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Kokubun, Yuji; Hosomi, Kenji; Nagaoka, Mika; Seya, Natsumi; Inoue, Kazumi; Koike, Yuko; Uchiyama, Rei; Sasaki, Kazuki; Maehara, Yushi; Matsuo, Kazuki; et al.
JAEA-Review 2024-054, 168 Pages, 2025/03
JAEA-Review-2024-054.pdf:2.73MB
The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2023 to March 2024 and the results of dose calculations for the surrounding public due to the release of radioactive materials from the plant into the atmosphere and ocean. In the results of the above environmental radiation monitoring, several items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Holdings, Inc. on April 1, 2016), which occurred in March 2011. In addition, environmental monitoring plan, analysis and measurement methods, monitoring data and their chronological change, meteorological data after statistical processing, status of radioactive waste release and evaluation results of the data over the normal range are included as appendices.
Sugimoto, Satoshi*; Araki, Yasufumi; Takahashi, Yukiko*; Ieda, Junichi; Kasai, Shinya*
Communications Physics (Internet), 8, p.100_1 - 100_9, 2025/03
Times Cited Count：0 Percentile：0.00(Physics, Multidisciplinary)
rays in the 
La(
)
La reactionOkuizumi, Mao*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ino, Takashi*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; et al.
Physical Review C, 111(3), p.034611_1 - 034611_6, 2025/03
Times Cited Count：0Kato, Toru*; Takahashi, Hiroki*; Yamashita, Meguru*; Doi, Akio*; Imabuchi, Takashi
Artificial Life and Robotics, 30(1), p.126 - 135, 2025/02
Ito, Kengo*; Takahashi, Shin*; Kato, Chizu*; Fukutani, Satoshi*; Matsumura, Tatsuro; Fujii, Toshiyuki*
Journal of Radioanalytical and Nuclear Chemistry, 334, p.2467 - 2475, 2025/02
Times Cited Count：0 Percentile：0.00(Chemistry, Analytical)In this study, the solvent extraction behavior of tin (Sn), specifically 
Sn, from high-level radioactive waste was evaluated using six different extractants in a HNO
system. Among the tested extractants, N,N-Didodecyl-2-hydroxyacetoamide (HAA) exhibited higher efficiency, still not sufficient for industrial implementation. In systems where HCl was added to HNO, both tributyl phosphate (TBP) and N,N,N,N'-tetra-2-ethylhexyl diglycolamide (TEHDGA) achieved D
values greater than 1 at 
1 M HCl. However, due to practical challenges in industrial applications, HAA extraction in HNO systems, particularly at low Sn concentrations (0.0008 M), may provide a more effective solution for Sn recovery.
Yamaguchi, Akiko; Okumura, Masahiko; Kawamura, Naomi*; Takahashi, Yoshio*
Science of the Total Environment, 964, p.178585_1 - 178585_13, 2025/02
There are many unresolved issues in the adsorption reactions of clay minerals. One of the reasons is the existence of multiple adsorption sites. It is known that the contribution of each adsorption site depends on the concentration of adsorbed ions, and there is a challenge in comprehensively correlate the results of atomic-level simulations that employ limited number of atoms and inevitably deal high-concentration samples with actual environmental samples where concentrations are orders of magnitude lower. In this study, we combined experiments using synchrotron radiation and first-principles calculations to comprehensively elucidate the systematic changes in the local structure of adsorption sites and adsorbed ions based on the adsorption concentration at the atomic level, and demonstrated that the interaction between adsorbed ions and clay minerals involves ionic bonding.
Takahashi, Yoshio*; Yamaguchi, Akiko; Yomogida, Takumi
Treatise on Geochemistry, 3rd edition, Vol.6, p.105 - 150, 2025/00
With the recent development of measurement techniques, new approaches to the environmental geochemistry of radionuclides have been applied for various research targets. In this review article, several topics within the last 10-15 years in the field of environmental geochemistry of radionuclides have been discussed. In particular, this article mainly focused on two topics, (i) studies on the migration of radionuclides emitted by the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident in 2011 and (ii) the development of X-ray absorption fine structure (XAFS) spectroscopy and its application to the geochemical processes of radionuclides.
