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論文

A Systematic approach for the adequacy analysis of a set of experimental databases: Application in the framework of the ATRIUM activity

Baccou, J.*; Glantz, T.*; Ghione, A.*; Sargentini, L.*; Fillion, P.*; Damblin, G.*; Sueur, R.*; Iooss, B.*; Fang, J.*; Liu, J.*; et al.

Nuclear Engineering and Design, 421, p.113035_1 - 113035_16, 2024/05

In the Best-Estimate Plus Uncertainty (BEPU) framework, the use of best-estimate code requires to go through a Verification, Validation and Uncertainty Quantification process (VVUQ). The relevance of the experimental data in relation to the physical phenomena of interest in the VVUQ process is crucial. Adequacy analysis of selected experimental databases addresses this problem. The outcomes of the analysis can be used to select a subset of relevant experimental data, to encourage designing new experiments or to drop some experiments from a database because of their substantial lack of adequacy. The development of a specific transparent and reproducible approach to analyze the relevance of experimental data for VVUQ still remains open and is the topic of this contribution. In this paper, the concept of adequacy initially introduced in the OECD/NEA SAPIUM (Systematic APproach for model Input Uncertainty quantification Methodology) activity is formalized. It is defined through two key properties, called representativeness and completeness, that allows considering the multifactorial dimension of the adequacy problem. A new systematic approach is then proposed to analyze the adequacy of a set of experimental databases. It relies on the introduction of two sets of criteria to characterize representativeness and completeness and on the use of multi-criteria decision analysis method to perform the analysis. Finally, the approach is applied in the framework of the new OECD/NEA ATRIUM activity which includes a set of practical IUQ exercises in thermal-hydraulics to test the SAPIUM guideline in determining input uncertainties and forward propagating them on an application case. It allows evaluating the adequacy of eight experimental databases coming from the Super Moby-dick, Sozzi-Sutherland and Marviken experiments and identifying the most adequate ones.

論文

Chiral Dirac fermion in a collinear antiferromagnet

Zhang, A.*; Deng, K.*; Sheng, J.*; Liu, P.*; Kumar, S.*; 島田 賢也*; Jiang, Z.*; Liu, Z.*; Shen, D.*; Li, J.*; et al.

Chinese Physics Letters, 40(12), p.126101_1 - 126101_8, 2023/12

 被引用回数:1 パーセンタイル:0(Physics, Multidisciplinary)

In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, itis predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral "Dirac-like" fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Here, by combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions.

論文

Extreme phonon anharmonicity underpins superionic diffusion and ultralow thermal conductivity in argyrodite Ag$$_{8}$$SnSe$$_{6}$$

Ren, Q.*; Gupta, M. K.*; Jin, M.*; Ding, J.*; Wu, J.*; Chen, Z.*; Lin, S.*; Fabelo, O.*; Rodriguez-Velamazan, J. A.*; 古府 麻衣子; et al.

Nature Materials, 22, p.999 - 1006, 2023/05

 被引用回数:21 パーセンタイル:99.22(Chemistry, Physical)

Ultralow thermal conductivity and fast ionic diffusion endow superionic materials with excellent performance both as thermoelectric converters and as solid-state electrolytes. Yet the correlation and interdependence between these two features remain unclear owing to a limited understanding of their complex atomic dynamics. Here we investigate ionic diffusion and lattice dynamics in argyrodite Ag$$_{8}$$SnSe$$_{6}$$ using synchrotron X-ray and neutron scattering techniques along with machine-learned molecular dynamics. We identify a critical interplay of the vibrational dynamics of mobile Ag and a host framework that controls the overdamping of low-energy Ag-dominated phonons into a quasi-elastic response, enabling superionicity. Concomitantly, the persistence of long-wavelength transverse acoustic phonons across the superionic transition challenges a proposed 'liquid-like thermal conduction' picture. Rather, a striking thermal broadening of low-energy phonons, starting even below 50 K, reveals extreme phonon anharmonicity and weak bonding as underlying features of the potential energy surface responsible for the ultralow thermal conductivity ($$<$$ 0.5 Wm$$^{-1}$$K$$^{-1}$$) and fast diffusion. Our results provide fundamental insights into the complex atomic dynamics in superionic materials for energy conversion and storage.

