined by SR-PES. SiC-MOS capacitors with Al electrodes were also fabricated to evaluate interface state density and conduction band offset. Experimental results indicate that hydrogen atoms are effective to terminate carbon-related defects. It can be concluded that interface quality degradation due to hydrogen desorption by vacuum annealing causes reduction of conduction band offset for thermally grown SiO/SiC structure.
