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Gretarsson, H.*; 野村 拓司; Jarrige, I.*; Lupascu, A.*; Upton, M. H.*; Kim, J.*; Casa, D.*; Gog, T.*; Yuan, R. H.*; Chen, Z. G.*; et al.
Physical Review B, 91(24), p.245118_1 - 245118_8, 2015/06
被引用回数:6 パーセンタイル:28.15(Materials Science, Multidisciplinary)We report an Fe -edge resonant inelastic X-ray scattering (RIXS) study of KFeSe. This material is an insulator, unlike many parent compounds of iron-based superconductors. We found a sharp excitation around 1 eV, which is resonantly enhanced when the incident photon energy is tuned near the pre-edge region of the absorption spectrum. The spectral weight and line shape of this excitation exhibit clear momentum dependence. In addition, we observe momentum-independent broad interband transitions at higher excitation energy of 3-7 eV. Calculations based on a 70 band orbital model, using a moderate = 2.5 eV, indicate that the 1 eV feature originates from the correlated Fe 3 electrons, with a dominant and orbital character. We find that a moderate yields a satisfying agreement with the experimental spectra, suggesting that the electron correlations in the insulating and metallic iron based superconductors are comparable.
Jarrige, I.*; 小谷 章雄*; 山岡 人志*; 辻井 直人*; 石井 賢司; Upton, M.*; Casa, D.*; Kim, J. H.*; Gog, T.*; Hancock, J. N.*
Physical Review Letters, 114(12), p.126401_1 - 126401_5, 2015/03
被引用回数:10 パーセンタイル:61.06(Physics, Multidisciplinary)We combine resonant inelastic X-ray scattering and model calculations in the Kondo lattice compound YbInCu, a system characterized by a dramatic increase in Kondo temperature and associated valence fluctuations below a first-order valence transition at T 42 K. The bulk-sensitive, element-specific, and valence-projected charge excitation spectra reveal an unusual quasigap in the Yb-derived state density which drives an instability of the electronic structure and renormalizes the low-energy effective Hamiltonian at the transition. Our results provide long-sought experimental evidence for a link between temperature-driven changes in the low-energy Kondo scale and the higher-energy electronic structure of this system.
Jarrige, I.*; 野村 拓司; 石井 賢司; Gretarsson, H.*; Kim, Y.-J.*; Kim, J.*; Upton, M.*; Casa, D.*; Gog, T.*; 石角 元志*; et al.
Physical Review B, 86(11), p.115104_1 - 115104_4, 2012/09
被引用回数:8 パーセンタイル:35.48(Materials Science, Multidisciplinary)鉄系高温超伝導体PrFeAsOとその親物質であるPrFeAsOに対して、運動量分解した共鳴非弾性X線散乱を初めて観測した。主な結果は次の2点である。まず、第一に、16バンドの模型を用いて、低エネルギーの励起が, 軌道の特性を有するバンド内遷移に支配されていることを示し、電子相関に強く依存していることを示す。これによって、クーロン斥力とフント結合を見積もることができる。特に軌道依存した電子相関におけるの果たす役割が明らかとなる。第二に、短距離の反強磁性相関が点での励起の説明には不可欠であることから、超伝導状態においてもそれが存在することが示される。