論文

Large collectivity in $$^{29}$$Ne at the boundary of the island of inversion

Revel, A.*; Wu, J.*; 岩崎 弘典*; Ash, J.*; Bazin, D.*; Brown, B. A.*; Chen, J.*; Elder, R.*; Farris, P.*; Gade, A.*; et al.

Physics Letters B, 838, p.137704_1 - 137704_7, 2023/03

 被引用回数:1 パーセンタイル:68.16(Astronomy & Astrophysics)

中性子数20近傍の中性子過剰核は、魔法数20が消滅して原子核が大きく変形していることが知られており、その魔法数が消滅する領域は逆転の島と呼ばれている。$$^{29}$$Neは中性子数19で逆転の島の境界線上に位置するとされてきたが、その変形度は不明だった。ミシガン州立大学の国立サイクロトロン研究所にて$$^{29}$$Neのクーロン励起反応実験を行った結果、931keVの励起状態への$$B(E2)$$値が163$$e^2$$fm$$^4$$と大きな値となり、大きく変形していることが確かめられた。この実験結果をよく使われているいくつかの殻模型計算と比較したところ、大きな$$B(E2)$$値は概ね再現するものの、励起エネルギーの一致は不十分であり、理論の改善が必要であるとわかった。

論文

Two-dimensional quantum universality in the spin-1/2 triangular-lattice quantum antiferromagnet Na$$_{2}$$BaCo(PO$$_{4}$$)$$_{2}$$

Sheng, J.*; Wang, L.*; Candini, A.*; Jiang, W.*; Huang, L.*; Xi, B.*; Zhao, J.*; Ge, H.*; Zhao, N.*; Fu, Y.*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 119(51), p.e2211193119_1 - e2211193119_9, 2022/12

 被引用回数:3 パーセンタイル:28(Multidisciplinary Sciences)

Although considerable progress has been made in the theoretical understanding of the low-dimensional frustrated quantum magnets, experimental realizations of a well-established scaling analysis are still scarce. This is particularly true for the two-dimensional antiferromagnetic triangular lattices. Owing to the small exchange strength, the newly discovered compound Na$$_{2}$$BaCo(PO$$_{4}$$)$$_{2}$$ provides a rare opportunity for clarifying the quantum criticality in an ideal triangular lattice with quantum spin S=1/2. In addition to the establishment of the complete phase diagrams, the spin Hamiltonian with a negligible interplane interaction has been determined through the spin wave dispersion in the polarized state, which is consistent with the observation of a two-dimensional quantum critical point with the Bose-Einstein condensation of diluted free bosons.

論文

Synergistic hybrid electrocatalysts of platinum alloy and single-atom platinum for an efficient and durable oxygen reduction reaction

Liu, B.*; Feng, R.*; Busch, M.*; Wang, S.*; Wu, H.*; Liu, P.*; Gu, J.*; Bahadoran, A.*; 松村 大樹; 辻 卓也; et al.

ACS Nano, 16(9), p.14121 - 14133, 2022/09

 被引用回数:49 パーセンタイル:98.33(Chemistry, Multidisciplinary)

Pt single-atom materials possess an ideal atom economy but suffer from limited intrinsic activity and side reaction of producing H$$_{2}$$O$$_{2}$$ in catalyzing the oxygen reduction reaction (ORR). Here, we demonstrate that anchoring platinum alloys on single-atom Pt-decorated carbon (Pt- SAC) surmounts their inherent deficiencies, thereby enabling a complete four-electron ORR pathway catalysis with high efficiency and durability. Pt$$_{3}$$Co@Pt-SAC demonstrates an exceptional mass and specific activities 1 order of magnitude higher than those of commercial Pt/C. They are durable throughout 50000 cycles, showing only a 10 mV decay in halfwave potential. The superior durability is attributed to the shielding effect of the Pt-SAC coating, which significantly mitigates the dissolution of Pt$$_{3}$$Co cores.

論文

Cross-shell excitations in $$^{46}$$Ca studied with fusion reactions induced by a reaccelerated rare isotope beam

Ash, J.*; 岩崎 弘典*; Mijatovi$'c$, T.*; Budner, T.*; Elder, R.*; Elman, B.*; Friedman, M.*; Gade, A.*; Grinder, M.*; Henderson, J.*; et al.