Nagasawa, Makoto*; Shimizu, Yusuke*; Yamaguchi, Akiko; Tokunaga, Kohei; Mukai, Hiroki*; Aoyagi, Noboru; Mei, H.; Takahashi, Yoshio*
Chemical Geology, 670, p.122431_1 - 122431_25, 2024/12
Times Cited Count：1 Percentile：0.00(Geochemistry & Geophysics)Yamaguchi, Akiko; Takahashi, Yoshio*; Okumura, Masahiko
Isotope News, (796), p.21 - 23, 2024/12
Clay minerals are abundant in soils and control the environmental behavior of various elements because they adsorb many cations. Since the strength of adsorption of clay minerals depends on the adsorption structure at the molecular level, a systematic understanding of what determines the adsorption structure at the molecular level is important. In this study, we systematically elucidated the adsorption structures of many cations, including radium, using extensive X-ray absorption fine structure (EXAFS) measurements and first-principles simulations. The results show that the size and hydration enthalpy of adsorbed ions are important in determining the adsorption structure.
Iwami, Satone*; Yamashita, Takuma*; Mitsuyasu, Yusuke*; Ono, Kenta*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.
KEK Proceedings 2024-6, p.91 - 95, 2024/12
We aim to improve the detection limit of the ESR dosimetry method. In this study, the saturation behavior of each radical was investigated by varying the microwave power during ESR measurement. Based on the difference in spin relaxation time between carbonate radicals and native radicals, it is expected that the signal-to-noise ratio improves and the detection limit can be lowered when the microwave power is increased to 4.0 mW.
Yamashita, Takuma*; Iwami, Satone*; Mitsuyasu, Yusuke*; Ono, Kenta*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.
KEK Proceedings 2024-6, p.85 - 90, 2024/12
To clarify the radiation effects of the accident at the TEPCO's Fukushima Daiichi NPP on living organisms, it is important to accurately estimate the dose to each individual. We have developed a multi-component analysis program using random number optimization to extract only the components derived from carbonate radicals from the ESR spectra.
Koizumi, Mitsuo; Ito, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Arikawa, Yasunobu*; Abe, Yuki*; Wei, T.*; Yogo, Akifumi*; et al.
Dai-45-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2024/11
Machida, Masahiko; Yamada, Susumu; Kim, M.; Tanaka, Satoshi*; Tobita, Yasuhiro*; Iwata, Ayako*; Aoki, Yuto; Aoki, Kazuhisa; Yanagisawa, Kenichi*; Yamaguchi, Takashi; et al.
RIST News, (70), p.3 - 22, 2024/09
Inside the Fukushima Daiichi Nuclear Power Plant (1F), there are many locations with high radiation levels due to contamination by radioactive materials that leaked from the reactor. These pose a significant obstacle to the smooth progress of decommissioning work. To help solve this issue, the Japan Atomic Energy Agency (JAEA), under a subsidy from the Ministry of Economy, Trade, and Industry's decommissioning and contaminated water management project, is conducting research and development on digital technologies to improve the radiation environment inside the decommissioning site. This project, titled "Development of Technology to Improve the Environment Inside Reactor Buildings (Enhancing Digital Technology for Environment and Source Distribution to Reduce Radiation Exposure)," began in April of FY 2023. In this project, the aim is to develop three interconnected systems: FrontEnd, Pro, and BackEnd. The FrontEnd system, based on the previously developed 3D-ADRES-Indoor (prototype) from FY 2021-2022, will be upgraded to a high-speed digital twin technology usable on-site. The Pro system will carry out detailed analysis in rooms such as the new office building at 1F, while the BackEnd system will serve as a database to centrally manage the collected and analyzed data. This report focuses on the FrontEnd system, which will be used on-site. After point cloud measurement, the system will quickly create a 3D mesh model, estimate the radiation source from dose rate measurements, and refine the position and intensity of the estimated source using recalculation techniques (re-observation instructions and re-estimation). The results of verification tests conducted on Unit 5 are also presented. Furthermore, the report briefly discusses the future research and development plans for this project.
Koizumi, Mitsuo; Ito, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Arikawa, Yasunobu*; Abe, Yuki*; Lan, Z.*; Wei, T.*; et al.
Scientific Reports (Internet), 14, p.21916_1 - 21916_9, 2024/09
Times Cited Count：0 Percentile：0.00(Multidisciplinary Sciences)Endo, Shunsuke; Abe, Ryota*; Fujioka, Hiroyuki*; Ino, Takashi*; Iwamoto, Osamu; Iwamoto, Nobuyuki; Kawamura, Shiori*; Kimura, Atsushi; Kitaguchi, Masaaki*; Kobayashi, Ryuju*; et al.