Physical Review C, 103(5), p.L051302_1 - L051302_6, 2021/05

 被引用回数:3 パーセンタイル:46.8(Physics, Nuclear)

カルシウム同位体は陽子魔法数20を持つため基底状態は球形であるが、変形共存と呼ばれる、数MeV上に変形した状態がある現象が予想されている。回転バンドの存在によってそれが実験的に確かめられるが、$$^{46}$$Caは安定核の融合反応で作るには中性子が多すぎるため、これまで回転バンドの存在が確かめられていなかった。この研究では、ミシガン州立大学の超伝導サイクロトロンにて中性子過剰核$$^{45}$$Kビームを作り、そこから$$^7$$Li($$^{45}$$K,$$alpha 2ngamma$$)$$^{46}$$Ca反応によって$$^{46}$$Caの高スピン状態を生成した。そこからの脱励起ガンマ線の観測により、$$6^+$$までの回転バンドの存在を確立した。そのエネルギー準位は、大規模殻模型計算の予言とよく合うことがわかり、$$^{46}$$Caでも変形共存が起こることが明らかになった。

論文

HPRL; International cooperation to identify and monitor priority nuclear data needs for nuclear applications

Dupont, E.*; Bossant, M.*; Capote, R.*; Carlson, A. D.*; Danon, Y.*; Fleming, M.*; Ge, Z.*; 原田 秀郎; 岩本 修; 岩本 信之; et al.

EPJ Web of Conferences, 239, p.15005_1 - 15005_4, 2020/09

 被引用回数:13 パーセンタイル:99.69(Nuclear Science & Technology)

The OECD-NEA High Priority Request List (HPRL) is a point of reference to guide and stimulate the improvement of nuclear data for nuclear energy and other nuclear applications. The HPRL is application-driven and the requests are submitted by nuclear data users or representatives of the user's communities. A panel of international experts reviews and monitors the requests in the framework of an Expert Group mandated by the NEA Nuclear Science Committee Working Party on International Nuclear Data Evaluation Cooperation (WPEC). After approval, individual requests are divided in two priority categories only, whereas a third category now includes groups of generic requests in a well-defined area (e.g., dosimetry, standard). The HPRL is hosted by the NEA in the form of a relational database publicly available on the web. This contribution provides an overview of HPRL entries, status and outlook. Examples of requests successfully completed will be given and new requests will be described with emphasis on updated nuclear data needs in the fields of nuclear energy, neutron standards, dosimetry, and medical applications.

論文

Shell structure of the neutron-rich isotopes $$^{69,71,73}$$Co

Lokotko, T.*; Leblond, S.*; Lee, J.*; Doornenbal, P.*; Obertelli, A.*; Poves, A.*; Nowacki, F.*; 緒方 一介*; 吉田 数貴; Authelet, G.*; et al.

Physical Review C, 101(3), p.034314_1 - 034314_7, 2020/03

 被引用回数:10 パーセンタイル:69.78(Physics, Nuclear)

中性子過剰核である$$^{69,71,73}$$Coに対する($$p,2p$$)ノックアウト反応が理化学研究所RIBFで測定された。$$gamma-gamma$$ coincidenceの方法で準位構造が決定され、測定された包括的断面積および排他的断面積から暫定的ではあるがスピン・パリティが決定された。殻模型計算との比較により、$$^{69,71,73}$$Coの低励起状態には球形核と変形核が共存することが示唆された。

論文

Passive sweat collection and colorimetric analysis of biomarkers relevant to kidney disorders using a soft microfluidic system

Zhang, Y.*; Guo, H.*; Kim, S. B.*; Wu, Y.*; Ostojich, D.*; Park, S. H.*; Wang, X.*; Weng, Z.*; Li, R.*; Bandodkar, A. J.*; et al.

Lab on a Chip, 19(9), p.1545 - 1555, 2019/05

 被引用回数:139 パーセンタイル:99.63(Biochemical Research Methods)

汗中のバイオマーカーおよび非侵襲的な方法で汗を集める方法は、健康および生理学的状態の評価のための汗利用の関心を生み出し、スポーツから臨床医学までの範囲の潜在的用途がある。本論文は、皮膚密着型のマイクロ流体システムを用いた2つの結果について述べる。(1)簡易な身体的および心理的刺激による汗の採取、(2)酵素化学および比色アプローチによる汗中のクレアチニンおよび尿素の濃度の検出。結果、乳児や高齢者などを対象に日常的で非薬理学的な汗の捕捉が可能になり、腎臓疾患のスクリーニング/モニタリングに汗を使用する可能性が示された。

論文

Nuclear structure of $$^{76}$$Ni from the ($$p$$,$$2p$$) reaction

Elekes, Z.*; Kripk$'o$, $'A$*; Sohler, D.*; Sieja, K.*; 緒方 一介*; 吉田 数貴; Doornenbal, P.*; Obertelli, A.*; Authelet, G.*; 馬場 秀忠*; et al.

Physical Review C, 99(1), p.014312_1 - 014312_7, 2019/01

 被引用回数:10 パーセンタイル:64.15(Physics, Nuclear)

($$p$$,$$2p$$)反応による$$^{76}$$Niの核構造の探索実験を行った。Lenzi, Nowacki, Poves, Sieja相互作用を用いた殻模型計算では実験結果を説明しうる陽子空孔状態が得られており、理論的な断面積計算は実験値とよい一致を与えた。実験で得られたすべての状態を理論的に一意に決定することはできなかったが、過去の実験結果と同様にNi同位体でのZ = 28の大きなshell gapを示す結果が得られた。

論文

A Fluorometric skin-interfaced microfluidic device and smartphone imaging module for ${{it in situ}}$ quantitative analysis of sweat chemistry

関根 由莉奈; Kim, S. B.*; Zhang, Y.*; Bandodkar, A. J.*; Xu, S.*; Choi, J.*; 入江 将大*; Ray, T. R.*; Kohli, P.*; 香西 直文; et al.

Lab on a Chip, 18(15), p.2178 - 2186, 2018/08

近年、スウェットに含まれる代謝産物やイオン等を用いたPoint of Careが高く注目されている。本研究では、それらのバイオマーカーを効果的にその場で検出することを目的として、ソフトで薄いウェアラブルマイクロ流路デバイスとスマートフォンを基盤とした蛍光イメージングシステムを提案する。精密に設計されたマイクロ流路は、皮膚から汗を時間シーケンス制御で集めることを可能にした。また、集められた汗から蛍光検出剤によって検出された塩化物,ナトリウム,亜鉛濃度をスマートフォンを基盤とした蛍光イメージングシステムで正確に定量分析することに成功した。このシステムを実際に試験したところ、正確に効率よく作動することを確認した。

論文

Atomically dispersed Pt on the surface of Ni particles; Synthesis and catalytic function in hydrogen generation from aqueous ammonia-borane

Li, Z.*; He, T.*; 松村 大樹; Miao, S.*; Wu, A.*; Liu, L.*; Wu, G.*; Chen, P.*

ACS Catalysis, 7(10), p.6762 - 6769, 2017/10

 被引用回数:158 パーセンタイル:96.49(Chemistry, Physical)

We report herein that the single-atom alloy (SAA) made of atomically dispersed Pt on the surface of Ni particles (Pt is surrounded by Ni atoms) exhibits improved catalytic activity on the hydrolytic dehydrogenation of ammonia-borane, a promising hydrogen storage method for onboard applications. Specifically, an addition of 160 ppm of Pt leads to ca. 3-fold activity improvement in comparison to that of pristine Ni/CNT catalyst. The turnover frequency based on the isolated Pt is 12000 mol$$_{rm{H}2}$$ mol$$_{rm{Pt}}$$$$^{-1}$$ min$$^{-1}$$, which is about 21 times the value of the best Pt-based catalyst ever reported. Our simulation results indicate that the high activity achieved stems from the synergistic effect between Pt and Ni, where the negatively charged Pt (Pt$$^{delta -}$$) and positively charged Ni (Ni$$^{delta +}$$) in the Pt-Ni alloy are prone to interact with H and OH of H$$_{2}$$O molecules, respectively, leading to an energetically favorable reaction pathway.