European Physical Journal A, 60(8), p.166_1 - 166_10, 2024/08
Times Cited Count：2 Percentile：0.00(Physics, Nuclear)Takyu, Sodai*; Matsumoto, Kenichiro*; Hirade, Tetsuya; Nishikido, Fumihiko*; Akamatsu, Go*; Tashima, Hideaki*; Takahashi, Miwako*; Yamaya, Taiga*
Japanese Journal of Applied Physics, 63(8), p.086003_1 - 086003_8, 2024/08
Times Cited Count：1 Percentile：46.22(Physics, Applied)Positrons and electrons sometimes exist as a bound state, positronium (Ps), in living organisms. The triplet Ps (ortho-Ps) annihilation time represents the ortho-Ps pick-off annihilation lifetime, and it varies depending on the surrounding electron density. The ortho-Ps lifetime may add new biological information to PET scan information. In order to discuss the feasibility of quantifying (free) radicals in vivo by the ortho-Ps lifetime, we used a clinical PET system to make ortho-Ps lifetime measurements in aqueous solutions containing radicals. The results suggested that differences in radical concentrations in aqueous solutions of the order of a few mM could be quantified by the ortho-Ps lifetime if the counting statistic of the positron annihilation events was more than 10
events. This concentration was higher than the radical concentration generated in the physiological functions of living organisms.
Kobayashi, Fuminori; Kamiya, Junichiro; Takahashi, Hiroki; Suzuki, Yasuo*; Tasaki, Ryuta*
JAEA-Technology 2024-007, 28 Pages, 2024/07
JAEA-Technology-2024-007.pdf:2.52MB
In J-PARC LINAC, the vacuum system is in place to maintain an ultra-high vacuum in the beam transport line (LINAC to 3GeV RCS beam transportation line: L3BT) between the LINAC to the 3GeV synchrotron. The vacuum system is installed in the LINAC and L3BT buildings and consists of vacuum pumps, vacuum gauges, beam line gate valves (BLGVs), and other vacuum. In existing vacuum systems, vacuum equipment is controlled independently for each area, and vacuum equipment can be operated regardless of the status of adjacent areas. This makes it impossible to eliminate erroneous operation due to human error. In addition, when a vacuum deterioration occurs in the beam transport line, the vacuum deterioration ILK signal is transmitted to the BLGV relay unit via the MPS transmission signal, which causes the BLGVs to be forcibly closed. Because the ILK signal transmission range extends to all BLGVs in the L3BT, however, BLGVs in areas unaffected by vacuum deterioration are also forced to close. This could cause problems such as unnecessary open/close operations leading to more frequent maintenance cycles of the BLGVs. In addition, since the BLGV is operated using the MPS signal path, maintenance of the vacuum control system requires work involving the MPS signal path, making it difficult to maintain the vacuum control system alone and making the work complicated. To solve these problems, it is necessary to improve maintainability by separating the signal paths and automatically controlling BLGV separately. Therefore, the vacuum control system was modified and constructed with the aim of realizing a control system that takes into account the safety and efficient maintenance and operation of the L3BT vacuum system. This report summarizes the development and use of the L3BT vacuum system control system.
Li-glass detector to gamma rays by a coincidence methodIto, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Mochimaru, Takanori*; Hori, Junichi*; Terada, Kazushi*; Koizumi, Mitsuo
Nuclear Instruments and Methods in Physics Research A, 1064, p.169465_1 - 169465_9, 2024/07
Times Cited Count：0 Percentile：0.00(Instruments & Instrumentation)Rodriguez, D.; Akamatsu, Shunsuke*; Rossi, F.; Suzuki, Satoshi*; Takahashi, Tone
Proceedings of 65th Annual Meeting of the Institute of Nuclear Materials Management (Internet), 9 Pages, 2024/07
Takahashi, Rieko*; Taniguchi, Naoki
Zairyo To Kankyo, 73(6), p.153 - 163, 2024/06
Carbon steel is one of the candidate materials for overpacks in geological disposal of high-level radioactive waste, and is known to susceptible to stress corrosion cracking(SCC) depending on the condition in carbonate environment. In order to understand the influence of temperature on the SCC susceptibility of carbon steel, slow strain rate test (SSRT) of rolled steel were performed in NaHCO aqueous solution with varying temperature in the range of 303-393K for conditions of 0.1-0.5 mol/dm
, which is assumed to be the upper limit of carbonate concentration in groundwater in a geological disposal environment. As the results, no obvious influence of temperature on mechanical properties such as fracture strain ratio and reduction area ratio were observed, but SCC susceptibility based on SCC fracture ratio increased at relatively low temperatures of 303K and 323K. It was suggested that the reason for the higher SCC sensitivity at lower temperatures was due to slower repassivation at lower temperatures. Regarding the type of SCC, intergranular SCC was dominant at low temperatures and tended to transition to intergranular SCC at higher temperatures. Transgranular SCC tended to be observed at lower potentials than those at which intergranular SCC was observed.