論文

Shell evolution beyond $$Z$$=28 and $$N$$=50; Spectroscopy of $$^{81,82,83,84}$$Zn

Shand, C. M.*; Podoly$'a$k, Zs.*; G$'o$rska, M.*; Doornenbal, P.*; Obertelli, A.*; Nowacki, F.*; Otsuka, T.*; Sieja, K.*; Tostevin, J. A.*; Tsunoda, T.*; et al.

Physics Letters B, 773, p.492 - 497, 2017/10

 被引用回数:25 パーセンタイル:87.36(Astronomy & Astrophysics)

Low-lying states in neutron-rich $$^{81,82.83.84}$$Zn nuclei were measured for the first time via in-beam $$gamma$$-ray spectroscopy at RIKEN. These include the 4$$_1^+$$ to 2$$_1^+$$ in $$^{82}$$Zn and the 2$$_1^+$$ to 0$$_1^+$$ and 4$$_1^+$$ to 2$$_1^+$$ in $$^{84}$$Zn. The reduced E($$2^+$$) energies and increased E(4$$^+$$)/E(2$$^+$$) ratios at $$N$$=52,54 compared to $$^{80}$$Zn attest that the magicity is confined just on the neutron number $$N$$=50 only. The levels observed in $$^{84}$$Zn suggest the onset of deformation towards heavier Zn isotopes. The data were compared to state-of-the-art shell model calculations.

論文

Observation of a $$gamma$$-decaying millisecond isomeric state in $$^{128}$$Cd$$_{80}$$

Jungclaus, A.*; Grawe, H.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Simpson, G. S.*; S$"o$derstr$"o$m, P.-A.*; 炭竃 聡之*; Taprogge, J.*; Xu, Z. Y.*; et al.

Physics Letters B, 772, p.483 - 488, 2017/09

 被引用回数:8 パーセンタイル:55.37(Astronomy & Astrophysics)

A new high-spin isomer in the neutron-rich nucleus $$^{128}$$Cd was populated in the projectile fission of a $$^{238}$$U beam at the Radioactive Isotope Beam Factory at RIKEN. A half-life of T$$_{1/2}$$ = 6.3(8) ms was measured for the new state which was tentatively assigned a spin/parity of (15$$^-$$). The isomeric state decays via the emission of a 309-keV $$gamma$$ ray with $$E3$$ multipolarity. The experimental results are compared to shell model calculations performed using state-of-the-art realistic effective interactions and to the neighbouring nucleus $$^{129}$$Cd. The comparison with calculations shows that adjustments of the pairing and multipole parts of the effective interaction derived from the CD-Bonn nucleon-nucleon potential are required in order to describe the properties of nuclei in the region around $$^{132}$$Sn.

論文

Type II shell evolution in $$A=70$$ isobars from the $$N geq 40$$ island of inversion

Morales, A. I.*; Benzoni, G.*; Watanabe, H.*; 角田 佑介*; Otsuka, T.*; 西村 俊二*; Browne, F.*; Daido, R.*; Doornenbal, P.*; Fang, Y.*; et al.

Physics Letters B, 765, p.328 - 333, 2017/02

 被引用回数:34 パーセンタイル:91.97(Astronomy & Astrophysics)

The level schemes of neutron-rich isotopes $$^{70}$$Co and $$^{70}$$Ni were populated in the $$beta$$ decay of $$^{70}$$Fe and studied using $$beta$$-delayed $$gamma$$-ray spectroscopy of the $$beta$$ decay, at the RIBF in RIKEN, Japan. The experimental results were compared to state-of-the-art shell-model calculations, and indicate a dominance of prolate deformation in the low-lying states, coexisting with spherical states. The $$beta$$ decay of the $$A=70$$ isobars is shown to progress in accordance to a new type of shell evolution, the so-called Type II, which involves many particle-hole excitations across energy gaps.

論文

$$beta$$ decay of semi-magic $$^{130}$$Cd; Revision and extension of the level scheme of $$^{130}$$In

Jungclaus, A.*; Grawe, H.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Simpson, G. S.*; S$"o$derstr$"o$m, P. A.*; 炭竃 聡之*; Taprogge, J.*; Xu, Z. Y.*; et al.

Physical Review C, 94(2), p.024303_1 - 024303_8, 2016/08

 被引用回数:18 パーセンタイル:77.39(Physics, Nuclear)

The $$beta$$ decay of the semi-magic nucleus $$^{130}$$Cd has been studied at the RIBF facility at the RIKEN Nishina Center. The high statistics of the present experiment allowed for a revision of the established level scheme of $$^{130}$$In and the observation of additional $$beta$$ feeding to high lying core-excited states in $$^{130}$$In. The experimental results are compared to shell-model calculations employing a model space consisting of the full major $$N=50-82$$ neutron and $$Z=28-50$$ proton shells, and good agreement is found.

論文

First observation of $$gamma$$ rays emitted from excited states south-east of $$^{132}$$Sn; The $$pi$$ g$$_{9/2}^{-1}$$ $$ otimes$$ $$nu f_{7/2}$$ multiplet of $$^{132}$$In$$_{83}$$

Jungclaus, A.*; Gargano, A.*; Grawe, H.*; Taprogge, J.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Shimizu, Y.*; Simpson, G. S.*; S$"o$derstr$"o$m, P.-A.*; et al.

Physical Review C, 93(4), p.041301_1 - 041301_6, 2016/04

 被引用回数:18 パーセンタイル:77.39(Physics, Nuclear)

For the first time, the decay of excited states in a nucleus situated "south-east" of $$^{132}$$Sn have been observed, in a region where experimental information is limited to ground-state properties. Six $$gamma$$ rays from $$^{133}$$Cd, produced in the fragmentation of a $$^{238}$$U beam at RIBF at RIKEN. The $$gamma$$ rays were studied using the EURICA array of Ge detectors. The new experimental information is compared to results from realistic shell-model calculations, which are the first in this region far from stability. Comparison with calculations suggests that at least four out of six new transitions can be attributed to the particle-hole configuration of one neutron in the $$f_{7/2}$$ and one proton hole in the $$g_{9/2}$$ orbits, respectively. This work constitutes an important first step towards the exploration of nuclear structure in this unknown region of the nuclear chart.

論文

Low-lying excitations in $$^{72}$$Ni

Morales, A. I.*; Benzoni, G.*; Watanabe, H.*; 西村 俊二*; Browne, F.*; Daido, R.*; Doornenbal, P.*; Fang, Y.*; Lorusso, G.*; Patel, Z.*; et al.

Physical Review C, 93(3), p.034328_1 - 034328_14, 2016/03

 被引用回数:25 パーセンタイル:85.25(Physics, Nuclear)

Low-lying excited states in $$^{72}$$Ni have been investigated at RIKEN by studying the $$beta$$ decay of $$^{72}$$Co to $$^{72}$$Ni. $$^{72}$$Co was separated with BigRIPS, implanted into the WaS3ABi Silicon array, and the $$gamma$$ ray measured using the EURICA $$gamma$$ spectrometer. From the analysis, 60 new $$gamma$$-ray transitions and 21 new levels in $$^{72}$$Ni were observed. The new experimental information is compared to shell-model calculations which include neutron excitation across the $$fpg$$ shell. The calculations reproduce rather well the observed states, implying that a clear understanding of these low-lying excitations has been achieved.

論文

Decay properties of $$^{68,69,70}$$Mn; Probing collectivity up to N=44 in Fe isotopic chain

Benzoni, G.*; Morales, A. I.*; Watanabe, H.*; 西村 俊二*; Coraggio, L.*; Itaco, N.*; Gargano, A.*; Browne, F.*; Daido, R.*; Doornenbal, P.*; et al.

Physics Letters B, 751, p.107 - 112, 2015/12

 被引用回数:20 パーセンタイル:78.02(Astronomy & Astrophysics)

The $$beta$$ decays of $$^{68,69,70}$$Mn have been measured at the RIBF facility at RIKEN using the EURICA $$gamma$$ spectrometer combined with an active stopper consisting of a stack of Si detectors. Half-lives and $$beta$$-delayed neutron emission probabilities have been extracted for these decays, together with first experimental information on excited states populated in $$^{69,70}$$Fe. The data indicate a continuously increasing deformation for Fe isotopes up to A=70, and interpreted to be due to the interplay between quadrupole correlation of specific neutron orbitals and the monopole component of the proton-neutron interaction.

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